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Stimulated Raman scattering is studied in liquid water using pulse laser at a wavelength of 532 nm. At a lower excitation energy, Stokes line and anti-Stokes line 3426 cm-1 can be observed in the forward Raman scattering. When excitation intensity is increased to 140 mJ, the low frequency 313 cm-1 line in the forward Raman scattering can be observed, and the 3389 cm-1 Stokes line and 3268 cm-1 Stokes line in the backward Raman scattering can also be observed. The experimental results demonstrate that the structure of water under the action of the intense excitation energy is similar to that of ice Ⅷ.
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Keywords:
- stimulated Raman scattering /
- light interaction with matter /
- ice Ⅷ
[1] Lee S,Kim J,Lee S J,Kim K S 1997 Phys.Rev.Lett.79 2038
[2] [3] Salzmann C G,Hallbrucker A,Finney J L,Mayer E 2006 Chem.Phys.Lett.429 469
[4] Chang H C,Huang K H,Yeh Y L,Lin S H 2000 Chem.Phys.Lett.326 93
[5] [6] Li F F,Cui Q L,He Z,Cui T,Zhang J,Zhou Q,Zou G T 2005 J.Chem.Phys.123 174511
[7] [8] Dorkenoo K D,Rivoire G 2002 Opt.Comm.202 113
[9] [10] [11] Goncharov A F,Struzhkin V V,Mao H,Hemley R J 1999 Phys.Rev.Lett.83 1998
[12] Kudryavtseva A D,Tcherniega N V 2002 J.Russ.Laser Res.23 288
[13] [14] [15] Yui H,Fujiwara H,Fujinami M,Sawada T 2001 Anal.Sci.17(Suppl.) i77
[16] [17] Ziane O,Zaiba S,Melikechi N 2007 Opt.Comm.273 200
[18] Anderson J D,Schubert G,Jacobson R A,Lau E L,Moore W B,Sjogren W L 1998 Science 280 1573
[19] [20] [21] Yui H,Kanoh K,Fujiwara H,Sawada T 2002 J.Phys.Chem.A 106 12041
[22] Siano S,Pini R,Salimbeni R,Vannini M 1996 Appl.Phys.B 62 503
[23] [24] Teng P,Nishioka N S,Anderson R R,Deutsch T F 1987 IEEE J.Quantum Elect.23 1845
[25] [26] [27] Pruzan Ph,Chervin J C,Wolanin E,Canny B,Gauthier M,Hanfland M 2003 J.Raman Spectrosc.34 591
[28] Yui H,Yoneda Y,Kitamori T,Sawada T 1999 Phys.Rev.Lett.82 4110
[29] [30] Lu X Z,Zhang Y,Zhao P,Fang S J 2011 J.Phys.Chem.B 115 71
[31] -
[1] Lee S,Kim J,Lee S J,Kim K S 1997 Phys.Rev.Lett.79 2038
[2] [3] Salzmann C G,Hallbrucker A,Finney J L,Mayer E 2006 Chem.Phys.Lett.429 469
[4] Chang H C,Huang K H,Yeh Y L,Lin S H 2000 Chem.Phys.Lett.326 93
[5] [6] Li F F,Cui Q L,He Z,Cui T,Zhang J,Zhou Q,Zou G T 2005 J.Chem.Phys.123 174511
[7] [8] Dorkenoo K D,Rivoire G 2002 Opt.Comm.202 113
[9] [10] [11] Goncharov A F,Struzhkin V V,Mao H,Hemley R J 1999 Phys.Rev.Lett.83 1998
[12] Kudryavtseva A D,Tcherniega N V 2002 J.Russ.Laser Res.23 288
[13] [14] [15] Yui H,Fujiwara H,Fujinami M,Sawada T 2001 Anal.Sci.17(Suppl.) i77
[16] [17] Ziane O,Zaiba S,Melikechi N 2007 Opt.Comm.273 200
[18] Anderson J D,Schubert G,Jacobson R A,Lau E L,Moore W B,Sjogren W L 1998 Science 280 1573
[19] [20] [21] Yui H,Kanoh K,Fujiwara H,Sawada T 2002 J.Phys.Chem.A 106 12041
[22] Siano S,Pini R,Salimbeni R,Vannini M 1996 Appl.Phys.B 62 503
[23] [24] Teng P,Nishioka N S,Anderson R R,Deutsch T F 1987 IEEE J.Quantum Elect.23 1845
[25] [26] [27] Pruzan Ph,Chervin J C,Wolanin E,Canny B,Gauthier M,Hanfland M 2003 J.Raman Spectrosc.34 591
[28] Yui H,Yoneda Y,Kitamori T,Sawada T 1999 Phys.Rev.Lett.82 4110
[29] [30] Lu X Z,Zhang Y,Zhao P,Fang S J 2011 J.Phys.Chem.B 115 71
[31]
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