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Rovibrational population transfer is controlled by a two-overlapping- pulse scheme in which the frequency ratio of the two pulses is 1:3. The calculated results show that nearly 100% of the population can be transferred from initial state |0,0to target state |3,1. The probability of population transfer can be controlled by pulse phase. When 1 =1.68 , the two pulses can be increased mutually and the probability of population transfer is also increased. When 1 =0.64 , the two pulses can be offset mutually and the probability of population transfer is reduced. The intensity of the second pulse has a significant effect on the population transfer.
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Keywords:
- population transfer /
- HF molecule /
- three photon transition /
- wave packet
[1] Shapiro E A, Shapiro M, Pe'er A, Ye J 2007 Phys. Rev. A 75 013405
[2] Magnier S, Persico M, Rahman N 1999 Phys. Rev. Lett. 83 2159
[3] Sussman B J, Townsend D, Ivanov M Y, Stolow A 2006 Science 314 278
[4] Serov V, Keller A, Atabek O, Figger H, Pavicic D 2005 Phys. Rev. A 72 033413
[5] Ma N, Wang M S, Yang C L, Xiong D L, Li X H, Ma X G 2010 Acta Phys. Sin. 59 215 (in Chinese) [马宁, 王美山, 杨传路, 熊德林, 李小虎, 马晓光 2010 59 215]
[6] Gao Y, Wu C Xu N, Zeng G, Jiang H, Yang H, Gong Q 2008 Phys. Rev. A 77 043404
[7] Liu Y Liu X, Deng Y, Wu C, Jiang H, Gong Q 2011 Phys. Rev. Lett. 106 073004
[8] Shu C C, Yu J, Yuan K J, Hu W H, Yang J, Cong S L 2009 Phys. Rev. A 79 023418
[9] Melinger J S, McMorrow, D, Hillegas C, Warren W S 1995 Phys. Rev. A 51 3366
[10] Mang L R, Ma J, Zhang L J, Xiao L T, Jia S T 2007 Acta Phys. Sin. 56 6373 (in Chinese) [汪丽蓉, 马杰, 张临杰, 肖连团, 贾锁堂 2007 56 6373]
[11] Remacle F, Levine R D 2006 Phys. Rev. A 73 033820
[12] Bergmann H T K, Shore B W 1998 Rev. Mod. Phys. 70 1003
[13] Wu C, Zeng G, Gao Y, Xu N, Peng L Y, Jiang H, Gong Q 2009 J. Chem. Phys. 130 231102
[14] Quack M, Stohner J 1993 J. Phys. Chem. 97 12574
[15] Niu Y Y, Wang S M, Cong S L 2006 Chem. Phys. Lett. 428 7
[16] Lin S H, Villaeys A A, Fujimura Y 2011 advances in multi-photon processes and spectroscopy (Vol. 20) (Singapore: World Scientific Press)pp53--94
[17] Combariza J E, Just B, Manz J, Paramonov G K 1991 J. Phys. Chem. 95 10351
[18] Vrábela I, Jakubetz W 2003 J. Chem. Phys. 118 7366
[19] Hornung T, Motzkus M, de Vivie-Riedle R 2002 Phys. Rev. A 65 021403(R)
[20] Shi S, Woody A, Rabitz H 1988 J. Chem. Phys. 88 6870
[21] Demkov Y N, Ostrovsky V N 2000 Phys. Rev. A 61 032705
[22] Chelkowski S, Bandrauk A D, Corkum P B 1990 Phys. Rev.Lett. 65 2355
[23] Gaubatz U, Rudecki P, Schiemann S, Bergmann K 1990 J. Chem. Phys. 92 5363
[24] Garraway B M, Suominen K A 1998 Phys. Rev. Lett. 80 932
[25] Korolkov M V, Paramonov G K 1997 Phys. Rev. A 56 3860
[26] Thomas S, Guérin S, Jauslin H R 2005 Phys. Rev. A 71 013402
[27] Niu Y Y, Wang R, Qiu M H 2010 Phys. Rev. A 81 043406
[28] Andrianov I V, Paramonov G K 1999 Phys. Rev. A 59 2134
[29] Ohmura H, Nakanaga T Tachiya M 2004 Phys. Rev. Lett. 92 113002
[30] Wang S M, Yuan K J, Niu Y Y, Han Y C, Cong S L 2006 Phys. Rev. A 74 043406
[31] Marston CC, Balint-Kurti G G 1989 J. Chem. Phys. 91 3571
[32] Feit M D, Fleck J A, Jr, Steiger A 1982 J. Comput. Phys. 47 412
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[1] Shapiro E A, Shapiro M, Pe'er A, Ye J 2007 Phys. Rev. A 75 013405
[2] Magnier S, Persico M, Rahman N 1999 Phys. Rev. Lett. 83 2159
[3] Sussman B J, Townsend D, Ivanov M Y, Stolow A 2006 Science 314 278
[4] Serov V, Keller A, Atabek O, Figger H, Pavicic D 2005 Phys. Rev. A 72 033413
[5] Ma N, Wang M S, Yang C L, Xiong D L, Li X H, Ma X G 2010 Acta Phys. Sin. 59 215 (in Chinese) [马宁, 王美山, 杨传路, 熊德林, 李小虎, 马晓光 2010 59 215]
[6] Gao Y, Wu C Xu N, Zeng G, Jiang H, Yang H, Gong Q 2008 Phys. Rev. A 77 043404
[7] Liu Y Liu X, Deng Y, Wu C, Jiang H, Gong Q 2011 Phys. Rev. Lett. 106 073004
[8] Shu C C, Yu J, Yuan K J, Hu W H, Yang J, Cong S L 2009 Phys. Rev. A 79 023418
[9] Melinger J S, McMorrow, D, Hillegas C, Warren W S 1995 Phys. Rev. A 51 3366
[10] Mang L R, Ma J, Zhang L J, Xiao L T, Jia S T 2007 Acta Phys. Sin. 56 6373 (in Chinese) [汪丽蓉, 马杰, 张临杰, 肖连团, 贾锁堂 2007 56 6373]
[11] Remacle F, Levine R D 2006 Phys. Rev. A 73 033820
[12] Bergmann H T K, Shore B W 1998 Rev. Mod. Phys. 70 1003
[13] Wu C, Zeng G, Gao Y, Xu N, Peng L Y, Jiang H, Gong Q 2009 J. Chem. Phys. 130 231102
[14] Quack M, Stohner J 1993 J. Phys. Chem. 97 12574
[15] Niu Y Y, Wang S M, Cong S L 2006 Chem. Phys. Lett. 428 7
[16] Lin S H, Villaeys A A, Fujimura Y 2011 advances in multi-photon processes and spectroscopy (Vol. 20) (Singapore: World Scientific Press)pp53--94
[17] Combariza J E, Just B, Manz J, Paramonov G K 1991 J. Phys. Chem. 95 10351
[18] Vrábela I, Jakubetz W 2003 J. Chem. Phys. 118 7366
[19] Hornung T, Motzkus M, de Vivie-Riedle R 2002 Phys. Rev. A 65 021403(R)
[20] Shi S, Woody A, Rabitz H 1988 J. Chem. Phys. 88 6870
[21] Demkov Y N, Ostrovsky V N 2000 Phys. Rev. A 61 032705
[22] Chelkowski S, Bandrauk A D, Corkum P B 1990 Phys. Rev.Lett. 65 2355
[23] Gaubatz U, Rudecki P, Schiemann S, Bergmann K 1990 J. Chem. Phys. 92 5363
[24] Garraway B M, Suominen K A 1998 Phys. Rev. Lett. 80 932
[25] Korolkov M V, Paramonov G K 1997 Phys. Rev. A 56 3860
[26] Thomas S, Guérin S, Jauslin H R 2005 Phys. Rev. A 71 013402
[27] Niu Y Y, Wang R, Qiu M H 2010 Phys. Rev. A 81 043406
[28] Andrianov I V, Paramonov G K 1999 Phys. Rev. A 59 2134
[29] Ohmura H, Nakanaga T Tachiya M 2004 Phys. Rev. Lett. 92 113002
[30] Wang S M, Yuan K J, Niu Y Y, Han Y C, Cong S L 2006 Phys. Rev. A 74 043406
[31] Marston CC, Balint-Kurti G G 1989 J. Chem. Phys. 91 3571
[32] Feit M D, Fleck J A, Jr, Steiger A 1982 J. Comput. Phys. 47 412
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