Semiclassical methods for strong field ionization of atoms

Xiao Xiang-Ru; Wang Mu-Xue; Li Min; Geng Ji-Wei; Liu Yun-Quan; Peng Liang-You

doi:10.7498/aps.65.220203

Abstract

As the advances of laser technology, more and more nonlinear phenomena are observed in the atoms and molecules driven by strong laser pulses. Systematic investigations on these findings, such as above threshold ionization and high-order harmonic generation, will lead us to understanding the mechanisms in the microscopic world. The most exact way to simulate the experimental measurements is to solve the time-dependent Schrdinger equation (TDSE) numerically, in which the system is described by the wave function and thus one cannot have an intuitive insight into the underling process. Therefore, several semiclassical methods have been developed to understand the strong field ionization. In the classical point of view, the electrons tunnel out when the strong laser field suppresses the Coulomb potential. Then the electrons are driven by the laser electric field according to the Newtonian equations. Semiclassical methods take into account the tunnelling of the electron, the classical orbit of the electron, and the action as the phase of trajectory, which have successfully explained main structures in the ionization spectrum. Two of the most popular semiclassical methods are the quantum trajectory Monte Carlo method and the Coulomb-corrected strong field approximation method. In the present review, we will introduce these basic methods and show how they have been developed step by step, covering the most relevant and important works in the strong field physics. Finally we give two example of applications to show how these methods work. With the advantage of the classical picture, we can identify different kind of structures in the 2D photoelectron momentum distributions and tell how the structures are formed. Nonadiabatic effects can be studied by comparing the results of the two methods, together with accurate simulation from the numerical solution of TDSE. The current semiclassical methods can be further developed into advanced ones, which can be used in more complex molecular systems or multi-electron systems, and be widely used in the study of dynamics of molecule and atoms in strong laser fields.

Keywords:

Authors and contacts

1.
State Key Laboratory for Mesoscopic Physics and School of Physics, Peking University, Beijing 100871, China;
2.
Wuhan National Laboratory for Optoelectronics and School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China;
3.
Collaborative Innovation Center of Quantum Matter, Beijing 100871, China

Corresponding author: Peng Liang-You, liangyou.peng@pku.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 11574010, 11322437) and the National Basic Research Program of China (Grant Nos. 2013CB922402, 2013CB922403).

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