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中国物理学会期刊

钇镓石榴石中Tb3+到Ce3+的无辐射能量传递特征

CSTR: 32037.14.aps.38.430

TRANSFER CHARACTERISTICS OF NONRADIATIVE ENERGY FROM Tb3+ TO Ce3+ IN YTTRIUM GALLIUM GARNETS

CSTR: 32037.14.aps.38.430
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  • 在Y3Ga5O12石榴石中,室温下采用紫外激光选择激发光谱研究了能量从Tb3+的5D3和5D4能级无辐射传递给Ce3+的2D3/2能级。实验结果符合Frster-IH直接无辐射传递理论。5D3(Tb3+)→2D3/2(Ce3+)能量传递是电偶-偶极子相互作用机理,其平均临界传递距离为R0=16.3?,而5D4(Tb3+)→2D3/2能量传递是起主导作用的电偶-偶极子相互作用,其平均临界传递距离为11.2?。在5D4的传递过程中,电偶-四极子相互作用也应予以考虑。

     

    Selection-excited spectra and fluorescence lifetimes of Tb3+ and Ce3+ ions in yttrium gallium garnets are obtained at room temperature. In Y3Ga5O12:Tb, Ce, Tb3+ (donor) emission spectrum and Ce3+( acceptor) excitation spectrum overlaps considerably. The observed fluorescence lifetimes of Tb3+ 5D3 and 5D4 levels decrease with Ce3+ concentration when the sample of Y3Ga5O12: Tb, Ce are excited by UV laser pulse. The mechanisms for nonradiative energy transfer from 5D3 and 5D4 states of Tb3+ to 2D3/2 state of Ce3+ are found to be electric dipole-dipole interaction. The critical distance, rate and efficiency of energy transfer from Tb3+ to Ce3+ ion are obtained. The average critical transfer distance (R0) for 5D3 and 5D4(Tb3+)→2D3/2(Ce3+) are 16.3 ? and 11.2 ?, respectively. Although the energy transfer from the 5D4 state is dominated by dipole-dipole interaction, the dipole-quadrupole interaction must also be considered.

     

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