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In recent years, significant progress has been made in the superconductivity of nickelates, with global teams discovering various nickelate superconductors under ambient and high pressure conditions. Research teams in China and USA have independently discovered ambient-pressure superconductivity in Ruddlesden-Popper bilayer nickelate thin films through different technical pathways, establishing a novel platform for probing high-temperature superconducting mechanisms. The Chinese teams have synthesized pure-phase bilayer nickelate films with atomically smooth surfaces by using their proprietary Gigantic-Oxidative Atomic-Layer-by-Layer Epitaxy (GOALL-Epitaxy) technique. After in situ strong oxidation processing of surface, surface-sensitive measurements, such as ARPES, can be conducted on these atomically flat films to reveal the electronic structure of the superconducting phase, and further in-depth experimental research on superconducting mechanisms is expected. Through synergistic efforts in lattice engineering, rare-earth/alkaline-earth element substitution, and interface strain engineering, this system has the potential to achieve higher superconducting transition temperatures.
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Keywords:
- high-temperature superconductivity /
- nickelate thin film /
- gigantic-oxidative atomic-layer-by-layer epitaxy
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图 1 (a) 铜氧化物超导体、(b) 方平面无限层结构镍氧化物超导体以及 (c) 双层RP结构镍氧化物超导体的晶体结构与电子结构示意图
Figure 1. Schematic diagrams of the crystal structures and electronic structures of (a) cuprate superconductors, (b) square-planar infinite-layer nickelate superconductors, and (c) bilayer RP nickelate superconductors under pressure.
图 2 (a)大范围扫描透射电子显微镜图像显示3 UC La2.85Pr0.15Ni2O7/SrLaAlO4薄膜的纯相晶体结构; (b)零电阻和(c)互感抗磁性测试证实常压下双层RP结构镍氧化物超导电性的存在, 图(c)中蓝色和红色的点为实验测试数据, 实线为视觉引导线[38]
Figure 2. (a) A large field of view scanning transmission electron microscopy image of 3 UC La2.85Pr0.15Ni2O7/SrLaAlO4 film with pure-phase crystalline structure; (b) zero resistance and (c) mutual inductance diamagnetism results confirm the existence of superconductivity of double-layer RP nickel oxide at ambient-pressure. In panel (c), the blue and red dots represent the experimental data, and the solid lines are guides to the eye[38].
图 4 常压RP结构镍氧化物超导薄膜研究路线图
Figure 4. Research roadmap of ambient-pressure RP phase nickelate superconducting thin films.
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