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Multiferroic xNFO-(1-x)BFO (x =0.00 0.10, 0.15, 0.20, 0.25) composite films are prepared through self-assembling growth on Au/Ti/SiO2/Si substrates by chemical solution deposition (CSD). X-ray diffraction analysis shows that the perovskite BiFeO3 and the spinel structured NiFe2O4 phases are formed and separated. The leakage current density (J) in the film decreases and the remnant polarizations (M r) increases with the introduction of NFO. The value of J in 0.25NFO—0.75BFO film is found to be nearly two orders of magnitude lower than that in the BFO film, and the M r and the saturation magnetization ( M s) reach maxima, i.e. 2.3μC/cm2 and 70.2 kA·m-1, respectively. Therefore, from the calculation for magnetic moment of NFO we can conjecture that magnetoelectric coupling exists in the composite films.
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Keywords:
- multiferroic composite films /
- magnetoelectric coupling /
- ferroelectric properties /
- magnetic properties
[1] Wood V E, Austin A E 1974 Int. J. Magn. 5 303
[2] Wang J, Neaton J B, Zheng H, Nagarajan V, Ogale S B, Liu B, Viehland D, Vaithyanathan V, Schlom D G, Waghmare U V, Spaldin N A, Rabe K M, Wuttig M, Ramesh R 2003 Science 299 1719
[3] Zavaliche F, Zheng H, Mohaddes-Ardabili L, Yang S Y, Zhan Q, Shafer P, Reilly E, Chopdekar R, Jia Y, Wright P, Schlom D G, Suzuki Y, Ramesh R 2005 Nano Lett. 5 1793
[4] Dix N, Muralidharan R, Caicedo J M, Hrabovsky D, Fina I, Fabrega L, Skumryev V, Varela M, Guyonnet J, Paruch P, Sanchez F, Fontcuberta J 2009 J. Magn. Magn. Mater. 321 1790
[5] Zheng H, Straub F, Zhan Q, Yang P L, Hsieh W K, Zavaliche F, Chu Y H, Dahmen U, Ramesh R 2006 Adv. Mater. 18 2747
[6] Kanamadi C M, Kim J S, Yang H K 2009 J. Alloys Compd. 481 781
[7] Dix N, Muralidharan R, Guyonnet J, Warot-Fonrose B, Varela M, Paruch P, Snchez F, Fontcuberta J 2009 Appl. Phys. Lett. 95 062907.
[8] Liu X M, Fu S Y, Huang C J 2005 Mater. Sci. Eng B 121 255
[9] Smolenskii G A, Chupis I E 1982 Sov. Phys. Usp. 25 475
[10] Sun Y, Huang Z F, Fan H G, Ming X, Wang C Z, Chen G 2009 Acta Phys. Sin. 58 193(in Chinese)[孙 源、黄祖飞、范厚刚、明 星、王春忠、陈 岗 2009 58 193]
[11] Schwartz R W, Schneller T, Waser R 2004 C. R. Chimie. 7 433
[12] Garino T J, Harrington M, Kingon A I, Myers E R, Tuttle B 1992 Mater. Res. Soc. Symp. Proc. 243 341
[13] Zheng H, Zhan Q, Zavaliche F, Sherburne M, Straub F, Cruz M P, Chen L, Dahmen U, Ramesh R 2006 Nano Lett. 6 1401
[14] Zavaliche F, Yang S Y, Shafer P, Ramesh R, Das R R, Kim D M, Eom C B 2005 Appl. Phys. Lett. 87 182912.
[15] Zhong C G, Jiang Q, Fang J H, Ge C W 2009 Acta Phys. Sin. 58 3491(in Chinese)[仲崇贵、蒋 青、方靖淮、葛存旺 2009 58 3491]
[16] Ruette B, Zvyagin S, Pyatakov A P, Bush A, Li J F , Belotelov V I, Zvezdin A K, Viehland D 2004 Phys. Rev. B 69 064114
[17] Zhang S T, Ding L Y, Lu M H, Luo Z L 2008 Solid State Commun. 148 420
[18] Zhang Z T, Rondinone A J, Ma J X, Shen J, Dai S 2005 Adv. Mater. 17 1415
[19] Kinemuchi Y, Ishizaka K, Suematsu H, Jiang W, Yatsui K 2002 Thin Solid Films 407 109
[20] Park T J, Papaefthymiou G C, Viescas A J, Moodenbaugh A R, Wong S S 2007 Nano Lett. 7 766
[21] Zhang H, Kajiyoshi K 2010 J. Am. Ceram. Soc. 93 3842
[22] Kumar M, Yadav K L 2007 J. Phys. Chem. Solids 68 1791
[23] Sun P N, Cui L, Lü T Q 2009 Chin. Phys. B 18 1658
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[1] Wood V E, Austin A E 1974 Int. J. Magn. 5 303
[2] Wang J, Neaton J B, Zheng H, Nagarajan V, Ogale S B, Liu B, Viehland D, Vaithyanathan V, Schlom D G, Waghmare U V, Spaldin N A, Rabe K M, Wuttig M, Ramesh R 2003 Science 299 1719
[3] Zavaliche F, Zheng H, Mohaddes-Ardabili L, Yang S Y, Zhan Q, Shafer P, Reilly E, Chopdekar R, Jia Y, Wright P, Schlom D G, Suzuki Y, Ramesh R 2005 Nano Lett. 5 1793
[4] Dix N, Muralidharan R, Caicedo J M, Hrabovsky D, Fina I, Fabrega L, Skumryev V, Varela M, Guyonnet J, Paruch P, Sanchez F, Fontcuberta J 2009 J. Magn. Magn. Mater. 321 1790
[5] Zheng H, Straub F, Zhan Q, Yang P L, Hsieh W K, Zavaliche F, Chu Y H, Dahmen U, Ramesh R 2006 Adv. Mater. 18 2747
[6] Kanamadi C M, Kim J S, Yang H K 2009 J. Alloys Compd. 481 781
[7] Dix N, Muralidharan R, Guyonnet J, Warot-Fonrose B, Varela M, Paruch P, Snchez F, Fontcuberta J 2009 Appl. Phys. Lett. 95 062907.
[8] Liu X M, Fu S Y, Huang C J 2005 Mater. Sci. Eng B 121 255
[9] Smolenskii G A, Chupis I E 1982 Sov. Phys. Usp. 25 475
[10] Sun Y, Huang Z F, Fan H G, Ming X, Wang C Z, Chen G 2009 Acta Phys. Sin. 58 193(in Chinese)[孙 源、黄祖飞、范厚刚、明 星、王春忠、陈 岗 2009 58 193]
[11] Schwartz R W, Schneller T, Waser R 2004 C. R. Chimie. 7 433
[12] Garino T J, Harrington M, Kingon A I, Myers E R, Tuttle B 1992 Mater. Res. Soc. Symp. Proc. 243 341
[13] Zheng H, Zhan Q, Zavaliche F, Sherburne M, Straub F, Cruz M P, Chen L, Dahmen U, Ramesh R 2006 Nano Lett. 6 1401
[14] Zavaliche F, Yang S Y, Shafer P, Ramesh R, Das R R, Kim D M, Eom C B 2005 Appl. Phys. Lett. 87 182912.
[15] Zhong C G, Jiang Q, Fang J H, Ge C W 2009 Acta Phys. Sin. 58 3491(in Chinese)[仲崇贵、蒋 青、方靖淮、葛存旺 2009 58 3491]
[16] Ruette B, Zvyagin S, Pyatakov A P, Bush A, Li J F , Belotelov V I, Zvezdin A K, Viehland D 2004 Phys. Rev. B 69 064114
[17] Zhang S T, Ding L Y, Lu M H, Luo Z L 2008 Solid State Commun. 148 420
[18] Zhang Z T, Rondinone A J, Ma J X, Shen J, Dai S 2005 Adv. Mater. 17 1415
[19] Kinemuchi Y, Ishizaka K, Suematsu H, Jiang W, Yatsui K 2002 Thin Solid Films 407 109
[20] Park T J, Papaefthymiou G C, Viescas A J, Moodenbaugh A R, Wong S S 2007 Nano Lett. 7 766
[21] Zhang H, Kajiyoshi K 2010 J. Am. Ceram. Soc. 93 3842
[22] Kumar M, Yadav K L 2007 J. Phys. Chem. Solids 68 1791
[23] Sun P N, Cui L, Lü T Q 2009 Chin. Phys. B 18 1658
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