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Cross section measurement of neutron capture reaction based on back-streaming white neutron source at China spallation neutron source

Zhang Qi-Wei Luan Guang-Yuan Ren Jie Ruan Xi-Chao He Guo-Zhu Bao Jie Sun Qi Huang Han-Xiong Wang Zhao-Hui Gu Min-Hao Yu Tao Xie Li-Kun Chen Yong-Hao An Qi Bai Huai-Yong Bao Yu Cao Ping Chen Hao-Lei Chen Qi-Ping Chen Yu-Kai Chen Zhen Cui Zeng-Qi Fan Rui-Rui Feng Chang-Qing Gao Ke-Qing Han Chang-Cai Han Zi-Jie He Yong-Cheng Hong Yang Huang Wei-Ling Huang Xi-Ru Ji Xiao-Lu Ji Xu-Yang Jiang Wei Jiang Hao-Yu Jiang Zhi-Jie Jing Han-Tao Kang Ling Kang Ming-Tao Li Bo Li Chao Li Jia-Wen Li Lun Li Qiang Li Xiao Li Yang Liu Rong Liu Shu-Bin Liu Xing-Yan Mu Qi-Li Ning Chang-Jun Qi Bin-Bin Ren Zhi-Zhou Song Ying-Peng Song Zhao-Hui Sun Hong Sun Kang Sun Xiao-Yang Sun Zhi-Jia Tan Zhi-Xin Tang Hong-Qing Tang Jing-Yu Tang Xin-Yi Tian Bin-Bin Wang Li-Jiao Wang Peng-Cheng Wang Qi Wang Tao-Feng Wen Jie Wen Zhong-Wei Wu Qing-Biao Wu Xiao-Guang Wu Xuan Yang Yi-Wei Yi Han Yu Li Yu Yong-Ji Zhang Guo-Hui Zhang Lin-Hao Zhang Xian-Peng Zhang Yu-Liang Zhang Zhi-Yong Zhao Yu-Bin Zhou Lu-Ping Zhou Zu-Ying Zhu Dan-Yang Zhu Ke-Jun Zhu Peng Zhu Xing-Hua

Citation:

Cross section measurement of neutron capture reaction based on back-streaming white neutron source at China spallation neutron source

Zhang Qi-Wei, Luan Guang-Yuan, Ren Jie, Ruan Xi-Chao, He Guo-Zhu, Bao Jie, Sun Qi, Huang Han-Xiong, Wang Zhao-Hui, Gu Min-Hao, Yu Tao, Xie Li-Kun, Chen Yong-Hao, An Qi, Bai Huai-Yong, Bao Yu, Cao Ping, Chen Hao-Lei, Chen Qi-Ping, Chen Yu-Kai, Chen Zhen, Cui Zeng-Qi, Fan Rui-Rui, Feng Chang-Qing, Gao Ke-Qing, Han Chang-Cai, Han Zi-Jie, He Yong-Cheng, Hong Yang, Huang Wei-Ling, Huang Xi-Ru, Ji Xiao-Lu, Ji Xu-Yang, Jiang Wei, Jiang Hao-Yu, Jiang Zhi-Jie, Jing Han-Tao, Kang Ling, Kang Ming-Tao, Li Bo, Li Chao, Li Jia-Wen, Li Lun, Li Qiang, Li Xiao, Li Yang, Liu Rong, Liu Shu-Bin, Liu Xing-Yan, Mu Qi-Li, Ning Chang-Jun, Qi Bin-Bin, Ren Zhi-Zhou, Song Ying-Peng, Song Zhao-Hui, Sun Hong, Sun Kang, Sun Xiao-Yang, Sun Zhi-Jia, Tan Zhi-Xin, Tang Hong-Qing, Tang Jing-Yu, Tang Xin-Yi, Tian Bin-Bin, Wang Li-Jiao, Wang Peng-Cheng, Wang Qi, Wang Tao-Feng, Wen Jie, Wen Zhong-Wei, Wu Qing-Biao, Wu Xiao-Guang, Wu Xuan, Yang Yi-Wei, Yi Han, Yu Li, Yu Yong-Ji, Zhang Guo-Hui, Zhang Lin-Hao, Zhang Xian-Peng, Zhang Yu-Liang, Zhang Zhi-Yong, Zhao Yu-Bin, Zhou Lu-Ping, Zhou Zu-Ying, Zhu Dan-Yang, Zhu Ke-Jun, Zhu Peng, Zhu Xing-Hua
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  • The data of neutron capture cross section are very important for the research of nuclear astrophysics, advanced nuclear energy development. Owing to the limitation of neutron source and detector, the experimental data of neutron capture cross section in an energy range of 1 eV–10 keV were almost blank in China. The first Chinese gamma-ray total absorption facility has been constructed in the key laboratory of nuclear data at China institute of atomic energy, which consists of 40 BaF2 detector units. The BaF2 crystal shell with a thickness of 15 cm and an inner radius of 10 cm covers 95.2% of the solid angle. On-line measurement method of neutron capture reaction cross section is established on the back-streaming white neutron source of China spallation neutron source by using the upgraded facility. The cross section of 197Au neutron capture reaction is measured for the first time under the experimental condition of irregular 30 mm neutron beam spot. The measured position of resonance peak is well consistent with the relevant data of ENDF evaluation database, which verifies the reliability of the measurement device and measurement technology, and thus laying the foundation for the acquisition of high precision cross section in future.
      Corresponding author: Luan Guang-Yuan, lgyciae@hotmail.com
    • Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 11605294, 11675268, 11790321, 11975317) and the National Key Research and Development Program of China (Grant No. 2016YFA0401601).
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    Arnould M, Katsuma M 2008 International Conference on Nuclear Data for Science and Technology Nice, France, April 22–27, 2007 7

    [2]

    Palmiotti G, Salvatores M, Assawaroongruengchot M 2009 International Conference on Fast Reactors and Related Fuel Cycles Kyoto, Japan, Dec. 07–11, 2009

    [3]

    Kompe D 1969 Nucl. Phys. 133 513Google Scholar

    [4]

    Wisshak K, Kappeler F, Reffo G 1984 Nucl. Sci. Eng. 88 594Google Scholar

    [5]

    Terada K, Katabuchi T, Mizumoto M, et al. 2015 Progress in Nuclear Energy 82 118Google Scholar

    [6]

    Kobayashi K, Lee S, Yamamoto S 2004 Nucl. Sci. Eng. 146 209Google Scholar

    [7]

    Lee J, Hori J I, Nakajima K, Sano T, Lee S 2017 J. Nucl. Sci. Tech. 54 1046Google Scholar

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    Kim H I, Paradela C, Sirakov I, et al. 2016 Eur. Phys. J. A 52 170Google Scholar

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    Mingrone F, Massimi C, Altstadt S, et al. 2014 International Conference on Nuclear Data for Science and Technology NewYork, USA, Mar. 4–8, 2013 18

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    Guber K H, Derrien H, Leal L C, Arbanas G, Wiarda D, Koehler P E, Harvey A 2010 Phys. Rev. C 82 057601Google Scholar

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    Ren J, Ruan X, Bao J, et al. 2019 Radiation Detection Technology and Methods 3 52Google Scholar

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    Wisshak K, Voss F, Kaeppeler F, Krticka M, Gallino R 2006 Phys. Rev. C 73 015802Google Scholar

    [13]

    Mendoza E, Cano-Ott D, Altstadt S, et al. 2018 Phys. Rev. C 97 054616Google Scholar

    [14]

    Mosby S, Bredeweg T A, Couture A, Jandel M, Kawano T, Ullmann J L, Henderson R A, Wu C Y 2018 Phys. Rev. C 97 041601

    [15]

    Zhong Q P, Zhou Z Y, Tang H Q, et al. 2008 Chin. Phys. C 32 102

    [16]

    石斌, 彭猛, 张奇玮, 贺国珠, 周祖英, 唐洪庆 2018 原子能科学技术 52 1537Google Scholar

    Shi B, Peng M, Zhang Q W, He G Z, Zhou Z Y, Tang H Q 2018 Atomic Energy Science and Technology 52 1537Google Scholar

    [17]

    张奇玮, 贺国珠, 栾广源, 程品晶, 阮锡超, 朱兴华 2021 强激光与粒子束 33 0440

    Zhang Q W, He G Z, Luan G Y, Cheng P J, Ruan X C, Zhu X H 2021 Power Laser and Particle Beams 33 0440

    [18]

    唐靖宇, 安琪, 白怀勇, 等 2019 原子能科学技术 53 2012

    Tang J Y, An Q, Bai H Y, et al. 2019 Atomic Energy Science and Technology 53 2012 (in Chinese)

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    An Q, Bai H Y, Bao J, et al. 2017 Journal of Instrumentation 12 7022

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    Tang J Y, Fu S N, Jing H T, Tang H Q, Wei J, Xia H H 2010 Chin. Phys. C 34 121Google Scholar

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    Jing H T, Tang J Y, Tang H Q, Xia H H, Liang T J, Zhou Z Y, Zhong Q P, Ruan X C 2010 Nucl. Instr. Meth. A 621 91Google Scholar

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    唐靖宇, 敬罕涛, 夏海鸿, 唐洪庆, 张闯, 周祖英, 阮锡超, 张奇玮, 杨征 2013 原子能科学技术 47 1089Google Scholar

    Tang J Y, Jing H T, Xia H H, Tang H Q, Zhang C, Zhou Z Y, Ruan X C, Zhang Q W, Yang Z 2013 Atomic Energy Science and Technology 47 1089Google Scholar

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    任杰, 阮锡超, 唐洪庆, 葛智刚, 黄翰雄, 敬罕涛, 唐靖宇, 黄蔚玲 2014 核技术 37 110521

    Ren J, Ruan X C, Tang H Q, Ge Z G, Huang H X, Jing H T, Tang J Y, Huang W L 2014 Nucl. Tech. 37 110521

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    Chen Y H, Luan G Y, Bao J, et al. 2019 Eur. Phys. J. A 55 115Google Scholar

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    鲍杰, 陈永浩, 张显鹏, 等 2019 68 080101Google Scholar

    Bao J, Chen Y H, Zhang X P, et al. 2019 Acta Phys. Sin. 68 080101Google Scholar

    [26]

    韩长材, 欧阳晓平, 张显鹏, 宋朝晖, 鲍杰, 严维鹏 2020 原子能科学技术 54 385Google Scholar

    Han C C, Ouyang X P, Zhang X P, Song Z H, Bao J, Yan W P 2020 Atomic Energy Science and Technology 54 385Google Scholar

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    马霄云, 仲启平, 周祖英, 等 2009 原子能科学技术 43 180

    Ma X Y, Zhong Q P, Zhou Z Y, et al. 2009 Atomic Energy Science and Technology 43 180

    [28]

    张奇玮, 贺国珠, 黄兴, 阮锡超, 李志宏, 朱兴华 2014 原子能科学技术 48 70

    Zhang Q W, He G Z, Huang X, Ruan X C, Li Z H, Zhu X H 2014 Atomic Energy Science and Technology 48 70

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    Yu T, Cao P, Ji X Y, et al. 2019 IEEE Transactions on Nuclear Science 66 1095Google Scholar

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    Wang Q, Cao P, Qi X, et al. 2018 Review of Scientific Instruments 89 013511Google Scholar

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    张奇玮, 贺国珠, 黄兴, 程品晶, 阮锡超, 朱兴华 2016 原子能科学技术 50 536Google Scholar

    Zhang Q W, He G Z, Huang X, Cheng P J, Ruan X C, Zhu X H 2016 Atomic Energy Science and Technology 50 536Google Scholar

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    张奇玮, 栾广源, 贺国珠, 程品晶, 阮锡超, 朱兴华 2020 原子核物理评论 37 771Google Scholar

    Zhang Q W, Luan G Y, He G Z, Cheng P J, Ruan X C, Zhu X H 2020 Nuclear Physics Review 37 771Google Scholar

  • 图 1  中子俘获反应测量原理

    Figure 1.  Measurement principle of neutron capture reaction.

    图 2  CSNS反角白光中子源布局

    Figure 2.  Arrangement of Back-n at CSNS.

    图 3  实验测得的实验厅2的中子束流能谱

    Figure 3.  Experimental result of neutron energy spectrum at End-station 2.

    图 4  中子束斑剖面及其在水平和垂直方向的分布

    Figure 4.  Neutron beam profile and distribution in horizontal and vertical directions.

    图 5  (a) BaF2探测器单元; (b) GTAF-II谱仪

    Figure 5.  (a) BaF2 detector unit; (b) GTAF-II spectrometer.

    图 6  BaF2探测器单元探测到的信号波形

    Figure 6.  Signal waveform detected by BaF2 detector.

    图 7  GTAF-II谱仪电子学电路图

    Figure 7.  Electronic diagram of GTAF-II spectrometer.

    图 8  过阈触发原理示意图

    Figure 8.  Schematic diagram of over threshold trigger.

    图 9  (a)飞行时间谱的比较; (b)加和能谱的比较

    Figure 9.  (a) Comparison of time-of-flight spectrum; (b) comparison of sum energy spectrum.

    图 10  晶体多重数的比较

    Figure 10.  Comparison of crystal multiplicity.

    图 11  197Au中子俘获反应截面的实验结果

    Figure 11.  Experimental results of neutron capture cross section of 197Au.

    表 1  不同准直器孔径下实验厅2中子束斑尺寸的模拟结果

    Table 1.  Simulation result of neutron beam spot size at End-station 2 with different collimator aperture.

    中子束斑
    尺寸
    中子开关
    孔径
    准直器1#
    孔径
    准直器2#
    孔径
    ϕ30 mmϕ12 mmϕ15 mmϕ40 mm
    ϕ60 mmϕ50 mmϕ50 mmϕ58 mm
    90 mm × 90 mm78 mm × 62 mm76 mm × 76 mm90 mm × 90 mm
    DownLoad: CSV

    表 2  实验样品参数

    Table 2.  The characteristics of experimental samples.

    样品密度/(g·cm–3)直径/mm厚度/mm纯度/%
    197Au19.32250.299.99
    natC2.2525199.99
    DownLoad: CSV
    Baidu
  • [1]

    Arnould M, Katsuma M 2008 International Conference on Nuclear Data for Science and Technology Nice, France, April 22–27, 2007 7

    [2]

    Palmiotti G, Salvatores M, Assawaroongruengchot M 2009 International Conference on Fast Reactors and Related Fuel Cycles Kyoto, Japan, Dec. 07–11, 2009

    [3]

    Kompe D 1969 Nucl. Phys. 133 513Google Scholar

    [4]

    Wisshak K, Kappeler F, Reffo G 1984 Nucl. Sci. Eng. 88 594Google Scholar

    [5]

    Terada K, Katabuchi T, Mizumoto M, et al. 2015 Progress in Nuclear Energy 82 118Google Scholar

    [6]

    Kobayashi K, Lee S, Yamamoto S 2004 Nucl. Sci. Eng. 146 209Google Scholar

    [7]

    Lee J, Hori J I, Nakajima K, Sano T, Lee S 2017 J. Nucl. Sci. Tech. 54 1046Google Scholar

    [8]

    Kim H I, Paradela C, Sirakov I, et al. 2016 Eur. Phys. J. A 52 170Google Scholar

    [9]

    Mingrone F, Massimi C, Altstadt S, et al. 2014 International Conference on Nuclear Data for Science and Technology NewYork, USA, Mar. 4–8, 2013 18

    [10]

    Guber K H, Derrien H, Leal L C, Arbanas G, Wiarda D, Koehler P E, Harvey A 2010 Phys. Rev. C 82 057601Google Scholar

    [11]

    Ren J, Ruan X, Bao J, et al. 2019 Radiation Detection Technology and Methods 3 52Google Scholar

    [12]

    Wisshak K, Voss F, Kaeppeler F, Krticka M, Gallino R 2006 Phys. Rev. C 73 015802Google Scholar

    [13]

    Mendoza E, Cano-Ott D, Altstadt S, et al. 2018 Phys. Rev. C 97 054616Google Scholar

    [14]

    Mosby S, Bredeweg T A, Couture A, Jandel M, Kawano T, Ullmann J L, Henderson R A, Wu C Y 2018 Phys. Rev. C 97 041601

    [15]

    Zhong Q P, Zhou Z Y, Tang H Q, et al. 2008 Chin. Phys. C 32 102

    [16]

    石斌, 彭猛, 张奇玮, 贺国珠, 周祖英, 唐洪庆 2018 原子能科学技术 52 1537Google Scholar

    Shi B, Peng M, Zhang Q W, He G Z, Zhou Z Y, Tang H Q 2018 Atomic Energy Science and Technology 52 1537Google Scholar

    [17]

    张奇玮, 贺国珠, 栾广源, 程品晶, 阮锡超, 朱兴华 2021 强激光与粒子束 33 0440

    Zhang Q W, He G Z, Luan G Y, Cheng P J, Ruan X C, Zhu X H 2021 Power Laser and Particle Beams 33 0440

    [18]

    唐靖宇, 安琪, 白怀勇, 等 2019 原子能科学技术 53 2012

    Tang J Y, An Q, Bai H Y, et al. 2019 Atomic Energy Science and Technology 53 2012 (in Chinese)

    [19]

    An Q, Bai H Y, Bao J, et al. 2017 Journal of Instrumentation 12 7022

    [20]

    Tang J Y, Fu S N, Jing H T, Tang H Q, Wei J, Xia H H 2010 Chin. Phys. C 34 121Google Scholar

    [21]

    Jing H T, Tang J Y, Tang H Q, Xia H H, Liang T J, Zhou Z Y, Zhong Q P, Ruan X C 2010 Nucl. Instr. Meth. A 621 91Google Scholar

    [22]

    唐靖宇, 敬罕涛, 夏海鸿, 唐洪庆, 张闯, 周祖英, 阮锡超, 张奇玮, 杨征 2013 原子能科学技术 47 1089Google Scholar

    Tang J Y, Jing H T, Xia H H, Tang H Q, Zhang C, Zhou Z Y, Ruan X C, Zhang Q W, Yang Z 2013 Atomic Energy Science and Technology 47 1089Google Scholar

    [23]

    任杰, 阮锡超, 唐洪庆, 葛智刚, 黄翰雄, 敬罕涛, 唐靖宇, 黄蔚玲 2014 核技术 37 110521

    Ren J, Ruan X C, Tang H Q, Ge Z G, Huang H X, Jing H T, Tang J Y, Huang W L 2014 Nucl. Tech. 37 110521

    [24]

    Chen Y H, Luan G Y, Bao J, et al. 2019 Eur. Phys. J. A 55 115Google Scholar

    [25]

    鲍杰, 陈永浩, 张显鹏, 等 2019 68 080101Google Scholar

    Bao J, Chen Y H, Zhang X P, et al. 2019 Acta Phys. Sin. 68 080101Google Scholar

    [26]

    韩长材, 欧阳晓平, 张显鹏, 宋朝晖, 鲍杰, 严维鹏 2020 原子能科学技术 54 385Google Scholar

    Han C C, Ouyang X P, Zhang X P, Song Z H, Bao J, Yan W P 2020 Atomic Energy Science and Technology 54 385Google Scholar

    [27]

    马霄云, 仲启平, 周祖英, 等 2009 原子能科学技术 43 180

    Ma X Y, Zhong Q P, Zhou Z Y, et al. 2009 Atomic Energy Science and Technology 43 180

    [28]

    张奇玮, 贺国珠, 黄兴, 阮锡超, 李志宏, 朱兴华 2014 原子能科学技术 48 70

    Zhang Q W, He G Z, Huang X, Ruan X C, Li Z H, Zhu X H 2014 Atomic Energy Science and Technology 48 70

    [29]

    Yu T, Cao P, Ji X Y, et al. 2019 IEEE Transactions on Nuclear Science 66 1095Google Scholar

    [30]

    Wang Q, Cao P, Qi X, et al. 2018 Review of Scientific Instruments 89 013511Google Scholar

    [31]

    张奇玮, 贺国珠, 黄兴, 程品晶, 阮锡超, 朱兴华 2016 原子能科学技术 50 536Google Scholar

    Zhang Q W, He G Z, Huang X, Cheng P J, Ruan X C, Zhu X H 2016 Atomic Energy Science and Technology 50 536Google Scholar

    [32]

    张奇玮, 栾广源, 贺国珠, 程品晶, 阮锡超, 朱兴华 2020 原子核物理评论 37 771Google Scholar

    Zhang Q W, Luan G Y, He G Z, Cheng P J, Ruan X C, Zhu X H 2020 Nuclear Physics Review 37 771Google Scholar

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Metrics
  • Abstract views:  7543
  • PDF Downloads:  160
  • Cited By: 0
Publishing process
  • Received Date:  19 April 2021
  • Accepted Date:  05 July 2021
  • Available Online:  16 August 2021
  • Published Online:  20 November 2021

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