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The dynamics of multi-photon ionization of CH3I under strong field has been studied experimentally by femtosecond photoelectron imaging. Ultrafast optical control of the vibrational excitation in a polyatomic ion by strong field multi-photon ionization is experimentally realized. The present work enhances the intensity of the ionization beam from 1.6×1013 to 2.5×1013 W/cm2. In the order of this higher field, a new energy component is observed and attributed. From the photoelectron imaging, photoelectron kinetic energy distributions and the photoelectron angular distributions are obtained. The discussions of the previous letter are mostly based on the photoelectron kinetic energy information, and the present study emphasizes on the trend of the photoelectron angular anisotropy. More detailed dynamics on vibrational optical control is further explored.
[1] Smith S J, Knight P L 1988 Multiphoton Processes (Cambridge: Cambridge University Press)
[2] Freeman R R, Bucksbaum P H, Milchberg H, Darack S, Schumacher D, Geusic M E 1987 Phys. Rev. Lett. 59 1092
[3] Freeman R R, Bucksbaum P H 1991 J. Phys. B: At. Mol. Opt. Phys. 24 325
[4] Kang H P, Wang C L, Lin Z Y, Chen Y J, Wu M Y, Quan W, Liu H P, Liu X J 2011 Chin. Phys. Lett. 28 083201
[5] Lin Z Y, Wu M Y, Quan W, Liu X J, Chen J, Cheng Y 2014 Chin. Phys. B 23 023201
[6] Alber G 1989 Phys. Rev. A 40 1321
[7] Potvliege R M, Vucic S 2006 Phys. Scr. 74 55
[8] Mevel E, Breger P, Trainham R, Petite G, Agostini P, Chambaret J P, Migus A, Antonetti A 1992 J. Phys. B: At. Mol. Opt. Phys. 25 401
[9] Posthumus J H 2004 Rep. Prog. Phys. 67 623
[10] Urbain X, Fabre B, Staicu-Casagrande E M, Ruette N, Andrianarijaona V M, Jureta J, Posthumus J H 2004 Phys. Rev. Lett. 92 163004
[11] Posthumus J H, Fabre B, Cornaggia C, Ruette N, Urbain X 2008 Phys. Rev. Lett. 101 233004
[12] Liu Y, Gerber T, Radi P, Sych Y, Knopp G 2014 Chem. Phys. Lett. 610–611 153
[13] Liu Y, Knopp G, Hemberger P, Sych Y, Radi P, Boedi A, Gerber T 2013 Phys. Chem. Chem. Phys. 15 18101
[14] Liu Y, Gerber T, Radi P, Sych Y, Knopp G 2013 Opt. Express 21 16639
[15] Liu Y Z, Xiao S R, Zhang C Y, Zheng G G, Chen Y Y 2012 Acta Phys. Sin. 61 193301 (in Chinese) [刘玉柱, 肖韶荣, 张成义, 郑改革, 陈云云 2012 61 193301]
[16] Eppink A T J B, Parker D H 1999 J. Chem. Phys. 110 832
[17] Walser A M, Meisinger M, Radi P, Gerber T, Knopp G 2009 Phys. Chem. Chem. Phys. 11 8456
[18] Gerber T, Liu Y, Knopp G, Hemberger P, Boedi A, Radi P, Sych Y 2013 Rev. Sci. Instrum. 84 033101
[19] Yang C N 1948 Phys. Rev. 74 764
[20] Seideman T 1999 Phys. Rev. Lett. 83 4971
[21] Reid K L 2003 Annu. Rev. Phys. Chem. 54 397
[22] Suzuki Y I, Horio T, Fuji T, Suzuki T 2011 J. Chem. Phys. 134 184313
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[1] Smith S J, Knight P L 1988 Multiphoton Processes (Cambridge: Cambridge University Press)
[2] Freeman R R, Bucksbaum P H, Milchberg H, Darack S, Schumacher D, Geusic M E 1987 Phys. Rev. Lett. 59 1092
[3] Freeman R R, Bucksbaum P H 1991 J. Phys. B: At. Mol. Opt. Phys. 24 325
[4] Kang H P, Wang C L, Lin Z Y, Chen Y J, Wu M Y, Quan W, Liu H P, Liu X J 2011 Chin. Phys. Lett. 28 083201
[5] Lin Z Y, Wu M Y, Quan W, Liu X J, Chen J, Cheng Y 2014 Chin. Phys. B 23 023201
[6] Alber G 1989 Phys. Rev. A 40 1321
[7] Potvliege R M, Vucic S 2006 Phys. Scr. 74 55
[8] Mevel E, Breger P, Trainham R, Petite G, Agostini P, Chambaret J P, Migus A, Antonetti A 1992 J. Phys. B: At. Mol. Opt. Phys. 25 401
[9] Posthumus J H 2004 Rep. Prog. Phys. 67 623
[10] Urbain X, Fabre B, Staicu-Casagrande E M, Ruette N, Andrianarijaona V M, Jureta J, Posthumus J H 2004 Phys. Rev. Lett. 92 163004
[11] Posthumus J H, Fabre B, Cornaggia C, Ruette N, Urbain X 2008 Phys. Rev. Lett. 101 233004
[12] Liu Y, Gerber T, Radi P, Sych Y, Knopp G 2014 Chem. Phys. Lett. 610–611 153
[13] Liu Y, Knopp G, Hemberger P, Sych Y, Radi P, Boedi A, Gerber T 2013 Phys. Chem. Chem. Phys. 15 18101
[14] Liu Y, Gerber T, Radi P, Sych Y, Knopp G 2013 Opt. Express 21 16639
[15] Liu Y Z, Xiao S R, Zhang C Y, Zheng G G, Chen Y Y 2012 Acta Phys. Sin. 61 193301 (in Chinese) [刘玉柱, 肖韶荣, 张成义, 郑改革, 陈云云 2012 61 193301]
[16] Eppink A T J B, Parker D H 1999 J. Chem. Phys. 110 832
[17] Walser A M, Meisinger M, Radi P, Gerber T, Knopp G 2009 Phys. Chem. Chem. Phys. 11 8456
[18] Gerber T, Liu Y, Knopp G, Hemberger P, Boedi A, Radi P, Sych Y 2013 Rev. Sci. Instrum. 84 033101
[19] Yang C N 1948 Phys. Rev. 74 764
[20] Seideman T 1999 Phys. Rev. Lett. 83 4971
[21] Reid K L 2003 Annu. Rev. Phys. Chem. 54 397
[22] Suzuki Y I, Horio T, Fuji T, Suzuki T 2011 J. Chem. Phys. 134 184313
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