高功率脉冲电子束辐照SiO2的光学和激光损伤性能

钟勉; 杨亮; 任玮; 向霞; 刘翔; 练友运; 徐世珍; 郭德成; 郑万国; 袁晓东

doi:10.7498/aps.63.246103

摘要

研究了不同剂量的60 kW高功率脉冲电子束辐照对高纯熔石英玻璃的微观结构、光学性能和激光损伤特性的影响规律. 光学显微图像表明, 辐照后熔石英样品由于热效应导致表面破裂, 裂纹密度和尺寸随辐照剂量增加而增大, 采用原子力显微镜分析表面裂纹的微观形貌, 裂纹宽度约1 um, 同时样品表面分布着大量尺寸约0.1–1μm的碎片颗粒. 吸收光谱测试表明, 所有样品均在394 nm处出现微弱的吸收峰, 吸收强度随着电子束辐照剂量增大呈现先增加后减小的趋势. 荧光光谱测试发现辐照前后样品均有3个荧光带, 分别位于460, 494和520 nm, 荧光强度随辐照剂量的变化趋势与吸收光谱一致. 利用355 nm激光研究了不同剂量电子束辐照对熔石英激光损伤阈值的影响, 结果表明熔石英的损伤阈值随着辐照剂量的增加而降低. 在剂量较低时, 导致熔石英激光损伤阈值下降的原因主要是色心缺陷; 剂量较高时, 导致损伤阈值降低的原因主要是样品表面产生的大量微裂纹和碎片颗粒对激光的调制和吸收.

关键词:

Abstract

A 60 kW electron beam is used to study the microstructure and optical property evolutions as well as laser induced damage threshold of fused silica after irradiation at room temperature. Optical microscopic results indicate that cracks appear at the surface of SiO2 after electron beam irradiation, owing to the thermal effect, and that the crack density and size increase with increasing radiation dose. The morphology of the surface cracks is analyzed by using atomic force microscope and the width of crack is about 1 μm. In addition, there are a large number of debris particles with sizes of 0.1-1 μm on the surface. From the optical absorption spectrum of each of all samples, a weak absorption peak at 394 nm is observed and the absorbance increases at the beginning then decreases with increasing electron-radiation dose. Before and after irradiation, three absorption bands at 460 nm, 496 nm and 520 nm are clearly observed and their intensities first increase and then decrease, which is consistent with the results of absorption spectra. The effect of electron dose on the laser induced damage threshold (LIDT) at 355 nm is investigated and the results indicate that the LIDT decreases with increasing dose. At the lower electron doses, the color centers are responsible for the decrease of LIDT. However, at the higher electron doses, the decrease of LIDT is due to the light modulation and absorption induced by microscale cracks and debris particles at the surface of irradiated fused silica.

Keywords:

作者及机构信息

1.
电子科技大学物理电子学院, 成都 610054;

2.
核工业西南物理研究院, 成都 610041;

3.
中国工程物理研究院激光聚变研究中心, 绵阳 621900

基金项目: 国家自然科学基金(批准号: 61178018)和中央高校基本科研业务费(批准号: ZYGX2012J057)资助的课题.

Authors and contacts

1.
School of Physical Electronics, University of Electronic Science and Technology of China, Chengdu 610054, China;

2.
Center for Fusion Science of Southwestern Institute of Physics, Chengdu 610041, China;

3.
Research Center of Laser Fusion, China Academy of Engineering Physics, Mianyang 621900, China

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 61178018) and the Fundamental Research Fund for the Central Universities, China (Grant No. ZYGX2012J057).

参考文献

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[33]	Lin J, Huang Y, Zhang J, Gao J M, Ding X X, Huang Z X, Tang C C, Hu L, Chen D F 2007 Chem. Mater. 19 2585
[34]	Hua J R, Zu X T, Li L, Xiang X, Chen M, Jiang X D, Yuan X D, Zheng W G 2010 Acta Phys. Sin. 59 2519 (in Chinese) [花金荣, 祖小涛, 李莉, 向霞, 陈猛, 蒋晓东, 袁晓东, 郑万国 2010 59 2519]
[35]	Hua J R, Li L, Xiang X, Zu X T 2011 Acta Phys. Sin. 60 044206 (in Chinese) [花金荣, 李莉, 向霞, 祖小涛 2011 60 044206]
[36]	Jiang Y 2012 Ph. D. Dissertation (Chengdu: University of Electronic Science and Technology of China) (in Chinese) [蒋勇 2012 博士学位论文 (成都: 电子科技大学)]

施引文献

[1]	Holtkamp N 2007 Fusion Eng. Des. 82 427
[2]	Ibarra A, Hodgson E R 2004 Nucl. Instrum. Meth. B 218 29
[3]	Yamamoto S, Shikama T, Belyakov V, Farnum E, Hodgson E, Nishitani T, Costley A, de Kock L, Walker C, Janeschitz G, 2000 J. Nucl. Mater. 283 60
[4]	Campbell J H, Hawley-Fedder R A, Stolz C J, Menapace J A, Borden M R, Whitman P K, Yu J, Runkel M J, Riley M O, Feit M D 2004 Proc. SPIE 5341 San Jose, USA, January 24-29, 2004 p84
[5]	Devine R A 1993 J. Non-Cryst. Solids. 152 50
[6]	Manzano J, Morono A, Hodgson E R 2009 Fusion Eng. Des. 84 1245
[7]	González S, Morono A, Hodgson E R 2005 Fusion Eng. Des. 74 831
[8]	León M, Martín P, Bravo D, López F, Ibarra A, Rascón A, Mota F 2008 J. Nucl. Mater. 374 386
[9]	León M, Martín P, Vila R, Molla J, Ibarra A 2009 Fusion Eng. Des. 84 1174
[10]	Galeener F L, Kerwin D B, Miller A J, Mikkelsen J C 1993 Phys. Rev. B 47 7760
[11]	N uritdinov I, Masharipov K Y, Doniev M 2003 Glass Phys. Chem. 29 11
[12]	Cannas M, Agnello S, Gelardi F, Boscaino R, Trukhin A, Liblik P, Lushchik C, Kink M, Maksimov Y, Kink R 2004 J. Phys.: Condens. Matter 16 7931
[13]	Martín P, León M, Ibarra A, Hodgson E R 2011 J. Nucl. Mater. 417 818
[14]	Fitting H J, Barfels T, Von Czarnowski A, Trukhin A N 2000 Mater. Sci. Eng. B 71 109
[15]	D' Amico M, Messina F, Cannas M, Leone M, Boscaino R 2009 Phys. Rev. B 79 064203
[16]	Nuccio L, Agnello S, Boscaino R, Boizot B, Parlato A 2007 J. Non-Cryst. Solids 353 581
[17]	Zoubir A, Rivero C, Grodsky R, Richardson K, Richardson M, Cardinal T, Couzi M 2006 Phys. Rev. B 73 224117
[18]	Sergeev P B, Sergeev A P, Zvorykin V D 2007 Quantum Electron. 37 711
[19]	Sergeev P B, Sergeev A P 2010 Quantum Electron. 40 804
[20]	Guizard S, Martin P, Petite G, D'Oliveira P, Meynadier P 1996 J. Phys.: Condens. Matter 8 1281
[21]	Skuja L, Hirano M, Hosono H, Kajihara K 2005 Phys. Stat. Sol. 2 15
[22]	Griscom D L 1991 J. Ceram. Soc. Jpn. 99 923
[23]	Chen L, Wang T S, Zhang G F, Yang K J, Peng H B, Zhang L M 2013 Chin. Phys. B 22 126101
[24]	Lian Y Y, Liu X, Xu Z Y, Song J P, Yu Y 2013 Fusion Eng. Des. 88 1694
[25]	Chen X Q, Zu X T, Zheng W G, Jiang X D, L H B, Ren H, Zhang Y Z, Liu C M 2006 Acta Phys. Sin. 55 1201 (in Chinese) [陈习权, 祖小涛, 郑万国, 蒋晓东, 吕海兵, 任寰, 张艳珍, 刘春明 2006 55 1201]
[26]	Wang P W, Kimberlin K R, Chengyu W, Ying T, Lin G Q, Aimin W, Jun X J 2005 Mater. Chem. Phys. 94 252
[27]	Skuja L 1994 J. Non-Cryst. Solids 167 229
[28]	Skuja L 1998 J. Non-Cryst. Solids 239 16
[29]	Skuja L, Streletsky A, Pakovich A 1984 Solid State Commun. 50 1069
[30]	Sakurai Y 2006 J. Non-Cryst. Solids 352 2917
[31]	Sakurai Y, Nagasawa K 2001 J. Non-Cryst. Solids 291 86
[32]	Wang F, Qin X F, Ren S H, Yang L X, Meng Y F, Ming Y F 2013 Mater. Res. Bull. 48 3640
[33]	Lin J, Huang Y, Zhang J, Gao J M, Ding X X, Huang Z X, Tang C C, Hu L, Chen D F 2007 Chem. Mater. 19 2585
[34]	Hua J R, Zu X T, Li L, Xiang X, Chen M, Jiang X D, Yuan X D, Zheng W G 2010 Acta Phys. Sin. 59 2519 (in Chinese) [花金荣, 祖小涛, 李莉, 向霞, 陈猛, 蒋晓东, 袁晓东, 郑万国 2010 59 2519]
[35]	Hua J R, Li L, Xiang X, Zu X T 2011 Acta Phys. Sin. 60 044206 (in Chinese) [花金荣, 李莉, 向霞, 祖小涛 2011 60 044206]
[36]	Jiang Y 2012 Ph. D. Dissertation (Chengdu: University of Electronic Science and Technology of China) (in Chinese) [蒋勇 2012 博士学位论文 (成都: 电子科技大学)]

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