Thermal effect of translucent gold nanofilm based on transient reflection/transmission technique

Wu Wen-Zhi; Gao Lai-Xu; Kong De-Gui; Gao Yang; Ran Ling-Ling; Chai Zhi-Jun

doi:10.7498/aps.65.046801

Abstract

In this work, the relaxation dynamics of optically excited electrons and lattice in translucent gold nanofilms is measured with femtosecond transient reflection and transmission technique. In order to investigate the mechanisms of heat transfer in metal nanofilm theoretically, the two-temperature model and the Crude-model approximation are used to estimate the profile of decays and the temperature of electrons and lattice. Ultrafast relaxation dynamics of gold nanofilm 60 nm in thickness is different obviously in transient reflection and transmission measurements. Electron-lattice coupling effect in the transmission method is stronger and more sensitive than that in the reflection method under the same experimental conditions. Gradient change of temperature along the direction of film thickness and interface thermal resistance due to the boundary scattering should be responsible for the difference between them. Experimental data suggest that both transient reflection and transient transmission of translucent films should be considered together in the investigation on the mechanism of heat transfer. With increasing energy of pump laser pulse, the rise time is about 1.0 ps, and the electron-lattice relaxation time becomes longer.

Keywords:

Authors and contacts

1.
School of Electronic Engineering, Heilongjiang University, Harbin 150080, China

Corresponding author: Wu Wen-Zhi, wuwenzhi@hlju.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 61204007), the New-Century Training Programme Foundation for the Talents by Heilongjiang Province, China (Grant No. 1254-NCET-018), the Foundation for University Key Teacher by Heilongjiang University, China (Grant No. 1252G047), the Heilongjiang Province Postdoctoral Science Foundation, China (Grant No. LBH-Q14139), and the Science Fund of Heilongjiang University for Young Scholars, China (Grant Nos. JCL201205, QL201211).

References

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[22]	Hostetler J L, Smith A N, Czajkowsky D M, Norris P M 1999 Appl. Opt. 38 3614
[23]	Guo L, Xu X F 2014 J. Heat Transfer 136 122401
[24]	Carpene E 2006 Phys. Rev. B 74 024301
[25]	Lioudakis E, Othonos A, Dimakis E, Iliopoulos E, Georgakilas A 2006 Appl. Phys. Lett. 88 121128
[26]	Schoenlein R W, Lin W Z, Fujimoto J G, Eesley G L 1987 Phys. Rev. Lett. 58 1680
[27]	Garduno-Mejia J, Higlett M P, Meech S R 2007 Chem. Phys. 341 276
[28]	Conforti M, Valle G D 2012 Phys. Rev. B 85 245423
[29]	Sun C K, Vallee F, Acioli L H, Ippen E P, Fujimoto J G 1994 Phys. Rev. B 50 15337
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[32]	Yang Q, Du G Q, Chen F, Wu Y M, Si J H, Hou X 2014 Chin. J. Lasers 41 502005 (in Chinese) [杨青, 杜广庆, 陈烽, 吴艳敏, 司金海, 侯洵2014 中国激光 41 502005]

Cited By

[1]	Zhang C W, Bi K D, Wang J L, Ni Z H, Chen Y F 2012 Sci. China Tech. Sci. 55 1044 (in Chinese) [张春伟, 毕可东, 王建立, 倪中华, 陈云飞 2012 中国科学:技术科学 55 1044]
[2]	SmithA N, HostetlerJ L, Norris P M 1999 Numerical Heat Transfer Part A 35 859
[3]	Nielsen J B, Savolainen J M, Christensen M S, Balling P 2011 Appl. Phys. A 103 447
[4]	Du G Q, Yang Q, Chen F, Ou Y, Wu Y M, Hou X 2015 Int. J. Thermal Sci. 90 197
[5]	Li Q, Lao H Y, Lin J, Chen Y P, Chen X F 2011 Appl. Phys. A 105 125
[6]	Du G Q, Yang Q, Chen F, Ou Y, Wu Y M, Lu Y, Bian H, Hou X 2014 Chem. Phys. Lett. 597 153
[7]	Chen J, Chen W K, Tang J, Rentzepis P M 2011 Proc. Nat. Acad. Sci. USA 108 18887
[8]	Rotenberg N, Bristow A D, Pfeiffer M, Betz M, van Driel H M 2007 Phys. Rev. B 75 155426
[9]	Guo L, Hodson S L, Fisher T S, Xu X F 2012 J. Heat Transfer 134 042402
[10]	Wang B L,Wang R, Liu R J, Lu X H, Zhao J M, Li Z Y 2013 Sci. Rep. 3 2358
[11]	Venkatakrishnan K, Tan B, Ngoi B K A 2002 Opt. Laser Technol. 34 199
[12]	Wang H D, Ma W G, Zhang X, Wang W 2010 Acta Phys. Sin. 59 3856 (in Chinese) [王海东, 马维刚, 张兴, 王玮 2010 59 3856]
[13]	Zhu L D, Sun F Y, Zhu J, Tang D W 2012 Acta Phys. Sin. 61 130512 (in Chinese) [朱丽丹, 孙方远, 祝捷, 唐大伟 2012 61 130512]
[14]	Anisimov S, Kapeliovich B, Perelman T 1974 Soviet Phys. JETP 39 375
[15]	Elsayed-Ali H E, Norris T B, Pessot M A, MourouG A 1987 Phys. Rev. Lett. 58 1212
[16]	Fang R R, Wei H, Li Z H, Zhang D M 2012 Solid State Commun. 152 108
[17]	Li S Q, Ye H A, Liu C Y, Dou Y F, Huang Y 2013 Chin. Phys. B 22 077302
[18]	Hohlfeld J, Wellershoff S S, Gudde J, Conrad U, Jahnke V, Matthias E 2000 Chem. Phys. 251 237
[19]	Hopkins P E, Kassebaum J L, Norris P M 2009 J. Appl. Phys. 105 023710
[20]	Jesus G M, Michael P H, Stephen R M 2008 Surf. Sci. 602 3125
[21]	Bonn M, Denzler D N, Funk S, Wolf M, Wellershoff S S, Hohlfeld J 2000 Phys. Rev. B 61 1101
[22]	Hostetler J L, Smith A N, Czajkowsky D M, Norris P M 1999 Appl. Opt. 38 3614
[23]	Guo L, Xu X F 2014 J. Heat Transfer 136 122401
[24]	Carpene E 2006 Phys. Rev. B 74 024301
[25]	Lioudakis E, Othonos A, Dimakis E, Iliopoulos E, Georgakilas A 2006 Appl. Phys. Lett. 88 121128
[26]	Schoenlein R W, Lin W Z, Fujimoto J G, Eesley G L 1987 Phys. Rev. Lett. 58 1680
[27]	Garduno-Mejia J, Higlett M P, Meech S R 2007 Chem. Phys. 341 276
[28]	Conforti M, Valle G D 2012 Phys. Rev. B 85 245423
[29]	Sun C K, Vallee F, Acioli L H, Ippen E P, Fujimoto J G 1994 Phys. Rev. B 50 15337
[30]	Sun C K, Vallee F, Acioli L, Ippen E P, Fujimoto J G 1993 Phys. Rev. B 48 12365
[31]	Hopkins P E, Norris P M 2007 Appl. Surf. Sci. 253 6289
[32]	Yang Q, Du G Q, Chen F, Wu Y M, Si J H, Hou X 2014 Chin. J. Lasers 41 502005 (in Chinese) [杨青, 杜广庆, 陈烽, 吴艳敏, 司金海, 侯洵2014 中国激光 41 502005]

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Vol. 65, Issue 4 - 2016-02-20

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