聚合物结晶理论进展

严大东; 张兴华

doi:10.7498/aps.65.188201

摘要

本文简要回顾了高分子结晶理论发展的历史. 在介绍传统的Hoffman-Lauritzen理论的基础上，总结了近年来高分子结晶实验特别是X光散射实验方面的最新进展. 介绍了建立在这些实验基础之上的一些新的结晶理论，主要代表工作包括Strobl的中介相模型、Olmsted的spinodal辅助结晶理论、Muthukuamr的分子模拟与成核理论等.

关键词:

聚合物 /
结晶 /
理论 /
模拟

In this paper, the history and the recent development of polymer crystallization have been reviewed briefly. After introducing the conventional Hoffman-Lauritzen theory, the recent new experimental results, especially on X-ray scattering, have been summarized. Some new models of crystallization have been reviewed, such as Strobl's mesomorphic phase model, Olmsted's spinodal-assisted crystallization theory, and Muthukumar's molecular modeling of polymer crystallization.

Keywords:

polymer /
crystallization /
theory /
simulation

作者及机构信息

严大东¹,
张兴华²

1.
北京师范大学物理系, 北京 100875;

2.
北京交通大学理学院, 北京 100044

通信作者: 严大东, yandd@bnu.edu.cn

基金项目: 国家自然科学基金(批准号: 21374011, 21434001)资助的课题.

Authors and contacts

Yan Da-Dong¹,
Zhang Xing-Hua²

1.
Department of Physics, Beijing Normal University, Beijing 100875, China;

2.
School of Science, Beijing Jiaotong University, Beijing 100044, China

Corresponding author: Yan Da-Dong, yandd@bnu.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 21374011, 21434001).

参考文献

[1]	Faraday-Discussion 1979 Organization of Macromolecules in the Condensed Phase (Faraday discussions of the Chemical Society) (Faraday Division, Chemical Society) 85
[2]	Lauritzen J I, Hoffman J D 1961 J. Res. Natl. Bur. Stand. Sect. A 64 73
[3]	Lauritzen J I, Hoffman J D 1961 J. Res. Natl. Bur. Stand. Sect. A 65 297
[4]	Hoffman J D, Davis G T, Lauritzen J I 1976 in Treaties on Solid State Chemistry (Ed. by N. B. Hannay) (Vol. 3) (New York: Plenum) p497
[5]	Rastogi S, Hikosaka M, Kawabata H, Keller A 1991 Macromolecules 24 6384
[6]	Keller A, Hikosaka M, Rastogi S, Toda A, Barham P, Goldbeck-Wood G 1994 J. Mater. Sci. 29 2579
[7]	Imai M, Kaji K, Kanaya T, Sakai Y 1995 Phys. Rev. B 52 12696
[8]	Hauser G, Schmidtke J, Strobl G 1998 Macromolecules 31 6250
[9]	Olmsted P D, Poon W C K, McLeish T C B, Terrill N J, Ryan A J 1998 Phys. Rev. Lett. 81 373
[10]	Liu C, Muthukumar M 1998 J. Chem. Phys. 109 2563
[11]	Muthukumar M, Welch P 2000 Polymer 41 8833
[12]	Welch P, Muthukumar M 2000 Phys. Rev. Lett. 87 218302
[13]	Muthukumar M 2003 Phil. Trans. R. Soc. Lond. A 361 539
[14]	Muthukumar M 2005 Adv. Polym. Sci. 191 241
[15]	Strobl G 2000 Eur. Phys. J. E 3 165
[16]	Strobl G 2009 Rev. Mod. Phys. 81 1287
[17]	Strobl G 2007 The Physics of Polymer (New York: Springer)
[18]	Bassett D C 1981 Principles of Polymer Morphology (Cambridge: Cambridge University Press)
[19]	Hoffman J D, Miller R L 1997 Polymer 38 3151
[20]	Imai M, Mori K, Mizukami T, Kaji K, Kanaya T 1992 Polymer 33 4457
[21]	Imai M, Kaji K, Kanaya T 1993 Phys. Rev. Lett. 71 4162
[22]	Imai M, Kaji K, Kanaya T 1994 Macromolecules 27 7102
[23]	Ezquerra T A, Lopezcabarcos E, Hsiao B S, Baltacalleja F J 1996 Phys. Rev. E 54 989
[24]	Terrill N J, Fairclough J P A, Komanschek B U, Young R J, Ryan A J 1998 Polymer 39 2381
[25]	Kaji K, Nishida K, Kanay T, Mstsuba G, Konishi T, Imai M 2005 Adv. Polym. Sci. 12 13
[26]	Tan H G, Miao B, Yan D D 2003 J. Chem. Phys. 19 2886
[27]	Gee R H, Lacevic N, Fried L 2006 Nature Mater. 5 39
[28]	Tang J Z, Zhang X H, Yan D D 2015 J. Chem. Phys. 143 204903
[29]	Jiang Y, Yan D D, Gao X, Han C C, Jin X G, Li L, WangY, Chan C M 2003 Macromolecules 36 3652

施引文献

[1]	Faraday-Discussion 1979 Organization of Macromolecules in the Condensed Phase (Faraday discussions of the Chemical Society) (Faraday Division, Chemical Society) 85
[2]	Lauritzen J I, Hoffman J D 1961 J. Res. Natl. Bur. Stand. Sect. A 64 73
[3]	Lauritzen J I, Hoffman J D 1961 J. Res. Natl. Bur. Stand. Sect. A 65 297
[4]	Hoffman J D, Davis G T, Lauritzen J I 1976 in Treaties on Solid State Chemistry (Ed. by N. B. Hannay) (Vol. 3) (New York: Plenum) p497
[5]	Rastogi S, Hikosaka M, Kawabata H, Keller A 1991 Macromolecules 24 6384
[6]	Keller A, Hikosaka M, Rastogi S, Toda A, Barham P, Goldbeck-Wood G 1994 J. Mater. Sci. 29 2579
[7]	Imai M, Kaji K, Kanaya T, Sakai Y 1995 Phys. Rev. B 52 12696
[8]	Hauser G, Schmidtke J, Strobl G 1998 Macromolecules 31 6250
[9]	Olmsted P D, Poon W C K, McLeish T C B, Terrill N J, Ryan A J 1998 Phys. Rev. Lett. 81 373
[10]	Liu C, Muthukumar M 1998 J. Chem. Phys. 109 2563
[11]	Muthukumar M, Welch P 2000 Polymer 41 8833
[12]	Welch P, Muthukumar M 2000 Phys. Rev. Lett. 87 218302
[13]	Muthukumar M 2003 Phil. Trans. R. Soc. Lond. A 361 539
[14]	Muthukumar M 2005 Adv. Polym. Sci. 191 241
[15]	Strobl G 2000 Eur. Phys. J. E 3 165
[16]	Strobl G 2009 Rev. Mod. Phys. 81 1287
[17]	Strobl G 2007 The Physics of Polymer (New York: Springer)
[18]	Bassett D C 1981 Principles of Polymer Morphology (Cambridge: Cambridge University Press)
[19]	Hoffman J D, Miller R L 1997 Polymer 38 3151
[20]	Imai M, Mori K, Mizukami T, Kaji K, Kanaya T 1992 Polymer 33 4457
[21]	Imai M, Kaji K, Kanaya T 1993 Phys. Rev. Lett. 71 4162
[22]	Imai M, Kaji K, Kanaya T 1994 Macromolecules 27 7102
[23]	Ezquerra T A, Lopezcabarcos E, Hsiao B S, Baltacalleja F J 1996 Phys. Rev. E 54 989
[24]	Terrill N J, Fairclough J P A, Komanschek B U, Young R J, Ryan A J 1998 Polymer 39 2381
[25]	Kaji K, Nishida K, Kanay T, Mstsuba G, Konishi T, Imai M 2005 Adv. Polym. Sci. 12 13
[26]	Tan H G, Miao B, Yan D D 2003 J. Chem. Phys. 19 2886
[27]	Gee R H, Lacevic N, Fried L 2006 Nature Mater. 5 39
[28]	Tang J Z, Zhang X H, Yan D D 2015 J. Chem. Phys. 143 204903
[29]	Jiang Y, Yan D D, Gao X, Han C C, Jin X G, Li L, WangY, Chan C M 2003 Macromolecules 36 3652

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