双色圆偏振飞秒脉冲驱动CO分子不对称解离

林康; 宫晓春; 宋其迎; 季琴颖; 马俊杨; 张文斌; 陆培芬; 曾和平; 吴健

doi:10.7498/aps.65.224209

摘要

利用反旋圆偏振双色飞秒激光脉冲，结合电子-离子三维动量符合测量，实验研究了CO分子的单电离和双电离解离过程.在激光偏振平面内观测到碳离子C+三叶草状的不对称动量分布.通过调节双色场中基频光和倍频光的相对相位，可以控制C+的出射方向，实现CO分子的二维不对称解离.

关键词:

We experimentally studied the dissociative single and double ionization of CO molecules by counter-rotating circularly polarized two-color (CRTC) laser fields. By coincidently measuring the electrons and the fragmented ions, trefoil asymmetric momentum distributions of C+ in the polarization plane were observed, which are mainly determined by the selective ionization of CO with asymmetric orbitals. The threefold pattern could rotate continuously in the two-dimensional space by finely tuning the relative phase of the CRTC fields, providing a new method to manipulate the directional bond breaking of molecules by strong laser fields.

Keywords:

作者及机构信息

1.
华东师范大学, 精密光谱科学与技术国家重点实验室, 上海 200062

通信作者: 陆培芬, pflu@lps.ecnu.edu.cn

基金项目: 上海市青年科技英才扬帆计划（批准号：16YF1402900）资助的课题.

Authors and contacts

1.
State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, China

Corresponding author: Lu Pei-Fen, pflu@lps.ecnu.edu.cn

Funds: Project supported by the Shanghai Sailing Program, China (Grant No. 16YF1402900).

参考文献

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[41]	Wu J, Schmidt L Ph H, Kunitski M, Meckel M, Voss S, Sann H, Kim H, Jahnke T, Czasch A, Dörner R 2012Phys. Rev. Lett. 108 183001
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施引文献

[1]	Zewail A H 1988Science 242 1645
[2]	Assion A, Baumert T, Bergt M, Brixner T, Kiefer B, Seyfried V, Strehle M, Gerber G 1998Science 282 919
[3]	Shapiro M, Brumer P 2012Quantum Control of Molecular Processes (New York:Wiley-VCH)
[4]	Kling M F, Siedschlag C, Verhoef A J, Khan J I, Schultze M, Uphues T, Ni Y, Uiberacker M, Drescher M, Krausz F, Vrakking M J J 2006Science 312 246
[5]	Kremer M, Fischer B, Feuerstein B, de Jesus V L B, Sharma V, Hofrichter C, Rudenko A, Thumm U, Schröter C D, Moshammer R, Ullrich J 2009Phys. Rev. Lett. 103 213003
[6]	Fischer B, Kremer M, Pfeifer T, Feuerstein B, Sharma V, Thumm U, Schröter C D, Moshammer R, Ullrich J 2010Phys. Rev. Lett. 105 223001
[7]	McKenna J, Anis F, Sayler A M, Gaire B, Johnson N G, Parke E, Carnes K D, Esry B D, Ben-Itzhak I 2012Phys. Rev. A 85 023405
[8]	Xu H, Xu T Y, He F, Kielpinski D, Sang R T, Litvinyuk I V 2014Phys. Rev. A 89 041403
[9]	Rathje T, Sayler A M, Zeng S, Wustelt P, Figger H, Esry B D, Paulus G G 2013Phys. Rev. Lett. 111 093002
[10]	Kling N G, Betsch K J, Zohrabi M, Zeng S, Anis F, Ablikim U, Jochim B, Wang Z, Kbel M, Kling M F, Carnes K D, Esry B D, Ben-Itzhak I 2013Phys. Rev. Lett. 111 163004
[11]	Charron E, Giusti-Suzor A, Mies F H 1993Phys. Rev. Lett. 71 692
[12]	Ohmura H, Saito N, Tachiya M 2006Phys. Rev. Lett. 96 173001
[13]	Wu J, Vredenborg A, Schmidt L P H, Jahnke T, Czasch A, Dörner R 2013Phys. Rev. A 87 023406
[14]	Sheehy B, Walker B, DiMauro L F 1995Phys. Rev. Lett. 74 4799
[15]	Ray D, He F, De S, Cao W, Mashiko H, Ranitovic P, Singh K P, Znakovskaya I, Thumm U, Paulus G G, Kling M F, Litvinyuk I V, Cocke C L 2009Phys. Rev. Lett. 103 223201
[16]	Betsch K J, Pinkham D W, Jones R R 2010Phys. Rev. Lett. 105 223002
[17]	Kotsina N, Kaziannis S, Danakas S, Kosmidisa C 2013J. Chem. Phys. 139 104313
[18]	Kaziannis S, Kotsina N, Kosmidis C 2014J. Chem. Phys. 141 104319
[19]	Ohmura H, Saito N 2014J. Phys. B 47 204007
[20]	Gong X C, He P L, Song Q Y, Ji Q Y, Pan H F, Ding J X, He F, Zeng H P, Wu J 2014Phys. Rev. Lett. 113 203001
[21]	Song Q Y, Gong X C, Ji Q Y, Lin K, Pan H F, Ding J X, Zeng H P, Wu J 2015J. Phys. B 48 094007
[22]	Lin K, Gong X C, Song Q Y, Ji Q Y, Zhang W B, Ma J Y, Lu P F, Pan H F, Ding J X, Zeng H P, Wu J 2016J. Phys. B 49 025603
[23]	He F, Ruiz C, Becker A 2007Phys. Rev. Lett. 99 083002
[24]	He F, Ruiz C, Becker A 2008J. Phys. B 41 081003
[25]	Singh K P, He F, Ranitovic P, Cao W, De S, Ray D, Chen S, Thumm U, Becker A, Murnane M M, Kapteyn H C, Litvinyuk I V, Cocke C L 2010Phys. Rev. Lett. 104 023001
[26]	Sansone G, Kelkensberg F, Pérez-Torres J F, Morales F, Kling M F, Siu W, Ghafur O, Johnsson P, Swoboda M, Benedetti E, Ferrari F, Lépine F, Sanz-Vicario J L, Zherebtsov S, Znakovskaya I, L'Huillier A, Ivanov M Y, Nisoli M, Martín F, Vrakking M J J 2010Nature 465 763
[27]	Wu J, Magrakvelidze M, Schmidt L P H, Kunitski M, Pfeifer T, Schöffler M, Pitzer M, Richter M, Voss S, Sann H, Kim H, Lower J, Jahnke T, Czasch A, Thumm U, Dörner R 2013Nat. Commun. 4 3177
[28]	Chaloupka J L, Hickstein D D 2016Phys. Rev. Lett. 116 143005
[29]	Mancuso C A, Dorney K M, Hickstein D D, Chaloupka J L, EllisJ L, Dollar F J, Knut R, Grychtol P, Zusin D, Gentry C, Gopalakrishnan M, Kapteyn H C, Murnane M M 2016Phys. Rev. Lett. 117 133201
[30]	Eckart S, Richter M, Kunitski M, Hartung A, Rist J, Henrichs K, Schlott N, Kang H, Bauer T, Sann H, Schmidt L Ph H, Schöffler M, Jahnke T, Dörner R 2016Phys. Rev. Lett. 117 133202
[31]	Bandrauk A D, Lu H Z 2003Phys. Rev. A 68 043408
[32]	Pisanty E, Sukiasyan S, Ivanov M 2014Phys. Rev. A 90 043829
[33]	Yuan K J, Bandrauk A D 2015Phys. Rev. A 92 063401
[34]	Blaga C I, Xu J, DiChiara A D, Sistrunk E, Zhang K, AgostiniP, Miller T A, DiMauro L F, Lin C D 2012Nature 483 194
[35]	Kfir O, Grychtol P, Turgut E, Knut R, Zusin D, Popmintchev D, Popmintchev T, Nembach H, Shaw J M, Fleischer A, Kapteyn H, Murnane M, Cohen O 2015Nat. Photon. 9 99
[36]	Chen C, Wu J, Zeng H P 2010Phys. Rev. A 82 033409
[37]	Mancuso C A, Hickstein D D, Grychtol P, Knut R, Kfir O, Tong X M, Dollar F, Zusin D, Gopalakrishnan M, Gentry C, Turgut E, Ellis J L, Chen M C, Fleischer A, Cohen O, Kapteyn H C, Murnane M M 2015Phys. Rev. A 91 031402
[38]	Baykusheva D, Ahsan M S, Lin N, Wörner H J 2016Phys. Rev. Lett. 116 123001
[39]	Betsch K J, Pinkham D W, Jones R R 2010Phys. Rev. Lett. 105 223002
[40]	Li H, Ray D, De S, Znakovskaya I, Cao W, Laurent G, Wang Z, Kling M F, Le A T, Cocke C L 2011Phys. Rev. A 84 043429
[41]	Wu J, Schmidt L Ph H, Kunitski M, Meckel M, Voss S, Sann H, Kim H, Jahnke T, Czasch A, Dörner R 2012Phys. Rev. Lett. 108 183001
[42]	Wu J, Vredenborg A, Schmidt L P H, Jahnke T, Czasch A, Dörner R 2013Phys. Rev. A 87 023406
[43]	Mashiko H, Gilbertson S, Li C Q, Khan S D, Shakya M M, Moon E, Chang Z 2008Phys. Rev. Lett. 100 103906
[44]	Chini M, Mashiko H, Wang H, Chen S, Yun C, Scott S, Gilbertson S, Chang Z 2009Opt. Express 17 21459
[45]	Dörner R, Mergel V, Jagutzki O, Spielberger L, Ullrich J, Moshammer R, Schmidt-Böcking H 2000Phys. Rep. 330 95
[46]	Ullrich J, Moshammer R, Dorn A, Dörner R, Schmidt L Ph H, Schmidt-Böcking H 2003Rep. Prog. Phys. 66 1463
[47]	Guo C 2006Phys. Rev. A. 73 041401

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