-
Considering the effect of molecular vibrational levels, inelastic currents through the "metal/single molecule/metal" in the frame of normal vibrational mode are studied. The results show that the Franck-Condon blockage is strongly dependent on the stable energy configuration of molecule in the charge transmission, thus the relation between stationary state and Franck-Condon blockage and the relations of intra molecular vibrational redistribution as well as the relative position of molecule and electrodes to the current-voltage character of the stationary molecule state are further studied theoretically.
[1] Joachim C, Ratne M A 2005 Proc. Natl. Acad. Sci. U.S.A. 102 8800
[2] Ventra M Di, Pantelides S T, Lang N D 2002 Phys. Rev. Lett. 88 046801
[3] Seideman T 2003 J. Phys. D:Condens. Matter 15 R521
[4] Park H, Park J, Lim A K L, Anderson E H, Alivisators A P, McEuen P L 2000 Nature 407 57
[5] Park J , Pasupathy A N, Goldsmith J I, Soldatov A V, Chang C, Yaish Y, Sethna J P, Abrun H D, Ralph D C, McEuen P L 2003 Thin Solid Film 438 457
[6] Qiu X H, Nazin G V, Ho W 2004 Phys. Rev. Lett. 92 20612
[7] Galperin M, Ratner M A, Nitzan A 2005 J. Chem. Phys. 121 11965
[8] Galperin M, Nitzan A 2005 Phys. Rev. Lett. 95 206802
[9] Galperin M, Nitzan A 2006 J. Chem. Phys. 124 234709
[10] Zheng X L, Zheng J M, Ren Z Y, Guo P, Tian J T, Bai J T 2009 Acta Phys. Sin. 58 5709 (in Chinese)[郑新亮、郑继明、任兆玉、郭 平、田进寿、白晋涛 2009 58 5709]
[11] Xia C J, Fang C F, Hu G C, Li D M, Liu D S, Xie S J 2007 Acta Phys. Sin. 56 4884 (in Chinese)[夏蔡娟、房常峰、胡贵超、李东梅、刘德胜、谢士杰 2007 56 4884]
[12] Li Y D, Li H H, Wang C G 2002 Acta Phys. Sin. 51 2349 (in Chinese)[李英德、李红海、王传奎 2002 51 2349]
[13] May V, Kühn O 2006 Chem. Rev. Lett. 420 192
[14] May V, Kühn O 2008 Phys. Rev. B 77 115439
[15] May V, Kühn O 2008 Phys. Rev. B 77 115440
[16] Koch J, Oppen F von 2005 Phys. Rev. Lett. 94 206804
[17] Koch J, Oppen F von, Nitzan A 2006 Phys. Rev. B 73 155306
[18] Welack S, Madddox J B, Esposito M, Harbola U, Mukamel S 2008 Nano Lett. 8 1137
-
[1] Joachim C, Ratne M A 2005 Proc. Natl. Acad. Sci. U.S.A. 102 8800
[2] Ventra M Di, Pantelides S T, Lang N D 2002 Phys. Rev. Lett. 88 046801
[3] Seideman T 2003 J. Phys. D:Condens. Matter 15 R521
[4] Park H, Park J, Lim A K L, Anderson E H, Alivisators A P, McEuen P L 2000 Nature 407 57
[5] Park J , Pasupathy A N, Goldsmith J I, Soldatov A V, Chang C, Yaish Y, Sethna J P, Abrun H D, Ralph D C, McEuen P L 2003 Thin Solid Film 438 457
[6] Qiu X H, Nazin G V, Ho W 2004 Phys. Rev. Lett. 92 20612
[7] Galperin M, Ratner M A, Nitzan A 2005 J. Chem. Phys. 121 11965
[8] Galperin M, Nitzan A 2005 Phys. Rev. Lett. 95 206802
[9] Galperin M, Nitzan A 2006 J. Chem. Phys. 124 234709
[10] Zheng X L, Zheng J M, Ren Z Y, Guo P, Tian J T, Bai J T 2009 Acta Phys. Sin. 58 5709 (in Chinese)[郑新亮、郑继明、任兆玉、郭 平、田进寿、白晋涛 2009 58 5709]
[11] Xia C J, Fang C F, Hu G C, Li D M, Liu D S, Xie S J 2007 Acta Phys. Sin. 56 4884 (in Chinese)[夏蔡娟、房常峰、胡贵超、李东梅、刘德胜、谢士杰 2007 56 4884]
[12] Li Y D, Li H H, Wang C G 2002 Acta Phys. Sin. 51 2349 (in Chinese)[李英德、李红海、王传奎 2002 51 2349]
[13] May V, Kühn O 2006 Chem. Rev. Lett. 420 192
[14] May V, Kühn O 2008 Phys. Rev. B 77 115439
[15] May V, Kühn O 2008 Phys. Rev. B 77 115440
[16] Koch J, Oppen F von 2005 Phys. Rev. Lett. 94 206804
[17] Koch J, Oppen F von, Nitzan A 2006 Phys. Rev. B 73 155306
[18] Welack S, Madddox J B, Esposito M, Harbola U, Mukamel S 2008 Nano Lett. 8 1137
Catalog
Metrics
- Abstract views: 7616
- PDF Downloads: 859
- Cited By: 0
下载:
