氘含量对DKDP晶体横向受激拉曼散射增益系数的影响

柴向旭; 李富全; 王圣来; 冯斌; 朱启华; 刘宝安; 孙洵; 许心光

doi:10.7498/aps.64.034213

摘要

本文测量了不同氘含量K(H1-xDx)2PO4晶体(DKDP晶体)在Z(XX)Y散射配置下的自发拉曼散射光谱, 并详细分析了氘含量对与横向受激拉曼散射(TSRS)增益系数有关的拉曼频移、半峰宽和散射强度的影响. 然后通过与去离子水拉曼散射对比得出了不同氘含量DKDP晶体的TSRS增益系数. 结果表明随着氘含量的增加DKDP晶体的TSRS增益系数先减小至KDP晶体的40.1%, 后增大至68.9%; 本文认为掺氘后拉曼半峰宽的变化是引起TSRS增益系数随氘含量变化的主要原因.

关键词:

Abstract

In this paper, the spontaneous Raman spectra of K(H1-xDx)2PO4 (DKDP) crystals with different deuteration degrees in the Z(XX)Y scattering geometry are measured. And the Raman spectroscopy parameters including Raman shift, full-width at half maximum, and scattering intensity, which are related to the transverse stimulated Raman scattering (TSRS) gain coefficients, are analyzed in detail. Using the Raman scattering from water as a reference, the TSRS gain coefficients of DKDP crystals with different deuteration degrees are derived. It is found that with increasing deuteration degree in DKDP crystal the TSRS gain coefficient first decreases to about 40.1% of the KDP crystal, then increases to about 68.9%. We regard the change of the full-width at half maximum as the main reason for the dependence of TSRS gain coefficient on the deuteration degree.

Keywords:

作者及机构信息

1.
山东大学晶体材料国家重点实验室, 晶体材料研究所, 济南 250100;

2.
中国工程物理研究院激光聚变研究中心, 绵阳 621900

Authors and contacts

1.
State Key Laboratory of Crystal Materials, Institute of Crystal Materials, Shandong University, Jinan 250100, China;

2.
Research Center of Laser Fusion, China Academy of Engineering Physics, Mianyang 621900, China

参考文献

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[13]	Guo Y J, Tang S X, Hui H C, Wang Y Y, Tang W, Zhu B Q, Lin Z Q 2013 Proc. SPIE 8786 87860U
[14]	Demos S G, Raman R N, Yang S T, Negres R A, Schaffers K I, Henesian M A 2011 Opt. Express 19 21050
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[21]	Liu B A, Zhou H L, Zhang Q H, Xu M X, Ji S H, Zhu L L, Zhang L S, Liu F F, Sun X, Xu X G 2013 Chin. Phys. Lett. 30 067804
[22]	Loiacono G M, Balascio J F, Osborne W 1974 Appl. Phys. Lett. 24 455
[23]	Wang K P, Huang Y 2011 Chin. Phys. B 20 077401
[24]	Ye L W, Li Z D, Su G B, Zhuang X X, Zheng G Z 2007 Opt. Commun. 275 399
[25]	Carollne M P, Adams W A 1979 J. Phys. Chem. 83 814
[26]	Tun Z, Nelmes R J, Kuhs W F, Stanfield R F D 1988 J. Phys. C 21 245
[27]	Anachkova E, Savatinova I 1985 Phys. Stat. Sol. (b) 131 K101
[28]	Li Z 2005 M. S. Thesis (Beijing: Beijing University of Technology) (In Chinese) [李政 2005 硕士学位论文 (北京: 北京工业大学)]
[29]	Chang R K, Lacina B, Pershan P S 1966 Phys. Rev. Lett. 17 755
[30]	Lacina W B, Pershan P S. 1970 Phys. Rev. B 1 1765
[31]	Bischel W K, Black G. 1983 AIP Conf. Proc. 100 181
[32]	Faris G W, Copeland R A 1997 Appl. Opt. 36 2686
[33]	Schiebener P, Straub J, Sengers J M H L, Gallagher J S 1990 J. Phys. Chem. Ref. Data 19 677
[34]	Yakshin M A, Kim D W, Kim Y S, Broslavets Y Y, Sidoryuk O E, Goldstein S 1997 Laser Phys. 7 941
[35]	Huser T, Hollars C W, Siekhaus W J 2004 Appl. Spectrosc. 58 349

施引文献

[1]	Zhang K C, Wang X M 2005 Nonlinear optical crystal material science (Second edition, Beijing: Science Press) pp133-151 (In Chinese) [张克从, 王希敏 2005 非线性光学晶体材料科学 (第二版, 北京: 科学出版社)第133–151页]
[2]	Yang Y S, Zheng W G, Han W, Che Y L, Tan J C, Xiang Y, Jia H T 2007 Acta Phys. Sin. 56 6468 (in Chinese) [杨义胜, 郑万国, 韩伟, 车雅良, 谭吉春, 向勇, 贾怀庭 2007 56 6468]
[3]	Wang J, Zhang X M, Li F Q, Han W, Li K Y, Fen B 2011 Chin. J. Lasers 38 0502011 (in Chinese) [王静, 张小民, 李富全, 韩伟, 李恪宇, 冯斌 2011 中国激光 38 0502011]
[4]	Barker C E, Sacks R A, Van Wonterghem B M, Caird J A, Murray J R, Campbell J H, Kyle K, Ehrlich R B, Nielsen N D 1997 Proc. SPIE 2633 501
[5]	Novikov V N, Belkov S A, Buiko S A, Voronich I N, Efimov D G, Zaretsky A I, Kochemasov G G, Kravchenko A G, Kulikov S M, Lebedev V A, Okutin G P, Rukavishnikov N N, Sukharev S A 1999 Proc. SPIE 3492 1009
[6]	Shur M S 1966 Soviet Phys. Crystallography 11 394
[7]	Chai X X, Zhu Q H, Li F Q, Wang S L, Zhou H L, Xu X G 2014 High Power Laser and Particle Beams 26 022014 (in Chinese) [柴向旭, 朱启华, 李富全, 王圣来, 周海亮, 许心光 2014 强激光与粒子束 26 022014]
[8]	Ji L L, Zhu B Q, Zhan T Y, Dai Y P, Zhu J, Ma W X, Lin Z Q 2011 Acta Phys. Sin. 60 094210 (in Chinese) [季来林, 朱宝强, 詹廷宇, 戴亚平, 朱检, 马伟新, 林尊琪2011 60 094210]
[9]	Wegner P J, Henesian M A, Speck D R, Bibeau C, Ehrlich R B, Laumann C W, Lawson J K, Weiland T L 1992 Appl. Opt. 31 6414
[10]	Han W, Wang F, Zhou L D, Li F Q, Feng B, Cao H B, Zhao J P, Li S, Zheng K X, Wei X F, Gong M L, Zheng W G 2013 Opt Express 21 30481
[11]	Smith W L, Henesian M A, Milanovich F P 1984 1983 Laser Program Annual Report (UCRL-50021-83) (Livermore CA: Lawrence Livermore National Laboratory) 6 61
[12]	Belkov S A, Kochemasov G G, Kulikov S M, Novikov V N, Rukavishnikov N N, Sukharev S A, Voronich I N, Zaretski A I 1997 Proc. SPIE 2633 506
[13]	Guo Y J, Tang S X, Hui H C, Wang Y Y, Tang W, Zhu B Q, Lin Z Q 2013 Proc. SPIE 8786 87860U
[14]	Demos S G, Raman R N, Yang S T, Negres R A, Schaffers K I, Henesian M A 2011 Opt. Express 19 21050
[15]	Demos S G, Raman R N, Yang S T, Negres R A, Schaffers K I, Henesian M A 2011 Proc. SPIE 8190 81900S
[16]	Cheng G X 2001 Principle and application of Raman and Brillouin scattering (Beijing: Science Press) pp 32-83 (In Chinese) [程光熙 2001 拉曼布里渊散射原理及应用 (北京: 科学出版社) 第32–83页]
[17]	Wang Q G, Su L B, Li H J, Xiong W, Yuan H, Zheng L H, Xu X D, Wu F, Tang H L, Jiang D P, Xu J 2012 Chin. Phys. B 21 054217
[18]	Maier M, Kaiser W 1969 Phys. Rev. 177 580
[19]	Loudon R 1964 Advan. Phys. 13 423
[20]	Liu B A, Yin X, Sun X, Xu M X, Ji S H, Xu X G, Zhang J F 2012 J. Appl. Cryst. 45 439
[21]	Liu B A, Zhou H L, Zhang Q H, Xu M X, Ji S H, Zhu L L, Zhang L S, Liu F F, Sun X, Xu X G 2013 Chin. Phys. Lett. 30 067804
[22]	Loiacono G M, Balascio J F, Osborne W 1974 Appl. Phys. Lett. 24 455
[23]	Wang K P, Huang Y 2011 Chin. Phys. B 20 077401
[24]	Ye L W, Li Z D, Su G B, Zhuang X X, Zheng G Z 2007 Opt. Commun. 275 399
[25]	Carollne M P, Adams W A 1979 J. Phys. Chem. 83 814
[26]	Tun Z, Nelmes R J, Kuhs W F, Stanfield R F D 1988 J. Phys. C 21 245
[27]	Anachkova E, Savatinova I 1985 Phys. Stat. Sol. (b) 131 K101
[28]	Li Z 2005 M. S. Thesis (Beijing: Beijing University of Technology) (In Chinese) [李政 2005 硕士学位论文 (北京: 北京工业大学)]
[29]	Chang R K, Lacina B, Pershan P S 1966 Phys. Rev. Lett. 17 755
[30]	Lacina W B, Pershan P S. 1970 Phys. Rev. B 1 1765
[31]	Bischel W K, Black G. 1983 AIP Conf. Proc. 100 181
[32]	Faris G W, Copeland R A 1997 Appl. Opt. 36 2686
[33]	Schiebener P, Straub J, Sengers J M H L, Gallagher J S 1990 J. Phys. Chem. Ref. Data 19 677
[34]	Yakshin M A, Kim D W, Kim Y S, Broslavets Y Y, Sidoryuk O E, Goldstein S 1997 Laser Phys. 7 941
[35]	Huser T, Hollars C W, Siekhaus W J 2004 Appl. Spectrosc. 58 349

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