搜索

x
中国物理学会期刊

红外光激发作用下分子导电纳米结的非弹性电流研究

CSTR: 32037.14.aps.60.047304

Theoretical study of inelastic current in molecularnano-junction excited by infrared field

CSTR: 32037.14.aps.60.047304
PDF
导出引用
  • 将"金属-单分子-金属"模型化为分子导电纳米结,应用扩展主方程方法研究了红外光激发作用下弱耦合分子导电纳米结的非弹性电流的传导过程.分别采用偶极跃迁的指数耦合、平方耦合以及线性耦合模型描述红外光场与分子的相互作用,研究了不同光场作用下非弹性电流与所加电压的关系,并讨论了分子内振动能重新分布效应对电流-电压特性的影响.

     

    Molecular nano-junction is modeled by 'metal/single molecule/metal’ structure. With the generalized master equation method, the inelastic current induced by the sequential charge transmission through the junction is studied under the excitation of infrared fields in the case of weak lead-molecule coupling.The interaction between infrared field and molecule is described with the models of exponential coupling, square coupling, and linear coupling respectively. In the excitation of varieties of infrared fields, the inelastic current-voltage characteristics and the effects of intramolecular vibrational energy redistribution are discussed.

     

    目录

    /

    返回文章
    返回
    Baidu
    map