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Method of solar occultation flux infrared spectroscopy to detect the pollution emission flux of sources is presented in detail. It is developed based on the FTIR technique. A Two-layer radiative transfer model is established theoretically. Algorithm of transmissivity calculation of pollution gas is expatiated. The method to obtain the absorption coefficient of molecules from HITRAN, NIST and QAsoft databases is mentioned. Levenberg-Marquardt algorithm is used to calculate column concentration of pollution gas from pollution source. The distribution of column concentration is drawn by software developed by our group. The total system and the sun tracker are shown in the paper. The distribution of column concentration of NH3 is measured in a chemical plant in Hefei China. The calculated distribution of column concentration of NH3 is consistent with the measured one in the chemical plant.
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Keywords:
- infrared solar occultation flux /
- FTIR /
- emission gas /
- environment monitoring
[1] Wu J G 1994 Modern Fourier Transform Infrared Spectroscopy and Its Application (Vol.1) (Beijing: Scientifical and Technical Documents Press) p492—505 (in Chinese) [吴谨光 1994 近代傅里叶变换红外光谱技术及应用(上册) (北京:科学技术文献出版社) 第492—505页]
[2] Manne K, 2005, Ph.D. Dissertation (Sweden: Chalmers University of Technology)
[3] Zhou B, Liu W Q, Zheng Z H, Zhang Y J, Song B C, Wang F P 2000 Acta Phys. Sin. 49 2507 (in Chinese) [周 斌、刘文清、郑朝辉、张玉钧、宋炳超、王锋平 2000 49 2507]
[4] Roland H, Peter R, Chris D, Anita J, Richard M, Benjamin T 2005 International Sociaty for Optical Engineering 5995 599510
[5] Cao T T, Luo S R, Zhao X Y, Liang H M, Wang H B, Yang J G 2007 Acta Phys. Sin. 56 5554 (in Chinese) [曹婷婷、罗时荣、赵晓艳、梁慧敏、王宏波、杨经国 2007 56 5554]
[6] Liu Z M,Liu W Q,Gao M G,Tong J J,Zhang T S,Xu L,Wei X L 2008 Chin. Phys. B 17 4184
[7] Zhou B, Liu W Q, Qi F, Li Z B, Cui Y J 2001 Acta Phys. Sin. 50 1818 (in Chinese) [周 斌、刘文清、齐 峰、李振壁、崔延军 2001 50 1818 ]
[8] Chaffin C T, Marshall T L, Chaffin N C 1999 Field Anal. Chem. Technol, 3 111
[9] Rothman L S, Jacquemart D, Barbe A, Chris Benner D, Birk M 2005 J Quant. Spectrosc. and Radiat. Transfer 96 139
[10] David W T Griffith. 1996 Appl. Spec. 50 59
[11] Liu Z M, Gao M G, Liu W Q, Zhang T S, Xu L, Wei X L, Chen H 2008 Spectrosc. Spect. Anal. 28 770 (in Chinese) [刘志明、高闽光、刘文清、张天舒、徐 亮、魏秀丽、陈 华 2008 光谱学与光谱分析 28 770]
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[1] Wu J G 1994 Modern Fourier Transform Infrared Spectroscopy and Its Application (Vol.1) (Beijing: Scientifical and Technical Documents Press) p492—505 (in Chinese) [吴谨光 1994 近代傅里叶变换红外光谱技术及应用(上册) (北京:科学技术文献出版社) 第492—505页]
[2] Manne K, 2005, Ph.D. Dissertation (Sweden: Chalmers University of Technology)
[3] Zhou B, Liu W Q, Zheng Z H, Zhang Y J, Song B C, Wang F P 2000 Acta Phys. Sin. 49 2507 (in Chinese) [周 斌、刘文清、郑朝辉、张玉钧、宋炳超、王锋平 2000 49 2507]
[4] Roland H, Peter R, Chris D, Anita J, Richard M, Benjamin T 2005 International Sociaty for Optical Engineering 5995 599510
[5] Cao T T, Luo S R, Zhao X Y, Liang H M, Wang H B, Yang J G 2007 Acta Phys. Sin. 56 5554 (in Chinese) [曹婷婷、罗时荣、赵晓艳、梁慧敏、王宏波、杨经国 2007 56 5554]
[6] Liu Z M,Liu W Q,Gao M G,Tong J J,Zhang T S,Xu L,Wei X L 2008 Chin. Phys. B 17 4184
[7] Zhou B, Liu W Q, Qi F, Li Z B, Cui Y J 2001 Acta Phys. Sin. 50 1818 (in Chinese) [周 斌、刘文清、齐 峰、李振壁、崔延军 2001 50 1818 ]
[8] Chaffin C T, Marshall T L, Chaffin N C 1999 Field Anal. Chem. Technol, 3 111
[9] Rothman L S, Jacquemart D, Barbe A, Chris Benner D, Birk M 2005 J Quant. Spectrosc. and Radiat. Transfer 96 139
[10] David W T Griffith. 1996 Appl. Spec. 50 59
[11] Liu Z M, Gao M G, Liu W Q, Zhang T S, Xu L, Wei X L, Chen H 2008 Spectrosc. Spect. Anal. 28 770 (in Chinese) [刘志明、高闽光、刘文清、张天舒、徐 亮、魏秀丽、陈 华 2008 光谱学与光谱分析 28 770]
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