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Infrared absorption of deuterium molecules at low temperature

Liu Jiang-Ping Li Jun Liu Yuan-Qiong Lei Hai-Le Wei Jian-Jun

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Infrared absorption of deuterium molecules at low temperature

Liu Jiang-Ping, Li Jun, Liu Yuan-Qiong, Lei Hai-Le, Wei Jian-Jun
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  • The vibration/rotation modes and the corresponding infrared spectra of deuterium molecules with the D2d/D2h structures are calculated using the coupled cluster singles and doubles method with the cc-PVTZ basis sets within the framework of the density function theory. The infrared (IR) absorption spectrum of liquid deuterium is experimentally measured in a home-made cryogenic target system by a home-made low-temperature infrared spectroscope. The experimental results show that the strongest IR absorption peak of liquid deuterium is related to the Q1(0)+S0(0) mode, which is in good agreement with the theoretical calculation.
    [1]

    Harris A B 1970 Phys. Rev. B 1 1881

    [2]

    Kranendonk J V 1983 Solid Hydrogen: Theory of the Properties of Solid H2 HD, D2 (New York: Plenum Press)

    [3]

    Sokol P E, Simmons R O 1985 Phys. Rev. B 31 620

    [4]

    Liu J P, Bi P, Lei H L, Li J, Wei J J 2013 Acta Phys. Sin. 62 163301 (in Chinese) [刘江平, 毕鹏, 雷海乐, 黎军, 韦建军 2013 62 163301]

    [5]

    Warren J A, Smith G R, Guillory W A 1980 J. Chem. Phys. 72 4901

    [6]

    Gillard P G, Prasad R D G 1984 J. Chem. Phys. 81 3458

    [7]

    Chan M C, Xu L W, Gabrys C M 1991 J. Chem. Phys. 95 9404

    [8]

    Miller R G J, Stace B C (Translated by Yu Q L) 1985 Laboratory Methods in Infrared Spectroscopy (2nd ed) (Beijing: Mechanical Industry Press) p67 (in Chinese) [密勒 R G J, 斯特斯 B C 著 (于铨林译) 1985 红外光谱学的实验方法 (第二版) (北京: 机械工业出版社) 第67页]

    [9]

    Bi P, Liu Y Q, Tang Y J, Yang X D, Lei H L 2009 Acta Phys. Sin. 59 7351 (in Chinese) [毕鹏, 刘元琼, 唐永建, 杨向东, 雷海乐 2009 59 7351]

    [10]

    Bi P, Lei H L, Liu Y Q, Li J, Yang X D 2012 Acta Phys. Sin. 61 062802 (in Chinese) [毕鹏, 雷海乐, 刘元琼, 黎军, 杨向东 2012 61 062802]

    [11]

    Bi P, Xie D, Lin W, Wang K, Liu J P, Tang Y J, Yang X D, Lei H L 2013 Chin. Phys. B 22 034401

    [12]

    Ching Y L, Gilbert A T B, Walker M A 2011 Astrophys. J. 736 91

    [13]

    Cao H H, Chen Q 2004 Chin. Phys. B 13 2121

    [14]

    Wu W D, Zhu Z H, Tang Y J 2002 Acta Phys. Sin. 51 1221 (in Chinese) [吴卫东, 朱正和, 唐永建 2002 51 1221]

    [15]

    Xu Y Z 1988 Theory of Molecule Spectroscopy (Beijing: Tsinghua University Press) p174 (in Chinese) [徐亦庄 1988 分子光谱理论 (北京: 清华大学出版社) 第174页]

    [16]

    Li Y J, Xie K, Xu J, Li X D, Han Y 2010 Acta Phys. Sin. 59 1082 (in Chinese) [李宇杰, 谢凯,许静, 李效东, 韩喻 2010 59 1082]

    [17]

    Lei H L, Li J, Tang Y J, Shi H L, Liu Y Q 2009 High Power Laser Particle Beams 21 53 (in Chinese) [雷海乐, 黎 军, 唐永建, 师洪丽, 刘元琼 2009 强激光与粒子束 21 53]

    [18]

    Chen G B, Bao R, Huang Y H 2006 Cryogenic Engineering Technical Data (Vol.2) (Beijing: Chemical Industry Press) p122 (in Chinese) [陈国邦, 包 锐, 黄永华 2006 低温工程技术数据 (第二卷) (北京: 化学工业出版社) 第122页]

    [19]

    Liu Y Q, Zhao X S, Lei H L, Xie D, Gao D Z 2010 High Power Laser Particle Beams 22 2880 (in Chinese) [刘元琼, 赵学森, 雷海乐, 谢端, 高党忠 2010 强激光与粒子 束22 2880]

    [20]

    Wang K, Lin W, Liu Y Q, Xie D, Li J, Ma K Q, Tang Y J, Lei H L 2012 Acta Phys. Sin. 61 195204 (in Chinese) [王凯, 林伟, 刘元琼, 谢端, 黎军, 马坤全, 唐永建, 雷海乐 2012 61 195204]

    [21]

    Lei H L, Li J, Tang Y J, Liu Y Q 2009 Rev. Sci. Instrum. 80 03310

    [22]

    Souers P C 1985 Hydrogen Properties for Fusion Energy (California: University of California Press) pp324–335

  • [1]

    Harris A B 1970 Phys. Rev. B 1 1881

    [2]

    Kranendonk J V 1983 Solid Hydrogen: Theory of the Properties of Solid H2 HD, D2 (New York: Plenum Press)

    [3]

    Sokol P E, Simmons R O 1985 Phys. Rev. B 31 620

    [4]

    Liu J P, Bi P, Lei H L, Li J, Wei J J 2013 Acta Phys. Sin. 62 163301 (in Chinese) [刘江平, 毕鹏, 雷海乐, 黎军, 韦建军 2013 62 163301]

    [5]

    Warren J A, Smith G R, Guillory W A 1980 J. Chem. Phys. 72 4901

    [6]

    Gillard P G, Prasad R D G 1984 J. Chem. Phys. 81 3458

    [7]

    Chan M C, Xu L W, Gabrys C M 1991 J. Chem. Phys. 95 9404

    [8]

    Miller R G J, Stace B C (Translated by Yu Q L) 1985 Laboratory Methods in Infrared Spectroscopy (2nd ed) (Beijing: Mechanical Industry Press) p67 (in Chinese) [密勒 R G J, 斯特斯 B C 著 (于铨林译) 1985 红外光谱学的实验方法 (第二版) (北京: 机械工业出版社) 第67页]

    [9]

    Bi P, Liu Y Q, Tang Y J, Yang X D, Lei H L 2009 Acta Phys. Sin. 59 7351 (in Chinese) [毕鹏, 刘元琼, 唐永建, 杨向东, 雷海乐 2009 59 7351]

    [10]

    Bi P, Lei H L, Liu Y Q, Li J, Yang X D 2012 Acta Phys. Sin. 61 062802 (in Chinese) [毕鹏, 雷海乐, 刘元琼, 黎军, 杨向东 2012 61 062802]

    [11]

    Bi P, Xie D, Lin W, Wang K, Liu J P, Tang Y J, Yang X D, Lei H L 2013 Chin. Phys. B 22 034401

    [12]

    Ching Y L, Gilbert A T B, Walker M A 2011 Astrophys. J. 736 91

    [13]

    Cao H H, Chen Q 2004 Chin. Phys. B 13 2121

    [14]

    Wu W D, Zhu Z H, Tang Y J 2002 Acta Phys. Sin. 51 1221 (in Chinese) [吴卫东, 朱正和, 唐永建 2002 51 1221]

    [15]

    Xu Y Z 1988 Theory of Molecule Spectroscopy (Beijing: Tsinghua University Press) p174 (in Chinese) [徐亦庄 1988 分子光谱理论 (北京: 清华大学出版社) 第174页]

    [16]

    Li Y J, Xie K, Xu J, Li X D, Han Y 2010 Acta Phys. Sin. 59 1082 (in Chinese) [李宇杰, 谢凯,许静, 李效东, 韩喻 2010 59 1082]

    [17]

    Lei H L, Li J, Tang Y J, Shi H L, Liu Y Q 2009 High Power Laser Particle Beams 21 53 (in Chinese) [雷海乐, 黎 军, 唐永建, 师洪丽, 刘元琼 2009 强激光与粒子束 21 53]

    [18]

    Chen G B, Bao R, Huang Y H 2006 Cryogenic Engineering Technical Data (Vol.2) (Beijing: Chemical Industry Press) p122 (in Chinese) [陈国邦, 包 锐, 黄永华 2006 低温工程技术数据 (第二卷) (北京: 化学工业出版社) 第122页]

    [19]

    Liu Y Q, Zhao X S, Lei H L, Xie D, Gao D Z 2010 High Power Laser Particle Beams 22 2880 (in Chinese) [刘元琼, 赵学森, 雷海乐, 谢端, 高党忠 2010 强激光与粒子 束22 2880]

    [20]

    Wang K, Lin W, Liu Y Q, Xie D, Li J, Ma K Q, Tang Y J, Lei H L 2012 Acta Phys. Sin. 61 195204 (in Chinese) [王凯, 林伟, 刘元琼, 谢端, 黎军, 马坤全, 唐永建, 雷海乐 2012 61 195204]

    [21]

    Lei H L, Li J, Tang Y J, Liu Y Q 2009 Rev. Sci. Instrum. 80 03310

    [22]

    Souers P C 1985 Hydrogen Properties for Fusion Energy (California: University of California Press) pp324–335

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Publishing process
  • Received Date:  22 September 2013
  • Accepted Date:  18 October 2013
  • Published Online:  05 January 2014

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