外场作用下BaF分子发射光子累积量及等待时间分布的研究

古丽姗; 彭勇刚

doi:10.7498/aps.65.094202

摘要

利用产生函数方法对BaF分子在激光场与射频场作用下发射光子的累积量及等待时间分布进行了研究. 累积量1 和2 表明在固有偶极和射频场的作用下, 系统表现出外场辅助吸收的现象, 即当1=nrf时, 系统存在吸收峰. 二阶、三阶等待时间分布呈现出明显的振荡现象.

关键词:

In this paper, we consider a single BaF molecule driven by an external field. When the symmetry is broken, the states of the BaF molecule demonstrate the permanent dipole moments. An external laser field to excite BaF molecule transition from its ground state to its excited state, and a radio frequency field couple with the permanent dipole moment of the BaF. The first order and second order cumulants of the emission photons and the waiting time distribution are studied via the recently developed generating function approach, which is very convenient to study the counting statistics and the corresponding probability distributions. The results demonstrate that the radio frequency field could help the BaF molecule to absorb photons from the driving field. The second and third order waiting time distributions oscillate with the evolution time, which reflects the states oscillating with the external radio frequency field.

Keywords:

作者及机构信息

古丽姗¹,
彭勇刚²

1.
昌吉学院物理系, 昌吉 831100;

2.
山东大学物理学院, 济南 250100

通信作者: 古丽姗, shanshan7900@163.com

基金项目: 新疆维吾尔自治区高校科研计划科学研究重点项目(批准号: XJEDU2011I53)、国家自然科学基金(批准号: 11404189)、山东省自然科学基金(批准号: ZR2013AQ020)和教育部博士点基金(批准号: 20130131120006)资助的课题.

Authors and contacts

Gu Li-Shan¹,
Peng Yong-Gang²

1.
Department of Physics, Changji University, Changji 831100, China;

2.
School of Physics, Shandong University, Jinan 250100, China

Corresponding author: Gu Li-Shan, shanshan7900@163.com

Funds: Project supported by the Scientific Research Program of the Higher Education Institution of Xinjiang, China (Grant No. XJEDU2011I53), the National Natural Science Foundation of China (Grant No. 1404189), the Natural Science Foundation of Shandong Province, China (Grant No. ZR2013AQ020), and the Doctoral Program of Higher Education of China (Grant No. 20130131120006).

参考文献

[1]	Moerner W E, Kador L 1989 Phys. Rev. Lett. 62 2535
[2]	Orrit M, Bernard J 1990 Phys. Rev. Lett. 65 2716
[3]	Moerner W E, Orrit M 1999 Science 283 1670
[4]	Plakhotnik T, Donley E A, Wild U P 1997 Annu. Rev. Phys. Chem. 48 181
[5]	Barkai E, Jung Y, Silbey R 2004 Annu. Rev. Phys. Chem. 55 457
[6]	Basche T, Moerner W E, Orrit M, Wild U P 1996 Single Molecule Optical Detection, Imaging and Spectroscopy (New York: VCH)
[7]	Lu H P, Xun L, Xie X S 1998 Science 282 1887
[8]	Xie X S 2002 J. Chem. Phys. 117 11024
[9]	Weiss S 1999 Science 283 1676
[10]	Jung Y, Barikai E, Silbey R J 2002 J. Chem. Phys. 117 10980
[11]	Bohmer M, Enderlein J 2003 Chem. Phys. Chem. 4 792
[12]	Lippitz M, Kulzer F, Orrit M 2005 Chem. Phys. Chem. 6 770
[13]	Barkai E, Brown F L H, Orrit M, Yang H 2008 Theory and Evaluation of Single Molecule Signals (Singapore: World Scientific Press)
[14]	Wang K, Cui L, Zhang X T, Li X Y 2013 Acta Phys. Sin. 62 164205 (in Chinese) [王堃, 崔亮, 张秀婷, 李小英 2013 62 164205]
[15]	Han W, Zhou L D, Li F Q, Wang F, Feng B, Zheng K X, Gong M L 2014 Acta Phys. Sin. 63 074204 (in Chinese) [韩伟, 周丽丹, 李富全, 王芳, 冯斌, 郑奎兴, 巩马理 2014 63 074204]
[16]	Li W F, Du J J, Wen R J, Yang P F, Li G, Zhang T C 2014 Acta Phys. Sin. 63 244205 (in Chinese) [李文芳, 杜金锦, 文瑞娟, 杨鹏飞, 李刚, 张天才 2014 63 244205]
[17]	Brown F L H 2003 Phys. Rev. Lett. 90 028302
[18]	Zheng Y J, Brown F L H 2003 Phys. Rev. Lett. 90 238305
[19]	Zheng Y J, Brown F L H 2003 J. Chem. Phys. 119 11814
[20]	Peng Y G, Xie S J, Zheng Y J, Brown F L H 2009 J. Chem. Phys. 131 214107
[21]	Peng Y G, Zheng Y J, Brown F L H 2007 J. Chem. Phys. 126 104303
[22]	Zheng Y J 2008 J. Chem. Phys. 129 246102
[23]	Han B P, Zheng Y J 2008 Phys. Rev. A 78 015402
[24]	Zheng Y J, Brown F L H 2013 J. Chem. Phys. 139 164120
[25]	Peng Y G, Zheng Y J 2013 Phys. Rev. A 88 013425
[26]	Peng Y G, Zheng Y J 2014 Eur. Phys. J. D 68 290
[27]	Steimle T C, Frey S, Le A 2011 Phys. Rev. A 84 012508
[28]	Titov A T, Mosyagin N S, Petrov A N, Isaev T A, Demile D 2006 Prog. Theor. Chem. Phys. 15 253
[29]	Berg L E, Gador N, Husain D, Ludwigs H, Royen P 1998 Chem. Phys. Lett. 287 89
[30]	Lemeshko M, Krems R V, Doyle J M, Kais S 2013 Mol. Phys. 111 1648
[31]	Han B P, Zheng Y J 2008 Phys. Rev. A 78 015402
[32]	Han B P, Zheng Y J 2009 J. Chem. Phys. 130 244502
[33]	Rozhkov I, Barkai E 2005 Phys. Rev. A 71 033810
[34]	Makarov D E, Metiu H 2001 J. Chem. Phys. 115 5989
[35]	van Kampen N G 2009 Stochastic Processes in Physics and Chemistry (Singapore: Elsevier)
[36]	Prohorov Y V, Rozanov Y A 1969 Probability Theory (Berlin: Springer)
[37]	Amoldus H F, Nienhuis G 1986 Opt. Acta 33 691

施引文献

[1]	Moerner W E, Kador L 1989 Phys. Rev. Lett. 62 2535
[2]	Orrit M, Bernard J 1990 Phys. Rev. Lett. 65 2716
[3]	Moerner W E, Orrit M 1999 Science 283 1670
[4]	Plakhotnik T, Donley E A, Wild U P 1997 Annu. Rev. Phys. Chem. 48 181
[5]	Barkai E, Jung Y, Silbey R 2004 Annu. Rev. Phys. Chem. 55 457
[6]	Basche T, Moerner W E, Orrit M, Wild U P 1996 Single Molecule Optical Detection, Imaging and Spectroscopy (New York: VCH)
[7]	Lu H P, Xun L, Xie X S 1998 Science 282 1887
[8]	Xie X S 2002 J. Chem. Phys. 117 11024
[9]	Weiss S 1999 Science 283 1676
[10]	Jung Y, Barikai E, Silbey R J 2002 J. Chem. Phys. 117 10980
[11]	Bohmer M, Enderlein J 2003 Chem. Phys. Chem. 4 792
[12]	Lippitz M, Kulzer F, Orrit M 2005 Chem. Phys. Chem. 6 770
[13]	Barkai E, Brown F L H, Orrit M, Yang H 2008 Theory and Evaluation of Single Molecule Signals (Singapore: World Scientific Press)
[14]	Wang K, Cui L, Zhang X T, Li X Y 2013 Acta Phys. Sin. 62 164205 (in Chinese) [王堃, 崔亮, 张秀婷, 李小英 2013 62 164205]
[15]	Han W, Zhou L D, Li F Q, Wang F, Feng B, Zheng K X, Gong M L 2014 Acta Phys. Sin. 63 074204 (in Chinese) [韩伟, 周丽丹, 李富全, 王芳, 冯斌, 郑奎兴, 巩马理 2014 63 074204]
[16]	Li W F, Du J J, Wen R J, Yang P F, Li G, Zhang T C 2014 Acta Phys. Sin. 63 244205 (in Chinese) [李文芳, 杜金锦, 文瑞娟, 杨鹏飞, 李刚, 张天才 2014 63 244205]
[17]	Brown F L H 2003 Phys. Rev. Lett. 90 028302
[18]	Zheng Y J, Brown F L H 2003 Phys. Rev. Lett. 90 238305
[19]	Zheng Y J, Brown F L H 2003 J. Chem. Phys. 119 11814
[20]	Peng Y G, Xie S J, Zheng Y J, Brown F L H 2009 J. Chem. Phys. 131 214107
[21]	Peng Y G, Zheng Y J, Brown F L H 2007 J. Chem. Phys. 126 104303
[22]	Zheng Y J 2008 J. Chem. Phys. 129 246102
[23]	Han B P, Zheng Y J 2008 Phys. Rev. A 78 015402
[24]	Zheng Y J, Brown F L H 2013 J. Chem. Phys. 139 164120
[25]	Peng Y G, Zheng Y J 2013 Phys. Rev. A 88 013425
[26]	Peng Y G, Zheng Y J 2014 Eur. Phys. J. D 68 290
[27]	Steimle T C, Frey S, Le A 2011 Phys. Rev. A 84 012508
[28]	Titov A T, Mosyagin N S, Petrov A N, Isaev T A, Demile D 2006 Prog. Theor. Chem. Phys. 15 253
[29]	Berg L E, Gador N, Husain D, Ludwigs H, Royen P 1998 Chem. Phys. Lett. 287 89
[30]	Lemeshko M, Krems R V, Doyle J M, Kais S 2013 Mol. Phys. 111 1648
[31]	Han B P, Zheng Y J 2008 Phys. Rev. A 78 015402
[32]	Han B P, Zheng Y J 2009 J. Chem. Phys. 130 244502
[33]	Rozhkov I, Barkai E 2005 Phys. Rev. A 71 033810
[34]	Makarov D E, Metiu H 2001 J. Chem. Phys. 115 5989
[35]	van Kampen N G 2009 Stochastic Processes in Physics and Chemistry (Singapore: Elsevier)
[36]	Prohorov Y V, Rozanov Y A 1969 Probability Theory (Berlin: Springer)
[37]	Amoldus H F, Nienhuis G 1986 Opt. Acta 33 691

[1]	张慧洁, 贺衎. 哈密顿量宇称-时间对称性的刻画. , 2024, 73(4): 040302. doi: 10.7498/aps.73.20230458
[2]	朱文华, 汪书潮, 王凯迪, 陈松懋, 马彩文, 苏秀琴. 光子计数成像系统的自适应累积时间扫描方法. , 2022, 71(15): 158702. doi: 10.7498/aps.71.20220173
[3]	吴亚珍, 孙中奎. Noise recycling作用下非对称双稳系统的驻留时间分布函数研究. , 2020, (): . doi: 10.7498/aps.69.20191752
[4]	吴亚珍, 孙中奎. 循环噪声驱动下非对称双稳系统的驻留时间分布函数研究. , 2020, 69(12): 120501. doi: 10.7498/aps.69.20201752
[5]	王雪花, 陈丹妮, 于斌, 牛憨笨. 基于累积量标准差的超分辨光学涨落成像解卷积优化. , 2016, 65(19): 198701. doi: 10.7498/aps.65.198701
[6]	左冬冬, 侯威, 王文祥. 中国西南地区干旱Copula函数模型对样本量的敏感性分析. , 2015, 64(10): 100203. doi: 10.7498/aps.64.100203
[7]	闫振纲, 林颖璐, 杨娟, 李振华, 卞保民. 光电探测器随机噪声特征量统计分布函数. , 2012, 61(20): 200502. doi: 10.7498/aps.61.200502
[8]	林颖璐, 闫振纲, 杨娟, 王春勇, 卞保民. 噪声信号特征量分布函数相似特性的研究. , 2012, 61(10): 100505. doi: 10.7498/aps.61.100505
[9]	古丽姗, 王东升, 彭勇刚, 郑雨军. 单量子点在双脉冲激发下偏振光子发射的统计特性. , 2011, 60(8): 084207. doi: 10.7498/aps.60.084207
[10]	彭勇刚, 张西忠, 张兆玉, 郑雨军. 单量子点在连续外场激发下发射光子性质的理论研究. , 2010, 59(3): 1791-1796. doi: 10.7498/aps.59.1791
[11]	郑雨军, 张兆玉, 张西忠. 单分子体系动力学的高阶累积量相似性. , 2009, 58(12): 8194-8198. doi: 10.7498/aps.58.8194
[12]	谢振华, 许录平, 倪广仁. 基于双谱的脉冲星累积脉冲轮廓时间延迟测量. , 2008, 57(10): 6683-6688. doi: 10.7498/aps.57.6683
[13]	叶晨光, 张靖. 利用PPKTP晶体产生真空压缩态及其Wigner准概率分布函数的量子重构. , 2008, 57(11): 6962-6967. doi: 10.7498/aps.57.6962
[14]	谢勇, 徐健学, 杨红军, 胡三觉. 皮层脑电时间序列的相空间重构及非线性特征量的提取. , 2002, 51(2): 205-214. doi: 10.7498/aps.51.205
[15]	. 二分量胶体悬浮系统的短时间动力学. , 2001, 50(9): 1810-1817. doi: 10.7498/aps.50.1810
[16]	包爱东, 朱建阳, 赵峥. 动态Rindler时空中Dirac旋量粒子的四分量波函数及Hawbing-Unruh热效应. , 1993, 42(10): 1550-1555. doi: 10.7498/aps.42.1550
[17]	祝可嘉, 秦晓岿, 陈鸿, 吴翔. 聚丁二烯中的等待时间效应. , 1993, 42(10): 1612-1616. doi: 10.7498/aps.42.1612
[18]	邓辉舫. 等待时间分布函数ψ(t)的渐近行为与连续时间无规行走问题的渐近解. , 1986, 35(11): 1436-1446. doi: 10.7498/aps.35.1436
[19]	侯伯宇. 局部坐标系中的旋量球函数及算子. , 1963, 19(6): 341-359. doi: 10.7498/aps.19.341
[20]	杨立铭. 原子核内核子轨道角動量分布与核子密度. , 1953, 9(4): 302-316. doi: 10.7498/aps.9.302

计量

文章访问数: 6153
PDF下载量: 121
被引次数: 0

姓名
邮箱
手机号码
标题
留言内容
验证码

搜索

留言板