Photovoltaic effect in ferroelectrics

Cai Tian-Yi; Ju Sheng

doi:10.7498/aps.67.20180979

Abstract

Ferroelectric oxides are attractive materials for constructing efficient solar cells. The mechanism includes the anomalous photovoltaic effect (APE) and the bulk photovoltaic effect (BPE). The BPE refers to the generation of a steady photocurrent and above-bandgap photovoltage in a single-phase homogeneous material lacking inversion symmetry. The mechanism of BPE is different from the typical p-n junction-based photovoltaic mechanism in heterogeneous materials. We survey the history, development and recent progress in understanding the mechanisms of BPE, with a focus on the shift current mechanism, an intrinsic BPE that is universal to all materials lacking inversion symmetry. We also review the important factors to the APE, i.e., the domain boundary, the Schottcky junction, and the depolarization field. The recent successful applications of inorganic and hybrid perovskite structured materials in solar cells emphasize that ferroelectrics can be used in conventional photovoltaic architectures. We review the development in this field, with a particular emphasis on the perovskite materials and the theoretical explanations. In addition to discussing the implication of a ferroelectric absorber layer and the solid state theory of polarization, the design principles and prospect for high-efficiency ferroelectric photovoltaics are also mentioned. Considering the coupling between the degrees of freedom, some special ferroelectrics are expected to have prominent multi-functionality. With the introduction of the additional degree of freedom, some ferroelectrics, i.e., ScFexCr1-xO3 (1/6 x 5/6), can be a promising candidate for highly efficient solar cells and spin photovoltaic devices.

Keywords:

Authors and contacts

1.
School of Physical Science and Technology, Soochow University, Suzhou 215006, China

Corresponding author: Cai Tian-Yi, caitianyi@suda.edu.cn;jusheng@suda.edu.cn ; Ju Sheng, caitianyi@suda.edu.cn;jusheng@suda.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 11374220, 11204193), the National Basic Research Program of China (Grant No. 2014CB920900), the Qinlan Project of Jiangsu Province, and the Dongwu Scholar Project of Soochow University.

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Cited By

[1]	Green M A, Bremner S P 2017 Nat. Mater. 16 23
[2]	Chapin D M, Fuller C S, Pearson G L A 1954 J. Appl. Phys. 25 676
[3]	Shockley W, Queisser H J 1961 J. Appl. Phys. 32 510
[4]	Lopez N, Reichertz L A, Yu K M 2011 Phys. Rev. Lett. 106 028701
[5]	Jackson E D 1958 Trans Conf. Use Solar Energy 5 122
[6]	Green M A, Keevers M J, Thomas I, Lasich J B, Emery K 2015 Prog. Photovolt. 23 685
[7]	Fridkin V M 1979 Photoferroelectrics (Berlin: Springer-Verlag)
[8]	King-Smith R D, Vanderbilt D 1993 Phys. Rev. B 47 1651
[9]	Seidel J, Eng L M 2014 Curr. Appl. Phys. 14 1083
[10]	Bulter K T, Frost J M, Walsh A 2015 Energy Environ. Sci. 8 838
[11]	Hu Z, Tian M, Nysten B, Jonas A M 2009 Nat. Mater. 8 62
[12]	Scott J F 2007 Science 315 954
[13]	Garcia V, Bibes M 2012 Nature 483 279
[14]	Lee D, Yang S M, Kim T H, Jeon B C, Kim Y S, Yoon J G, Lee H N, Baek S H, Eom C B, Noh T W 2012 Adv. Mater. 24 402
[15]	Dong S, Liu J M, Cheong S W, Ren Z 2015 Adv. Phys. 64 519
[16]	Garcia V, Bibes M, Bocher L, Valencia S, Kronast F, Crassous A, Moya X, Enouz-Vedrenne S, Gloter A, Imhoff D, Deranlot C, Mathur N D, Fusil S, Bouzehouane K, Barthlmy A 2010 Science 327 1106
[17]	Ramesh R 2010 Nat. Mater. 9 380
[18]	Meyerheim H L, Klimenta F, Ernst A, Mohseni K, Ostanin S, Fechner M, Parihar S, Maznichenko I V, Mertig I, Kirschner J 2011 Phys. Rev. Lett. 106 087203
[19]	Cai T Y, Ju S, Sun H, Li Z Y 2008 Prog. Phys. 1 50 (in Chinese) [蔡田怡, 雎胜, 孙华, 李振亚 2008 物理学进展 1 50]
[20]	Weng Y K, Lin L F, Dagotto E, Dong S 2016 Phys. Rev. Lett. 117 037601
[21]	Cai T Y, Ju S, Lee J, Sai N, Demkov A A, Niu Q, Li Z Y, Shi J R, Wang E G 2009 Phys. Rev. B 80 140415
[22]	Cai T Y, Liu S C, Ju S, Liu C Y, Guo G Y 2017 Phys. Rev. Appl. 8 034034
[23]	Yuan Y, Xiao Z, Yang B, Huang J 2014 J. Mater. Chem. A 2 6027
[24]	Tan L Z, Zheng F, Young S M, Wang F, Liu S, Rappe A M 2016 npj Comput. Mater. 2 16026
[25]	Yang S Y, Seidel J, Byrnes S J, Shafer P, Yang C H, Rossell M D, Yu P, Chu Y H, Scott J F, Ager Ⅲ J W, Martin L W, Ramesh R 2010 Nat. Nanotechnol. 5 143
[26]	Young S M, Rappe A M 2012 Phys. Rev. Lett. 109 116601
[27]	Grinberg I, West D V, Torres M, Gou G, Stein D M, Wu L, Chen G, Gallo E M, Akbashev A R, Davies P K, Spanier J E, Rappe A M 2013 Nature 503 509
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[34]	Park N G 2013 J. Phys. Chem. Lett. 4 2423
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[36]	Bhachu D, Scanlon D, Saban E, Bronstein H, Parkin I, Carmalt C, Palgrave R 2015 J. Mater. Chem. A 3 9071
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Vol. 67, Issue 15 - 2018-08-05

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