Molecular orbital imaging with high spatial and temperal resolutions

Zhu Xiao-Song; Zhang Qing-Bin; Lan Peng-Fei; Lu Pei-Xiang

doi:10.7498/aps.65.224207

Abstract

When atoms and molecules are excited by ultrashort laser pulses, highly nonlinear strong-field processes like above-threshold ionization and high harmonic generation occur. By analyzing the emitted light and electron signals, the atomic and molecular structures and ultrafast dynamics can be detected with a combination of Angstrom spatial resolution and sub-femtosecond temporal resolution, which provides a powerful tool to study the basic structures and physical processes in the microscopic world. The molecular orbital tomography (MOT) developed since 2004 enables one to image the wavefunction of the molecular orbital itself, which will help people gain deeper insight into the chemical reactions. In this paper, the theory of MOT will be introduced, and the progresses of MOT in the past ten years will be reviewed.

Keywords:

Authors and contacts

1.
School of Physics and Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, China;
2.
Laboratory of Optical Information Technology, Wuhan Institute of Technology, Wuhan 430205, China

Corresponding author: Lan Peng-Fei, pengfeilan@mail.hust.edu.cn;lupeixiang@mail.hust.edu.cn ; Lu Pei-Xiang, pengfeilan@mail.hust.edu.cn;lupeixiang@mail.hust.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 11404123, 11234004, 61275126, 11422435, 11574101).

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Cited By

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[9]	Li W, Zhou X, Lock R, Patchkovskii S, Stolow A, Kapteyn H C, Murnane M M 2008Science 322 1207
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[11]	Lein M 2007J. Phys. B:At. Mol. Opt. Phys. 40 R135
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