Non linear wavelength dependence of electron localization in strong-field dissociation of D2+

Ji Ling-Ling; Tong Ming-Qiang; Wang Yu-Hua

doi:10.7498/aps.63.180301

Abstract

The wavelength dependence of the electron localization in dissociating molecular ion D2+ is investigated via solving the time-dependent Schrödinger equation of the two-state model of the molecular ion. Our results reveal an anomalous dependence of the electron localization on the laser wavelength. Overall, the degree of the electron localization shows a growing trend with the increase of wavelength, but it drops off obviously at some wavelengths. It is found that the localization asymmetries for some vibrational states become opposite in phase when the wavelength is changed, leading to the decline of the electron localization. Further analysis shows that the nuclear and electronic motions that determine the electron localization respond inconsistently to the variation of the wavelength, ultimately resulting in the non-linear dependence of the electron localization on the laser wavelength.

Keywords:

Authors and contacts

1.
Department of Applied Physics, Wuhan University of Science and Technology, Wuhan 430081, China
Funds: Project supported by the National Natural Science Foundation of China (Grant No. 10904120).

References

[1]	Zewail A H 2000 J. Phys. Chem. A 104 5660
[2]	Posthumus J H 2004 Rep. Prog. Phys. 67 623
[3]	Bandrauk A D, Chelkowski S, Nguyen H S 2004 Int. J. Quant. Chem. 100 834
[4]	Liu K L, Zhang Q B, Lan P F, Lu P X 2013 Opt. Express 21 5107
[5]	Lan P F, Lu P X, Cao W, Li Y H, Wang X L 2007 Phys. Rev. A 76 011402
[6]	Corkum P B, Krausz F 2007 Nature Phys. 3 381
[7]	Krausz F, Ivanov M 2009 Rev. Mod. Phys. 81 163
[8]	Lan P F, Lu P X, Cao W, Wang X L, Hong W Y 2007 Opt. Lett. 32 1186
[9]	Goulielmakis E, Schultze M, Hofstetter M, Yakovlev V S, Gagnon J, Uiberacker M, Aquila A L, Gullikson E M, Attwood D T, Kienberger R, Krausz F, Kleineberg U 2008 Science 320 1614
[10]	Cao W, Lu P, Lan P, Wang X, Yang G 2006 Phys. Rev. A 74 063821
[11]	Hong W Y, Lu P F, Cao W, Lan P, Wang X 2007 J. Phys. B 40 2321
[12]	Weber T, Giessen H, Weckenbrock M, Urbasch G, Staudte A, Spielberger L, Jagutzki O, Mergel V, Vollmer M, Dörner R 2000 Nature 405 658
[13]	Zhou Y M, Huang C, Liao Q, Lu P 2012 Phys. Rev. Lett. 109 053004
[14]	Kienberger R, Goulielmakis E, Uiberacker M, Baltuska A, Yakovlev V, Bammer F, Scrinzi A, Westerwalbesloh Th, Kleineberg U, Heinzmann U, Drescher M, Krausz F 2007 Nature 427 817
[15]	Cao W, Lu P, Lan P, Wang X, Li Y 2007 Phys. Rev. A 75 063423
[16]	Lan P F, Lu P X, Li F, Li Y, Yang Z 2008 Opt. Express 16 5868
[17]	Zeng Z N, Li R X, Xie X H, Xu Z Z 2004 Acta Phys. Sin. 53 2316(in Chinese)[曾志男, 李儒新, 谢新华, 徐志展 2004 53 2316]
[18]	Zhang Q B, Hong W Y, Lan P F, Yang Z Y, Lu P X 2008 Acta Phys. Sin. 57 7848(in Chinese)[张庆斌, 洪伟毅, 兰鹏飞, 杨振宇, 陆培祥 2008 57 7848]
[19]	Wang S Y, Hong W Y, Zhang Q B, Li Q G, Lu P X 2010 Chin. Phys. B 19 083203
[20]	Luo L Y, Du H C, Hu B T 2012 Chin. Phys. B 21 033202
[21]	Cavalieri A L, Mller N, Uphues T, Yakovlev V S, Baltuška A, Horvath B, Schmidt B, Blmel L, Holzwarth R, Hendel S, Drescher M, Kleineberg U, Echenique P M, Kienberger R, Krausz F, Heinzmann U 2007 Nature 449 1029
[22]	Zhu X S, Zhang Q B, Hong W Y, Lu P X, Xu Z Z 2011 Opt. Express 19 24198
[23]	Wang J, Liu F, Yue D G, Zhao J, Xu Y, Meng Q T, Liu W K 2012 Chin. Phys. B 21 123301
[24]	Yue D G, Zheng X Y, Liu H, Wang C X, Meng Q T 2009 Chin. Phys. B 18 1479
[25]	Liu K L, Zhang Q B, Lu P X 2012 Phys. Rev. A 86 033410
[26]	Madsen C B, Anis F, Madsen L B, Esry B D 2012 Phys. Rev. Lett. 109 163003
[27]	Kling M F, Siedschlag C, Verhoef A J, Khan J I, Schultze M, Uphues T, Ni Y, Uiberacker M, Drescher M, Krausz F, Vrakking M J 2006 Science 312 246
[28]	He F, Ruiz C, Becker A 2007 Phys. Rev. Lett. 99 083002
[29]	Kremer M, Fischer B, Feuerstein B, de Jesus V L B, Sharma V, Hofrichter C, Rudenko A, Thumm U, SchrŚter C D, Moshammer R, Ullrich J 2009 Phys. Rev. Lett. 103 213003
[30]	Kling N G, Betsch K J, Zohrabi M, Zeng S, Anis F, Ablikim U, Jochim B, Wang Z, Kbel M, Kling M F, Carnes K D, Esry B D, Ben-Itzhak I 2013 Phys. Rev. Lett. 111 163004
[31]	Liu K L, Hong W Y, Lu P F 2011 Opt. Express 19 20279
[32]	Znakovskaya I, von den Hoff P, Zherebtsov S, Wirth A, Herrwerth O, Vrakking M, de Vivie-Riedle R, Kling M 2009 Phys. Rev. Lett. 103 103002
[33]	Lan P F, Lu P X, Cao W, Li Y H, Wang X L 2007 Phys. Rev. A 76 021801
[34]	Takemoto N, Becker A 2010 Phys. Rev. Lett. 105 203004
[35]	Zhang Q B, Lu P X, Lan P F, Hong W Y, Yang Z 2008 Opt. Express 16 9795
[36]	Hong W Y, Lu P X, Lan P F, Zhang Q B, Wang X L 2009 Opt. Express 17 5139
[37]	Hong W Y, Lu P X, Lan P F, Yang Z, Li Y H, Liao Q 2008 Phys. Rev. A 77 033410
[38]	Magrakvelidze M, He F, Niederhausen T, Litvinyuk I V, Thumm U 2009 Phys. Rev. A 79 033410
[39]	Silva F, Austin D R, Thai A, Baudisch M, Hemmer M, Faccio D, Couairon A, Biegert J 2012 Nature Comm. 3 807
[40]	Hong Z F, Zhang Q B, Lu P X 2013 Opt. Express 21 9491
[41]	Lan P F, Lu P X, Li Q, Li F, Hong W Y, Zhang Q 2009 Phys. Rev. A 79 043413
[42]	Tate J, Auguste T, Muller H G, Salières P, Agostini P, DiMauro L F 2007 Phys. Rev. Lett. 98 013901
[43]	Hong W Y, Lu P F, Li Q, Zhang Q B 2009 Opt. Lett. 34 2102
[44]	Liu K L, Hong W Y, Zhang Q B, Lu P X 2011 Opt. Express 19 26359
[45]	Znakovskaya I, von den Hoff P, Marcus G, Zherebtsov S, Bergues B, Gu X, Deng Y, Vrakking M J J, Kienberger R, Krausz F, de Vivie-Riedle R, Kling M F 2012 Phys. Rev. Lett. 108 063002
[46]	Liao Q, Zhou Y M, Huang C, Lu P X 2012 New J. Phys. 14 013001
[47]	Kelkensberg F, Sansone G, Ivanov M Y, Vrakking M 2011 Phys. Chem. Chem. Phys. 13 8647
[48]	Jia Z M, Zeng Z N, Li R X, Xu Z Z, Deng Y P 2014 Phys. Rev. A 89 023419
[49]	Xu T Y, He F 2013 Phys. Rev. A 88 043426

Cited By

[1]	Zewail A H 2000 J. Phys. Chem. A 104 5660
[2]	Posthumus J H 2004 Rep. Prog. Phys. 67 623
[3]	Bandrauk A D, Chelkowski S, Nguyen H S 2004 Int. J. Quant. Chem. 100 834
[4]	Liu K L, Zhang Q B, Lan P F, Lu P X 2013 Opt. Express 21 5107
[5]	Lan P F, Lu P X, Cao W, Li Y H, Wang X L 2007 Phys. Rev. A 76 011402
[6]	Corkum P B, Krausz F 2007 Nature Phys. 3 381
[7]	Krausz F, Ivanov M 2009 Rev. Mod. Phys. 81 163
[8]	Lan P F, Lu P X, Cao W, Wang X L, Hong W Y 2007 Opt. Lett. 32 1186
[9]	Goulielmakis E, Schultze M, Hofstetter M, Yakovlev V S, Gagnon J, Uiberacker M, Aquila A L, Gullikson E M, Attwood D T, Kienberger R, Krausz F, Kleineberg U 2008 Science 320 1614
[10]	Cao W, Lu P, Lan P, Wang X, Yang G 2006 Phys. Rev. A 74 063821
[11]	Hong W Y, Lu P F, Cao W, Lan P, Wang X 2007 J. Phys. B 40 2321
[12]	Weber T, Giessen H, Weckenbrock M, Urbasch G, Staudte A, Spielberger L, Jagutzki O, Mergel V, Vollmer M, Dörner R 2000 Nature 405 658
[13]	Zhou Y M, Huang C, Liao Q, Lu P 2012 Phys. Rev. Lett. 109 053004
[14]	Kienberger R, Goulielmakis E, Uiberacker M, Baltuska A, Yakovlev V, Bammer F, Scrinzi A, Westerwalbesloh Th, Kleineberg U, Heinzmann U, Drescher M, Krausz F 2007 Nature 427 817
[15]	Cao W, Lu P, Lan P, Wang X, Li Y 2007 Phys. Rev. A 75 063423
[16]	Lan P F, Lu P X, Li F, Li Y, Yang Z 2008 Opt. Express 16 5868
[17]	Zeng Z N, Li R X, Xie X H, Xu Z Z 2004 Acta Phys. Sin. 53 2316(in Chinese)[曾志男, 李儒新, 谢新华, 徐志展 2004 53 2316]
[18]	Zhang Q B, Hong W Y, Lan P F, Yang Z Y, Lu P X 2008 Acta Phys. Sin. 57 7848(in Chinese)[张庆斌, 洪伟毅, 兰鹏飞, 杨振宇, 陆培祥 2008 57 7848]
[19]	Wang S Y, Hong W Y, Zhang Q B, Li Q G, Lu P X 2010 Chin. Phys. B 19 083203
[20]	Luo L Y, Du H C, Hu B T 2012 Chin. Phys. B 21 033202
[21]	Cavalieri A L, Mller N, Uphues T, Yakovlev V S, Baltuška A, Horvath B, Schmidt B, Blmel L, Holzwarth R, Hendel S, Drescher M, Kleineberg U, Echenique P M, Kienberger R, Krausz F, Heinzmann U 2007 Nature 449 1029
[22]	Zhu X S, Zhang Q B, Hong W Y, Lu P X, Xu Z Z 2011 Opt. Express 19 24198
[23]	Wang J, Liu F, Yue D G, Zhao J, Xu Y, Meng Q T, Liu W K 2012 Chin. Phys. B 21 123301
[24]	Yue D G, Zheng X Y, Liu H, Wang C X, Meng Q T 2009 Chin. Phys. B 18 1479
[25]	Liu K L, Zhang Q B, Lu P X 2012 Phys. Rev. A 86 033410
[26]	Madsen C B, Anis F, Madsen L B, Esry B D 2012 Phys. Rev. Lett. 109 163003
[27]	Kling M F, Siedschlag C, Verhoef A J, Khan J I, Schultze M, Uphues T, Ni Y, Uiberacker M, Drescher M, Krausz F, Vrakking M J 2006 Science 312 246
[28]	He F, Ruiz C, Becker A 2007 Phys. Rev. Lett. 99 083002
[29]	Kremer M, Fischer B, Feuerstein B, de Jesus V L B, Sharma V, Hofrichter C, Rudenko A, Thumm U, SchrŚter C D, Moshammer R, Ullrich J 2009 Phys. Rev. Lett. 103 213003
[30]	Kling N G, Betsch K J, Zohrabi M, Zeng S, Anis F, Ablikim U, Jochim B, Wang Z, Kbel M, Kling M F, Carnes K D, Esry B D, Ben-Itzhak I 2013 Phys. Rev. Lett. 111 163004
[31]	Liu K L, Hong W Y, Lu P F 2011 Opt. Express 19 20279
[32]	Znakovskaya I, von den Hoff P, Zherebtsov S, Wirth A, Herrwerth O, Vrakking M, de Vivie-Riedle R, Kling M 2009 Phys. Rev. Lett. 103 103002
[33]	Lan P F, Lu P X, Cao W, Li Y H, Wang X L 2007 Phys. Rev. A 76 021801
[34]	Takemoto N, Becker A 2010 Phys. Rev. Lett. 105 203004
[35]	Zhang Q B, Lu P X, Lan P F, Hong W Y, Yang Z 2008 Opt. Express 16 9795
[36]	Hong W Y, Lu P X, Lan P F, Zhang Q B, Wang X L 2009 Opt. Express 17 5139
[37]	Hong W Y, Lu P X, Lan P F, Yang Z, Li Y H, Liao Q 2008 Phys. Rev. A 77 033410
[38]	Magrakvelidze M, He F, Niederhausen T, Litvinyuk I V, Thumm U 2009 Phys. Rev. A 79 033410
[39]	Silva F, Austin D R, Thai A, Baudisch M, Hemmer M, Faccio D, Couairon A, Biegert J 2012 Nature Comm. 3 807
[40]	Hong Z F, Zhang Q B, Lu P X 2013 Opt. Express 21 9491
[41]	Lan P F, Lu P X, Li Q, Li F, Hong W Y, Zhang Q 2009 Phys. Rev. A 79 043413
[42]	Tate J, Auguste T, Muller H G, Salières P, Agostini P, DiMauro L F 2007 Phys. Rev. Lett. 98 013901
[43]	Hong W Y, Lu P F, Li Q, Zhang Q B 2009 Opt. Lett. 34 2102
[44]	Liu K L, Hong W Y, Zhang Q B, Lu P X 2011 Opt. Express 19 26359
[45]	Znakovskaya I, von den Hoff P, Marcus G, Zherebtsov S, Bergues B, Gu X, Deng Y, Vrakking M J J, Kienberger R, Krausz F, de Vivie-Riedle R, Kling M F 2012 Phys. Rev. Lett. 108 063002
[46]	Liao Q, Zhou Y M, Huang C, Lu P X 2012 New J. Phys. 14 013001
[47]	Kelkensberg F, Sansone G, Ivanov M Y, Vrakking M 2011 Phys. Chem. Chem. Phys. 13 8647
[48]	Jia Z M, Zeng Z N, Li R X, Xu Z Z, Deng Y P 2014 Phys. Rev. A 89 023419
[49]	Xu T Y, He F 2013 Phys. Rev. A 88 043426

[1]	Zhang Ying, Wang Xing, Xu Zhong-Feng, Ren Jie-Ru, Zhang Yan-Ning, Zhou Xian-Ming, Liang Chang-Hui, Zhang Xiao-An. Ab initio molecular dynamics study on dissociation process of 2-thiouracil and its tautomers under low-energy electron interactions. Acta Physica Sinica, 2024, 73(2): 023101. doi: 10.7498/aps.73.20231304
[2]	Ning Hui, Wang Kai-Cheng, Wang Shao-Meng, Gong Yu-Bin. Vibrational dynamics of hydrogen molecules under intense THz waves. Acta Physica Sinica, 2021, 70(24): 243101. doi: 10.7498/aps.70.20211482
[3]	Wu Yong-Gang, Liu Jia-Xing, Liu Hong-Ling, Xu Mei, Linghu Rong-Feng. Spectrum and dissociation properties of fluoro trichloro methane molecule in radiational field. Acta Physica Sinica, 2019, 68(6): 063102. doi: 10.7498/aps.68.20182121
[4]	Fu Bao-Qin, Hou Qing, Wang Jun, Qiu Ming-Jie, Cui Jie-Chao. Molecular dynamics study of trapping and detrapping process of hydrogen in tungsten vacancy. Acta Physica Sinica, 2019, 68(24): 240201. doi: 10.7498/aps.68.20190701
[5]	Yao Hong-Bin, Jiang Xiang-Zhan, Cao Chang-Hong, Li Wen-Liang. Theoretical study of dissociation dynamics of HD⁺ and its quantum control with an intense laser field. Acta Physica Sinica, 2019, 68(17): 178201. doi: 10.7498/aps.68.20190400
[6]	Wang Xiao-Li, Yao Guan-Xin, Yang Xin-Yan, Qin Zheng-Bo, Zheng Xian-Feng, Cui Zhi-Feng. Experimental investigation on ultraviolet multiphoton dissociation dynamics of methylamine. Acta Physica Sinica, 2018, 67(24): 243301. doi: 10.7498/aps.67.20181731
[7]	Qin Chao-Chao, Huang Yan, Peng Yu-Feng. Photodissociation dynamics of Br2 in wavelength range of 360-610 nm. Acta Physica Sinica, 2017, 66(19): 193301. doi: 10.7498/aps.66.193301
[8]	Wu Hong-Lin, Song Yun-Fei, Wang Yang, Yu Guo-Yang, Yang Yan-Qiang. Photodissociation dynamics of organic molecules in condensed phase by femtosecond transient grating spectroscopy. Acta Physica Sinica, 2017, 66(3): 033301. doi: 10.7498/aps.66.033301
[9]	Liu Yu-Zhu, Xiao Shao-Rong, Wang Jun-Feng, He Zhong-Fu, Qiu Xue-Jun, Gregor Knopp. Multi-photon dissociation dynamics of Freon 1110 induced by femtosecond laser pulse. Acta Physica Sinica, 2016, 65(11): 113301. doi: 10.7498/aps.65.113301
[10]	Liu Yu-Zhu, Chen Yun-Yun, Zheng Gai-Ge, Jin Feng, Gregor Knopp. Multiphoton ionization and dissociation dynamics of Freon-113 induced by femtosecond laser pulse. Acta Physica Sinica, 2016, 65(5): 053302. doi: 10.7498/aps.65.053302
[11]	Liu Yu-Zhu, Deng Xu-Lan, Li Shuai, Guan Yue, Li Jing, Long Jin-You, Zhang Bing. Multi-photon dissociation dynamics of Freon 114B2 under UV radiation by femtosecond laser pulse. Acta Physica Sinica, 2016, 65(19): 193301. doi: 10.7498/aps.65.193301
[12]	Liu Can-Dong, Jia Zheng-Mao, Zheng Ying-Hui, Ge Xiao-Chun, Zeng Zhi-Nan, Li Ru-Xin. Research progress of the control and measurement of the atomic and molecular ultrafast electron dynamics using two-color field. Acta Physica Sinica, 2016, 65(22): 223206. doi: 10.7498/aps.65.223206
[13]	Shen Zhuang-Zhi. Dynamical behaviors of cavitation bubble under acoustic standing wave field. Acta Physica Sinica, 2015, 64(12): 124702. doi: 10.7498/aps.64.124702
[14]	He Man-Li, Wang Xiao, Gao Si-Feng. Cross sections for the electron impact non-dissociative ion of hydrogen and its isotopic molecule. Acta Physica Sinica, 2012, 61(4): 043404. doi: 10.7498/aps.61.043404
[15]	J. Ullrich, A. Dorn, Ma Xin-Wen, Xu Shen-Yue, Ren Xue-Guang, T. Pflüger. Dissociative ionization of methane by 54 eV electron impact. Acta Physica Sinica, 2011, 60(9): 093401. doi: 10.7498/aps.60.093401
[16]	Tang Xiao-Feng, Niu Ming-Li, Zhou Xiao-Guo, Liu Shi-Lin. Spectroscopic studies of molecular ions and their dissociation dynamics by the threshold photoelectron-photoion coincidence. Acta Physica Sinica, 2010, 59(10): 6940-6947. doi: 10.7498/aps.59.6940
[17]	Chi Yu-Hua, Liu Xue-Shen, Ding Pei-Zhu. The classical dissociation of HF molecule by chirped laser pulse. Acta Physica Sinica, 2006, 55(12): 6320-6325. doi: 10.7498/aps.55.6320
[18]	Xu Hai-Feng, Liu Shi-Lin, Ma Xing-Xiao, Dai Dong-Xu, Xie Jin-Chun, Sha Guo-He. . Acta Physica Sinica, 2002, 51(2): 240-246. doi: 10.7498/aps.51.240
[19]	KONG QING, ZHU LI-JUN, WANG JIA-XIANG, HUO YU-KUN. ELECTRON DYNAMICS IN THE EXTRA-INTENSE STATIONARY LASER FIELD. Acta Physica Sinica, 1999, 48(4): 650-660. doi: 10.7498/aps.48.650
[20]	DING SHI-LIANG, MA JIE, GUAN DA-REN. A DIATOMIC MOLECULE MULTIPHOTON DISSOCIATION IN INTENSE FIELDS. Acta Physica Sinica, 1996, 45(10): 1629-1635. doi: 10.7498/aps.45.1629

Catalog

Vol. 63, Issue 18 - 2014-09-20

Metrics

Abstract views: 5118
PDF Downloads: 371
Cited By: 0

姓名
邮箱
手机号码
标题
留言内容
验证码

Search

Article

留言板