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As the first safety barrier of high level radioactive waste, the tolerance to radiation of vitrification is critical. Vitrification is a kind of specialized glass used as the package of high-level radioactive waste in nuclear power industry. Because of its structural consistency with the main structure of vitrification (silicon-oxygen tetrahedron), fused silica is used to study the irradiation effect on network of vitrification in the present study. Borosilicate glass, a simplified version of vitrification, is studied under the same conditions for comparison. Hardness values, moduli and refractive indexes of fused silica and borosilicate glass are measured before and after irradiation with nanoindentation technology and elliptic polarization instrument. It is shown in this study that the hardness values of fused silica and borosilicate glass decrease with increasing dose. On the other hand, with dose increasing, the modulus of borosilicate glass decreases but the modulus of silica increases. Change in modulus might be attributed to the change of density, which is consistent with results from the refractive index.
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Keywords:
- fused silica /
- borosilicate glass /
- effect of irradiation
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[2] Weber W J 1988 Nucl. Instrum. Meth. B 32 471
[3] Weber W J, Ewing R C, Angell C A, Arnold G W, Cormack A N, Delaye J M, Griscom D L, Hobbs L W, Navrotsky A, Price D L, Stoneham A M, Weinberg M C 1997 J. Mater. Res. 12 1948
[4] Peuget S, Fares T, Maugeri E A, Caraballo R, Charpentier T, Martel L, Somers J, Janssen A, Wiss T, Rozenblum F, Magnin M, Deschanels X, Jgou C 2014 Nucl. Instrum. Meth. B 327 22
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[6] Peuget S, Delaye J M, Jgou C 2014 J. Nucl. Mater. 444 76
[7] Peuget S, Broudic V, Jgou C, Frugier P, Roudil D, Deschanels X, Rabiller H, Noel P 2007 J. Nucl. Mater. 362 474
[8] Ollier N, Champagnon B, Boizot B, Guyot Y, Panczer G, Padlyak B 2003 J. Non-Cryst. Solids 323 200
[9] Ollier N, Boizot B, Reynard B, Ghaleb D, Petite G 2005 J. Nucl. Mater. 340 209
[10] Ollier N, Boizot B, Reynard B, Ghaleb D, Petite G 2004 Nucl. Instrum. Meth. B 218 176
[11] Mohapatra M, Kadam R M, Mishra R K, Kaushik C P, Tomar B S, Godbole S V 2011 Physica B 406 3980
[12] Mohapatra M, Kadam R M, Mishra R K, Dutta D, Pujari P K, Kaushik C P, Kshirsagar R J, Tomar B S, Godbole S V 2011 Nucl. Instrum. Meth. B 269 2057
[13] Mohapatra M, Manchanda V K 2009 IOP Conf. Ser.: Mater. Sci. Eng. 2 012022
[14] Yang K J, Wang T S, Zhang G F, Peng H B, Chen L, Zhang L M, Li C X, Tian F, Yuan W 2013 Nucl. Instrum. Meth. B 307 541
[15] Zhang G F, Wang T S, Yang K J, Chen L, Zhang L M, Peng H B, Yuan W, Tian F 2013 Nucl. Instrum. Meth. B 316 218
[16] Chen L, Wang T S, Yang K J, Peng H B, Zhang G F, Zhang L M, Jiang H, Wang Q 2013 Nucl. Instrum. Meth. B 307 566
[17] Chen L, Yuan W, Nan S, Du X, Zhang D F, L P, Peng H B, Wang T S 2016 Nucl. Instrum. Meth. B 370 42
[18] Peng H B, Sun M L, Yang K J, Chen H, Yang D, Yuan W, Chen L, Duan B H, Wang T S 2016 J. Non-Cryst. Solids 443 143
[19] Wang T S, Duan B H, Tian F, Peng H B, Chen L, Zhang L M, Yuan W 2015 Chin. Phys. B 24 076102
[20] Wang T S, Du X, Yuan W, Duan B H, Zhang J D, Chen L, Peng H B, Yang D, Zhang G F, Zhu Z H 2016 Surf. Coat. Technol. 306 245
[21] Karakurt G, Abdelouas A, Guin J P, Nivard M, Sauvage T, Paris M, Bardeau J F 2016 J. Nucl. Mater. 475 243
[22] Inagaki Y, Furuya H, Idemitsu K, Banba Y, Matsumoto S, Muraoka S 1991 Mater. Res. Soc. Symp. Proc. 257 199
[23] Mir A H, Monnet I, Toulemonde M, Bouffard S, Jegou C, Peuget S 2016 J. Nucl. Mater. 469 244
[24] Mir A H, Toulemonde M, Jegou C, Miro S, Serruys Y, Bouffard S, Peuget S 2016 Sci. Rep. 6 30191
[25] Routbort J L, Matzke H 1983 J. Mater. Sci. Eng. 58 229
[26] Joslin D L, Oliver W C 1990 J. Mater. Res. 5 123
[27] Zhu D R, Lai T S 1997 Acta Sci. Natur. Univ. 36 31 (in Chinese) [朱德瑞, 赖天树 1997 中山大学学报 (自然科学版) 36 31]
[28] Peng H, Sun M, Du X, Yuan W, Yang D, Chen L, Duan B, Wang T 2017 Nucl. Instrum. Meth. B 406 561
[29] Peuget S, Cachia J N, Jgou C, Deschanels X, Roudil D, Broudic V, Delaye J M, Bart J M 2006 J. Nucl. Mater. 354 1
[30] Arndt J, Devine R A B, Revesz A G 1991 J. Non-Cryst. Solids 131-133 1206
[31] Arndt J, Stffler D 1969 Phys. Chem. Glasses 10 117
[32] Makishima A, Mackenzie J 1973 J. Non-Cryst. Solids 12 35
[33] Chi Y S, Shen J Y, Chen X X, Miu Z X 2002 J. Inorg. Mater. 17 475 (in Chinese) [迟玉山, 沈菊云, 陈学贤, 缪之训 2002 无机材料学报 17 475]
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[1] Weber W J, Matzke H, Routort J L 1984 J. Mater. Sci. 19 2533
[2] Weber W J 1988 Nucl. Instrum. Meth. B 32 471
[3] Weber W J, Ewing R C, Angell C A, Arnold G W, Cormack A N, Delaye J M, Griscom D L, Hobbs L W, Navrotsky A, Price D L, Stoneham A M, Weinberg M C 1997 J. Mater. Res. 12 1948
[4] Peuget S, Fares T, Maugeri E A, Caraballo R, Charpentier T, Martel L, Somers J, Janssen A, Wiss T, Rozenblum F, Magnin M, Deschanels X, Jgou C 2014 Nucl. Instrum. Meth. B 327 22
[5] Peuget S, Nol P Y, Loubet J L, Pavan S, Nivet P, Chenet A 2006 Nucl. Instrum. Meth. B 246 379
[6] Peuget S, Delaye J M, Jgou C 2014 J. Nucl. Mater. 444 76
[7] Peuget S, Broudic V, Jgou C, Frugier P, Roudil D, Deschanels X, Rabiller H, Noel P 2007 J. Nucl. Mater. 362 474
[8] Ollier N, Champagnon B, Boizot B, Guyot Y, Panczer G, Padlyak B 2003 J. Non-Cryst. Solids 323 200
[9] Ollier N, Boizot B, Reynard B, Ghaleb D, Petite G 2005 J. Nucl. Mater. 340 209
[10] Ollier N, Boizot B, Reynard B, Ghaleb D, Petite G 2004 Nucl. Instrum. Meth. B 218 176
[11] Mohapatra M, Kadam R M, Mishra R K, Kaushik C P, Tomar B S, Godbole S V 2011 Physica B 406 3980
[12] Mohapatra M, Kadam R M, Mishra R K, Dutta D, Pujari P K, Kaushik C P, Kshirsagar R J, Tomar B S, Godbole S V 2011 Nucl. Instrum. Meth. B 269 2057
[13] Mohapatra M, Manchanda V K 2009 IOP Conf. Ser.: Mater. Sci. Eng. 2 012022
[14] Yang K J, Wang T S, Zhang G F, Peng H B, Chen L, Zhang L M, Li C X, Tian F, Yuan W 2013 Nucl. Instrum. Meth. B 307 541
[15] Zhang G F, Wang T S, Yang K J, Chen L, Zhang L M, Peng H B, Yuan W, Tian F 2013 Nucl. Instrum. Meth. B 316 218
[16] Chen L, Wang T S, Yang K J, Peng H B, Zhang G F, Zhang L M, Jiang H, Wang Q 2013 Nucl. Instrum. Meth. B 307 566
[17] Chen L, Yuan W, Nan S, Du X, Zhang D F, L P, Peng H B, Wang T S 2016 Nucl. Instrum. Meth. B 370 42
[18] Peng H B, Sun M L, Yang K J, Chen H, Yang D, Yuan W, Chen L, Duan B H, Wang T S 2016 J. Non-Cryst. Solids 443 143
[19] Wang T S, Duan B H, Tian F, Peng H B, Chen L, Zhang L M, Yuan W 2015 Chin. Phys. B 24 076102
[20] Wang T S, Du X, Yuan W, Duan B H, Zhang J D, Chen L, Peng H B, Yang D, Zhang G F, Zhu Z H 2016 Surf. Coat. Technol. 306 245
[21] Karakurt G, Abdelouas A, Guin J P, Nivard M, Sauvage T, Paris M, Bardeau J F 2016 J. Nucl. Mater. 475 243
[22] Inagaki Y, Furuya H, Idemitsu K, Banba Y, Matsumoto S, Muraoka S 1991 Mater. Res. Soc. Symp. Proc. 257 199
[23] Mir A H, Monnet I, Toulemonde M, Bouffard S, Jegou C, Peuget S 2016 J. Nucl. Mater. 469 244
[24] Mir A H, Toulemonde M, Jegou C, Miro S, Serruys Y, Bouffard S, Peuget S 2016 Sci. Rep. 6 30191
[25] Routbort J L, Matzke H 1983 J. Mater. Sci. Eng. 58 229
[26] Joslin D L, Oliver W C 1990 J. Mater. Res. 5 123
[27] Zhu D R, Lai T S 1997 Acta Sci. Natur. Univ. 36 31 (in Chinese) [朱德瑞, 赖天树 1997 中山大学学报 (自然科学版) 36 31]
[28] Peng H, Sun M, Du X, Yuan W, Yang D, Chen L, Duan B, Wang T 2017 Nucl. Instrum. Meth. B 406 561
[29] Peuget S, Cachia J N, Jgou C, Deschanels X, Roudil D, Broudic V, Delaye J M, Bart J M 2006 J. Nucl. Mater. 354 1
[30] Arndt J, Devine R A B, Revesz A G 1991 J. Non-Cryst. Solids 131-133 1206
[31] Arndt J, Stffler D 1969 Phys. Chem. Glasses 10 117
[32] Makishima A, Mackenzie J 1973 J. Non-Cryst. Solids 12 35
[33] Chi Y S, Shen J Y, Chen X X, Miu Z X 2002 J. Inorg. Mater. 17 475 (in Chinese) [迟玉山, 沈菊云, 陈学贤, 缪之训 2002 无机材料学报 17 475]
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