Recent advances in planar heterojunction organic-inorganic hybrid perovskite solar cells

Wang Fu-Zhi; Tan Zhan-Ao; Dai Song-Yuan; Li Yong-Fang

doi:10.7498/aps.64.038401

Abstract

The development of highly efficient and low-cost solar cells is the key to large-scale application of solar photovoltaic technology. In recent years, the solution-processed organic-inorganic perovskite solar cells attracted considerable attention because of their advantages of high energy conversion efficiency, low cost, and ease of processing. The ambipolar semiconducting characteristic of perovskite enables the construction of planar heterojunction architecture to be possible in perovskite-based solar cells. This kind of architecture avoids the use of mesoporous metal oxide film, which simplifies the processing route and makes it easier to fabricate flexible and tandem perovskite-based solar cells. Planar heterojunction perovskite solar cells can be divided into n-i-p type and p-i-n type according to the charge flow direction. Two interfaces are formed between perovskite film and hole/electron transport layer, where efficient charge separation can be realized. Hole and electron transport layers can form separated continuous paths for the transport of holes and electrons, thus beneficial to improving exciton separation, charge transportation, and collection efficiency. In addition, this planar architecture avoids the use of high temperature sintered mesoporous metal oxide framework; this is beneficial to expanding the choice of the charge transport materials. In this paper, we review the recent progress on the planar heterojunction perovskite solar cells. First, we introduce the material properties of perovskite, the evolution of device architecture, and the working principle of p-i-n type and n-i-p type planar heterojunction perovskite solar cells. Then, we review the recent progress and optimization of planar heterojunction perovskite solar cells from every aspect of perovskite preparation and the selection of electron/hole transport materials. Finally, we would like to give a perspective view on and address the concerns about perovskite solar cells.

Keywords:

Authors and contacts

1.
Beijing Key Laboratory of Novel Thin Film Solar Cells, School of Renewable Energy, North China Electric Power University, Beijing 102206, China;
2.
Beijing Key Laboratory of Energy Security and Clean Utilization, North China Electric Power University, Beijing 102206, China;
3.
Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 51173040, 91023039, 51303052), the Specialized Research Fund for the Doctoral Program (Grant No. 20130036110007), the Program for New Century Excellent Talents in University of China (Grant No. NCET-12-0848), Beijing Higher Education Young Elite Program (Grant No. YETP0713), and the Fundamental Research Funds for the Central Universities, China (Grant Nos. 13ZD11, 2014ZD11, 2014MS35, 2014ZZD07).

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Cited By

[1]	Yella A, Lee H W, Tsao H N, Yi C, Chandiran A K, Nazeeruddin M K, Diau E W, Yeh C Y, Zakeeruddin S M, Grätzel M 2011 Science 334 629
[2]	Mathew S, Yella A, Gao P, Humphry-Baker R, CurchodBasile F E, Ashari-Astani N, Tavernelli I, Rothlisberger U, NazeeruddinMd K, Grätzel M 2014 Nat. Chem. 6 242
[3]	Kojima A, Teshima K, Shirai Y, Miyasaka T 2009 J. Am. Chem. Soc. 131 6050
[4]	Burschka J, Pellet N, Moon S J, Humphry-Baker R, Gao P, Nazeeruddin M K, Grätzel M 2013 Nature 499 316
[5]	Liu M, Johnston M B, Snaith H J 2013 Nature 501 395
[6]	Zhou H, Chen Q, Li G, Luo S, Song T B, Duan H S, Hong Z, You J, Liu Y, Yang Y 2014 Science 345 542
[7]	Albert V A, Barbazuk W B, dePamphilis C W, Der J P, Leebens-Mack J, Ma H, Palmer J D, Rounsley S, Sankoff D, Schuster S C, Soltis D E, Soltis P S, Wessler S R, Wing R A, Albert V A, Ammiraju J S, Barbazuk W B, Chamala S, Chanderbali A S, dePamphilis C W, Der J P, Determann R, Leebens-Mack J, Ma H, Ralph P, Rounsley S, Schuster S C, Soltis D E, Soltis P S, Talag J, Tomsho L, Walts B, Wanke S, Wing R A, Albert V A, Barbazuk W B, Chamala S, Chanderbali A S, Chang T H, Determann R, Lan T, Soltis D E, Soltis P S, Arikit S, Axtell M J, Ayyampalayam S, Barbazuk W B, Burnette J M 3rd, Chamala S, De Paoli E, dePamphilis C W, Der J P, Estill J C, Farrell N P, Harkess A, Jiao Y, Leebens-Mack J, Liu K, Mei W, Meyers B C, Shahid S, Wafula E, Walts B, Wessler S R, Zhai J, Zhang X, Albert V A, Carretero-Paulet L, dePamphilis C W, Der J P, Jiao Y, Leebens-Mack J, Lyons E, Sankoff D, Tang H, Wafula E, Zheng C, Albert V A, Altman N S, Barbazuk W B, Carretero-Paulet L, dePamphilis C W, Der J P, Estill J C, Jiao Y, Leebens-Mack J, Liu K, Mei W, Wafula E, Altman NS, Arikit S, Axtell M J, Chamala S, Chanderbali A S, Chen F, Chen J Q, Chiang V, De Paoli E, dePamphilis C W, Der J P, Determann R, Fogliani B, Guo C, Harholt J, Harkess A, Job C, Job D, Kim S, Kong H, Leebens-Mack J, Li G, Li L, Liu J, Ma H, Meyers B C, Park J, Qi X, Rajjou L, Burtet-Sarramegna V, Sederoff R, Shahid S, Soltis D E, Soltis P S, Sun Y H, Ulvskov P, Villegente M, Xue J Y, Yeh T F, Yu X, Zhai J, Acosta J J, Albert VA, Barbazuk W B, Bruenn R A, Chamala S, de Kochko A, dePamphilis C W, Der JP, Herrera-Estrella LR, Ibarra-Laclette E, Kirst M, Leebens-Mack J, Pissis S P, Poncet V, Schuster S C, Soltis D E, Soltis P S, Tomsho L 2013 Science 342 1438
[8]	Kim H S, Im S H, Park N G 2014 J. Phys. Chem. C 118 5615
[9]	Sun S, Salim T, Mathews N, Duchamp M, Boothroyd C, Xing G, Sum T C, Lam Y M 2014 Energ. Environ. Sci. 7 399
[10]	Tanaka K, Takahashi T, Ban T, Kondo T, Uchida K, Miura N 2003 Solid State Commun. 127 619
[11]	Stoumpos C C, Malliakas C D, Kanatzidis M G 2013 Inorg. Chem. 52 9019
[12]	Stranks S D, Eperon G E, Grancini G, Menelaou C, Alcocer M J P, Leijtens T, Herz L M, Petrozza A, Snaith H J 2013 Science 342 341
[13]	Baikie T, Fang Y, Kadro J M, Schreyer M, Wei F, Mhaisalkar S G, Graetzel M, White T J 2013 J. Mater. Chem. A 1 5628
[14]	Lee M M, Teuscher J, Miyasaka T, Murakami T N, Snaith H J 2012 Science 338 643
[15]	Edri E, Kirmayer S, Cahen D, Hodes G 2013 J. Phys. Chem. Lett. 4 897
[16]	Wojciechowski K, Saliba M, Leijtens T, Abate A, Snaith H J 2014 Energ. Environ. Sci. 7 1142
[17]	Xiao M, Huang F, Huang W, Dkhissi Y, Zhu Y, Etheridge J, Gray-Weale A, Bach U, Cheng Y B, Spiccia L 2014 Angew. Chem. Int. Ed. Engl. 53 9898
[18]	Im J H, Lee C R, Lee J W, Park S W, Park N G 2011 Nanoscale 3 4088
[19]	Kim H S, Lee C R, Im J H, Lee K B, Moehl T, Marchioro A, Moon S J, Humphry-Baker R, Yum J H, Moser J E 2012 Sci. Rep. 2 591
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Vol. 64, Issue 3 - 2015-02-05

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