面向高性能摩擦纳米发电机的电介质材料

邓浩程; 李祎; 田双双; 张晓星; 肖淞

doi:10.7498/aps.73.20240150

摘要

摩擦纳米发电机(triboelectric nanogenerator, TENG)作为微纳电源或自取能传感器近年来在多领域表现出广阔的应用潜力. TENG的输出性能提升与作为摩擦起电层的电介质材料接触起电特性密切相关. 本文首先介绍了TENG及其电介质摩擦起电层的相关基础理论和模型; 其次, 阐述了TENG电介质材料的选材、改性(表面改性、体改性)和结构设计策略, 其中表面改性和体改性涉及表面粗糙度控制、官能团调控、电介质材料介电参数优化, 在电介质的结构设计方面, 重点介绍了电荷传输层、捕获层、阻挡层的原理及通过多层结构来提高TENG介电性能的典型方法; 最后, 强调了本领域发展面临的挑战和未来发展趋势, 为面向高性能TENG的纳米电介质材料开发提供参考.

关键词:

Abstract

Triboelectric nanogenerator (TENG), as a micro-nano power source or self-powered sensor, has shown great prospects in various industries in recent years. The TENG output performance is closely related to the contact electrification characteristics of the triboelectric dielectric material. Herein, we first introduce the relevant fundamental theory and models of TENG and tribo-dielectrics. Then, we introduce the material selection, modification method (including surface modification and bulk modification) and structural design strategy of TENG dielectric material. Surface and bulk modification mainly involve surface roughness control, surface functional group regulation, and optimization of dielectric parameters. In terms of dielectric structural design, the principle of charge transport, trapping, and blocking layers as well as typical techniques to improve the dielectric properties of TENGs through multi-layer structures are highlighted. Finally, challenges and directions for future research are discussed, which is conducive to the fabricating of high-performance TENG dielectric materials.

Keywords:

作者及机构信息

1.
武汉大学电气与自动化学院, 电网环境保护全国重点实验室, 武汉　430072

2.
湖北工业大学电气与电子工程学院, 新能源及电网装备安全监测湖北省工程研究中心, 武汉　430068

通信作者: 肖淞, xiaosong@whu.edu.cn

基金项目: 国家自然科学基金(批准号: 52207169)资助的课题.

Authors and contacts

1.
State Key Laboratory of Power Grid Environmental Protection, School of Electrical Engineering and Automation, Wuhan University, Wuhan 430072, China

2.
Hubei Engineering Research Center for Safety Monitoring of New Energy and Power Grid Equipment, School of Electrical and Electronic Engineering, Hubei University of Technology, Wuhan 430068, China

Corresponding author: Xiao Song, xiaosong@whu.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 52207169).

文章全文 : translate this paragraph

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施引文献

图 1 高性能摩擦纳米发电机的电介质材料改性与设计策略^[13-18]

Fig. 1. Schematic diagram of dielectric modification and design strategies for high-performance triboelectric nanogenerator^[13-18].

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图 2 (a) CS-TENG的理论模型^[22], 电介质-电介质型(i)和导体-电介质型(ii); (b) 纳米电介质的界面模型^[25]

Fig. 2. (a) Theoretical models for CS-TENG^[22], dielectric-to-dielectric mode (i), and conductor-to-dielectric mode (ii); (b) interface model of nanodielectrics^[25].

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图 3 表面粗糙度控制策略　(a) 表面改性机制^[41]; (b) 表面图案化^[13]; (c) 砂纸模版法^[44]; (d) 静电纺丝ZnO/PAN纤维膜^[46]; (e) 静电纺丝SMPU纤维膜^[47]

Fig. 3. Surface roughness control strategy: (a) Surface modification mechanism^[41]; (b) surface patterning^[13]; (c) sandpaper template method^[44]; (d) electrospun ZnO/PAN fiber membrane^[46]; (e) electrospun SMPU fiber membrane^[47].

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图 4 表面官能团修饰策略　(a) 原子层面修饰^[14]; (b) 纤维素分子修饰^[51]; (c) 离子改性^[52]; (d) 等离子体处理^[54]; (e) 中性束处理^[55]

Fig. 4. Surface functional group modification strategy: (a) Atomic level modification^[14]; (b) cellulose molecule modification^[51]; (c) ion modification^[52]; (d) plasma treatment^[54]; (e) neutral beam treatment^[55].

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图 5 提高相对介电常数的策略　(a) 极性相诱导示意图^[57]; (b) Bi₂WO₆:PVDF-TrFE纳米纤维膜^[15]; (c) 微电容器模型示意图^[67]; (d) Co-NPC/PVDF介质形成的微电容器^[69]; (e) MOF纳米片/丝素蛋白复合膜^[70]; (f) Cs₃Bi₂Br₉/PVDF-HFP纳米纤维膜^[72]

Fig. 5. Strategies for improving relative permittivity: (a) Schematic diagram of polar phase induction^[57]; (b) Bi₂WO₆:PVDF-TrFE nanofiber membrane^[15]; (c) schematic diagram of the microcapacitor model^[67]; (d) microcapacitor formed by Co-NPC/PVDF dielectric^[69]; (e) MOF nanoflakes/silk fibroin composite membrane^[70]; (f) Cs₃Bi₂Br₉/PVDF-HFP nanofiber membrane^[72].

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图 6 抑制相对介电损耗、提高介电强度的策略　(a) Ag@C纳米颗粒掺入PDMS基质^[16]; (b) Al@Al₂O₃纳米颗粒掺入PVDF基质^[74]; (c) Ba(Zr_0.21Ti_0.79)O₃和BNNS共同掺入PVDF基质^[76]; (d) TiO₂纳米棒阵列掺入PVDF基质^[75]

Fig. 6. Strategies to suppress relative dielectric loss and improve dielectric strength (a) Ag@C nanoparticles incorporated into PDMS matrix^[16]; (b) Al@Al₂O₃ nanoparticles incorporated into PVDF matrix^[74]; (c) Ba(Zr_0.21Ti_0.79)O₃ and BNNS incorporated into PVDF matrix^[76]; (d) TiO₂ nanorod array incorporated into PVDF matrix^[75].

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图 7 电荷传输层、储存层、阻挡层　(a) rGO-AgNPs充当电荷捕获层^[86]; (b) 摩擦电介质体积电导率对电荷捕获的影响^[87]; (c) PVA-PVA/CNT-PS充当电荷收集层、传输层和储存层^[17]; (d) TiO_x充当电荷阻挡层^[84]

Fig. 7. Charge transport-storage-blocking layer: (a) rGO-AgNPs functioning as charge trapping layer^[86]; (b) effect of tribo-layer volume conductivity on charge trapping^[87]; (c) PVA-PVA/CNT-PS functioning as charge transport, transfer, and storage layer^[17]; (d) TiO_x functioning as charge blocking layer^[84].

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图 8 多层电介质结构设计　(a) Maxwell-Sillar-Wagner模型^[90]; (b) 铁电多层纳米复合电介质^[91]; (c) PVDF/BNNS-PVDF/BST-PVDF/BNNS三层结构电介质^[92]; (d) 梯度浓度的PVDF/BaTiO₃三层结构电介质^[94]

Fig. 8. Multilayered dielectric structure design: (a) Maxwell-Sillar-Wagner model^[90]; (b) ferroelectric multilayer nanocomposite dielectric^[91]; (c) PVDF/BNNS-PVDF/BST-PVDF/BNNS three-layer structure dielectric^[92]; (d) PVDF/BaTiO₃ three-layer structure dielectric with gradient concentration^[94].

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map

[1]	Fan F R, Tian Z Q, Lin Wang Z 2012 Nano Energy 1 328 Google Scholar
[2]	Kim W G, Kim D W, Tcho I W, Kim J K, Kim M S, Choi Y K 2021 ACS Nano 15 258 Google Scholar
[3]	Chang A, Uy C, Xiao X, Xiao X, Chen J 2022 Nano Energy 98 107282 Google Scholar
[4]	Wang Z L 2021 Rep. Prog. Phys. 84 096502 Google Scholar
[5]	Deng H C, Xiao S, Yang A J, Wu H Y, Tang J, Zhang X X, Li Y 2023 Nano Energy 115 108738 Google Scholar
[6]	Fan Y Y, Zhang L, Li D C, Wang Z L 2023 Nano Energy 118 108959 Google Scholar
[7]	Chen G, Wang J, Xu G Q, Fu J J, Gani A B, Dai J H, Guan D, Tu Y P, Li C Y, Zi Y L 2023 EcoMat 5 e12410 Google Scholar
[8]	Liang Y, Xu X Y, Zhao L B, Lei C Y, Dai K J, Zhuo R, Fan B B, Cheng E, Hassan M A, Gao L X, Mu X J, Hu N, Zhang C 2023 Small 2308469 Google Scholar
[9]	Zhou L L, Liu D, Wang J, Wang Z L 2020 Friction 8 481 Google Scholar
[10]	Jiang F, Zhan L X, Lee J P, Lee P S 2023 Adv. Mater. 36 2308197
[11]	Liu Y H, Mo J L, Fu Q, Lu Y X, Zhang N, Wang S F, Nie S X 2020 Adv. Funct. Mater. 30 2004714 Google Scholar
[12]	Tao X L, Chen X, Wang Z L 2023 Energy Environ. Sci. 16 3654 Google Scholar
[13]	Ahn J, Zhao Z J, Choi J, Jeong Y, Hwang S, Ko J, Gu J, Jeon S, Park J, Kang M, Del Orbe D V, Cho I, Kang H, Bok M, Jeong J H, Park I 2021 Nano Energy 85 105978 Google Scholar
[14]	Shin S H, Bae Y E, Moon H K, Kim J, Choi S H, Kim Y, Yoon H J, Lee M H, Nah J 2017 ACS Nano 11 6131 Google Scholar
[15]	Bharti D K, Veeralingam S, Badhulika S 2022 Mater. Horiz. 9 663 Google Scholar
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[22]	Niu S, Wang Z L 2015 Nano Energy 14 161 Google Scholar
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