Interfacial rheological study of silica nanoparticle monolayer by an indentation approach

Zang Du-Yang; Zhang Yong-Jian

doi:10.7498/aps.61.026803

Abstract

We propose a novel approach for the study of rheological properties of silica nanoparticle monolayers at the air-water interface. The layers are deformed by indenting and raising a titanium cone. The surface pressure variations in these down-up cycles are recorded and analysed. The oscillation amplitude of surface pressure d results from the tensile deformation of the particle layer. d and the relaxation time are strongly dependent on the adsorption energy of particles at the interface, thereby significantly changing the particle hydrophobicity. The results provide a deeper insight into the viscoelastic behaviour of particle layer, suggesting that the proposed method can be utilized for the rheological study of the layers of this kind.

Keywords:

Authors and contacts

1.
Key Laboratory of Space Applied Physics and Chemistry of Ministry of Education, School of Science, Northwestern Polytechnical University, Xi’an 710129, China;
2.
State Key Laboratory of Solidification Processing, School of Materials Science and Engineering, Northwestern Polytechnical University, Xi’an 710072, China
Funds: Project supported by the NPU Foundation for Fundamental Research (NPU-FFR-JC20100242).

References

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[13]	Grzelczak M, Vermant J, Furst E M, Liz-Marzán L M 2010 ACS Nano 4 3591
[14]	Oettel M, Dietrich S 2008 Langmuir 24 1425
[15]	Gaines G L 1966 Insoluble monolayers at liquid-gas surfaces, John Wiley, New York
[16]	Connors K 1990 Chemical Kinetics, VCH Publishers
[17]	Tschogel N W 1989 The phenomenological Theory of Linear Viscoelastic Behaviour (Springer-Verlag, Berlin)

Cited By

[1]	Binks B P 2007Phys. Chem. Chem. Phys. 9 6298
[2]	Herzig E M, White K A, Schofield A B, Poon W C K, Clegg P S 2007 Nat. Mater. 6 966
[3]	Sanz E, White K A, Clegg P S, Cates M E 2009 Phys. Rev. Lett. 103 255502
[4]	Lin B J, Chen L J 2007 J. Chem. Phys. 126 034706
[5]	Stankiewicz J, Cabrerizo V′?lchez M A, Alvarez R H 1993 Phys. Rev. E 47 2663
[6]	Vella D, Aussillous P, Mahadevan L 2004 Europhys. Lett. 68 212
[7]	Zang D Y, Rio E, Langevin D, Wei B, Binks B P 2010 Eur. Phys. J. E 31 125
[8]	Zang D Y, Rio E, Delon G, Langevin D, Wei. B, Binks B P 2011 Mol. Phys. 109 1057
[9]	Zang D Y, Zhang Y J, Langevin D 2011 Acta Phys. Sin. 60 076801 (in Chinese) [臧渡洋, 张永建, Langevin Dominique 2011 60 076801]
[10]	Madivala B, Fransaer J, Vermant J 2009 Langmuir 25 2718
[11]	Safouane M, Langevin D, Binks B P 2007 Langmuir 23 11546
[12]	Zang D Y, Langevin D, Binks B P, Wei B 2010 Phys. Rev. E 81 011604
[13]	Grzelczak M, Vermant J, Furst E M, Liz-Marzán L M 2010 ACS Nano 4 3591
[14]	Oettel M, Dietrich S 2008 Langmuir 24 1425
[15]	Gaines G L 1966 Insoluble monolayers at liquid-gas surfaces, John Wiley, New York
[16]	Connors K 1990 Chemical Kinetics, VCH Publishers
[17]	Tschogel N W 1989 The phenomenological Theory of Linear Viscoelastic Behaviour (Springer-Verlag, Berlin)

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Catalog

Vol. 61, Issue 2 - 2012-01-20

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