微观尺度下的水:从准一维、二维受限空间到生物以及材料表面

方海平

doi:10.7498/aps.65.186101

摘要

地球上的各种过程，包括物理、化学、环境和生物等，大多数与微观尺度下的界面水息息相关. 界面水有大量悬而未决的基础科学问题，长期以来水都是重要的科学研究对象. 本文通过从一维受限空间、二维表面以及生物大分子和材料表面上的水等角度概述当前的一些研究进展，讨论与界面水相关的一些前沿问题，以及在界面水方面的基础研究和新技术的突破对于解决这些前沿问题的必要性。

关键词:

A majority of the physical, biological, chemical and environmental processes relate to the interfacial water. However, for the interfacial water itself, there are still many puzzles unsolved, which have made the interfacial water an important scientific research object for quite a long time. In this paper, we review some recent progress on the dynamics of interfacial water confined in one-dimensional and two- dimensional spaces, and on the surfaces on biomolecules and materials as well.

Keywords:

interfacial water /
quasi-one dimension and two-dimension confined space /
biomolecules surfaces /
materials surfaces

作者及机构信息

方海平

1.
中国科学院上海应用物理研究所, 中国科学院微观界面物理与探测重点实验室, 水科学与技术研究室, 上海 201800

通信作者: 方海平, fanghaiping@sinap.ac.cn

基金项目: 国家自然科学基金（批准号：11290164）、中国科学院知识创新工程领域前沿项目（批准号：KJZD-EW-M03）、上海超级计算中心、中科院计算机网络信息中心、国家超级计算深圳中心（云计算中心）、NSFC-广东联合基金（第二期）超级计算科学应用研究专项和国家超级计算广州中心资助的课题.

Authors and contacts

Fang Hai-Ping

1.
Division of Interfacial Water, Key Laboratory of Interfacial Physics and Technology, Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800, China

Corresponding author: Fang Hai-Ping, fanghaiping@sinap.ac.cn

Funds: Project supported by the National Science Foundation of China (Grant No. 11290164), the Key Research Program of Chinese Academy of Sciences (Grant No. KJZD-EW-M03), the Shanghai Supercomputer Center of China, the Computer Network Information Center of Chinese Academy of Sciences, the National Supercomputing Center in Shenzhen (Shenzhen Cloud Computing Center), China, and the Special Program for Applied Research on Super Computation of the NSFC-Guangdong Joint Fund (the Second Phase), China.

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施引文献

[1]	Ewing G E 2006 Chem. Rev. 106 1511
[2]	Verdaguer A, Sacha G M, Bluhm H, Salmeron M 2006 Chem. Rev. 106 1478
[3]	Brown G E 2001 Science 294 67
[4]	Ball P 2008 Chem. Rev. 108 74
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[6]	Service R F 2006 Science 313 1088
[7]	Bocquet L, Charlaix E 2010 Chem. Soc. Rev. 39 1073
[8]	Bonn D, Eggers J, Indekeu J, Meunier J, Rolley E 2009 Rev. Mod. Phys. 81 739
[9]	Somorjai G A, Li Y 2001 Proc. Natl. Acad. Sci. USA 108 917
[10]	Pal S K, Zewail A H 2004 Chem. Rev. 104 2099
[11]	Hummer G, Rasaiah J C, Noworyta J P 2001 Nature 414 188
[12]	Cambré S, Schoeters B, Luyckx S, Goovaerts E, Wenseleers W 2010 Phys. Rev. Lett. 104 207401
[13]	Ghosh S, Sood A K, Kumar N 2003 Science 299 1042
[14]	Holt J K, Park H G, Wang Y, Stadermann M, Artyukhin A B, Grigoropoulos C P, Noy A, Bakajin O 2006 Science 312 1034
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[43]	Zhao W H, Bai J, Yuan L F, Yang J, Zeng X C 2014 Chem. Sci. 5 1757
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[59]	Wan R, Wang C, Lei X, Zhou G, Fang H P 2015 Phys. Rev. Lett. 115 195901
[60]	Wang C L, Yang Y Z, Fang H P 2014 Sci. China: Phys. Mech. Astron. 57 802
[61]	Rotenberg B, Patel A, Chandler D 2011 J. Am. Chem. Soc. 133 20521
[62]	Limmer D, Willard A, Madden P, Chandler D 2013 Proc. Natl. Acad. Sci. USA 110 4200
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[66]	Wang Y, Duan Z, Fan D 2013 Sci. Rep. 3 3505
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[80]	Angel T E, Chance M R, Palczewski K 2009 Proc. Natl. Acad. Sci. USA 106 8555
[81]	Franck J M, Ding Y, Stone K, Qin P Z, Han S 2015 J. Am. Chem. Soc. 137 12013
[82]	Zhang Y, Zhang J, Wang W 2011 J. Am. Chem. Soc. 133 6882
[83]	Athri P, Wilson W D 2009 J. Am. Chem. Soc. 131 7618
[84]	Wei D, Wilson W D, Neidle S 2013 J. Am. Chem. Soc. 135 1369
[85]	Khrová P, Otyepka M, čponer J, Banáš P 2014 J. Chem. Theory Compu. 10 401
[86]	Gong X J, Li J Y, Zhang H, Wan R Z, Lu H J, Wang S, Fang H P 2008 Phys. Rev. Lett. 101 257801
[87]	Fang H, Wan R, Gong X, Lu H, Li S 2008 J. Phys. D: Appl. Phys. 41 103002
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[89]	Zhao W, Moilanen D E, Fenn E E, Fayer M D 2008 J. Am. Chem. Soc. 130 13927
[90]	Hishida M, Tanaka K 2011 Phys. Rev. Lett. 106 158102
[91]	Nihonyanagi S, Mondal J A, Yamaguchi S, Tahara T 2013 Annu. Rev. Phys. Chem. 64 579
[92]	Chen X, Hua W, Huang Z, Allen H C 2010 J. Am. Chem. Soc. 132 11336
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[94]	Re S, Nishima W, Tahara T, Sugita Y 2014 J. Phys. Chem. Lett. 5 4343
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