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Three-photon absorption coefficient obtained by current nonlinear transmittance method has large fitting error because of uneven laser radiation distribution. Relatively small three-photon absorption cross section values of present nonlinear molecules restrict their practical applications. In this paper, an accurate three-photon absorption coefficient fitting method is presented, which is applicable for a variety of laser distributions. A fluorene-based derivative, 2, 7-bis(4-methoxyphenylacetylene)-9-thoine-fluorene, is synthesized. Apparent three-photon-absorption-induced optical stabilization effect is shown.
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Keywords:
- three-photon absorption /
- optical stabilization /
- absorption cross-section /
- upconversion fluorescence
[1] Göppert-Mayer M 1931 Ann. Phys. 9 273
[2] Min G 1996 Opt. Lett. 21 988
[3] Maiti S, Shear J B, Wolliams R M, Zipfel W R, Webb W W 1997 Science 275 530
[4] Leeder J M, Andrews D L 2011 J. Chem. Phys. 134 094503
[5] Belfield K D, Bondar M V, Hernández F E, Przhonska O V, Wang X, Yao S 2011 Phys. Chem. Chem. Phys. 13 4303
[6] Cohanoschi I, Echeverría L, Hernández F E 2006 Chem. Phys. Lett. 419 33
[7] He G S, Bhawalkar J D, Prasad P N, Reinhardt B A 1995 Opt. Lett. 20 1524
[8] Morel Y, Irimia A, Najechalski P, Kervella Y, Stephan O, Baldeck P L, Andraud C 2001 J. Chem. Phys. 114 5391
[9] Bhawalkar J D, Kumar N D, Zhao C F, Prasad P N 1997 J. Clin. Laser Med. Surg. 15 201
[10] He G S, Markowicz P P, Lin T, Prasad P N 2002 Nature 415 767
[11] Feng X J, Wu P L, Li K F, Wong M S, Cheah K W 2011 Chem. A Eur. J. 17 2518
[12] Belfield K D, Bondar M V, Yanez C O, Hernandez F E, Przhonska O V 2009 J. Mater. Chem. 19 7498
[13] Parthenopoulos D A, Rentzepis P M 1990 J. Appl. Phys. 68 5814
[14] Parthenopoulos D A, Rentzepis P M 1989 Science 245 843
[15] Dvornikov A S, Rentzepis P M 1995 Opt. Commun. 119 341
[16] Belfield K D, Schafer K J, Liu Y, Liu J, Ren X, Vanstryland E W 2000 J. Phys. Org. Chem. 13 837
[17] Cumpston B H, Ananthavel S P, Barlow S, Dyer D L, Ehrlich J E, Erskine L L, Heikal A A, Kuebler S M, Lee Sandy I Y, McCord-Maughon D, Qin J, Rochel H, Rumi M, Wu X L, Marder S R, Perry J W 1999 Nature 398 51
[18] Albota M A, Xu C, Webb W W 1998 Appl. Opt. 37 7352
[19] Florencio E H, Kevin D B, Ion C 2004 Chem. Phys. Lett. 391 22
[20] Liu J H, Li G F, Wang Y X 2012 J. Phys. Chem. A 116 7445
[21] Bhawalkar J D, He G S, Prasad P N 1996 Rep. Prog. Phys. 59 1041
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[1] Göppert-Mayer M 1931 Ann. Phys. 9 273
[2] Min G 1996 Opt. Lett. 21 988
[3] Maiti S, Shear J B, Wolliams R M, Zipfel W R, Webb W W 1997 Science 275 530
[4] Leeder J M, Andrews D L 2011 J. Chem. Phys. 134 094503
[5] Belfield K D, Bondar M V, Hernández F E, Przhonska O V, Wang X, Yao S 2011 Phys. Chem. Chem. Phys. 13 4303
[6] Cohanoschi I, Echeverría L, Hernández F E 2006 Chem. Phys. Lett. 419 33
[7] He G S, Bhawalkar J D, Prasad P N, Reinhardt B A 1995 Opt. Lett. 20 1524
[8] Morel Y, Irimia A, Najechalski P, Kervella Y, Stephan O, Baldeck P L, Andraud C 2001 J. Chem. Phys. 114 5391
[9] Bhawalkar J D, Kumar N D, Zhao C F, Prasad P N 1997 J. Clin. Laser Med. Surg. 15 201
[10] He G S, Markowicz P P, Lin T, Prasad P N 2002 Nature 415 767
[11] Feng X J, Wu P L, Li K F, Wong M S, Cheah K W 2011 Chem. A Eur. J. 17 2518
[12] Belfield K D, Bondar M V, Yanez C O, Hernandez F E, Przhonska O V 2009 J. Mater. Chem. 19 7498
[13] Parthenopoulos D A, Rentzepis P M 1990 J. Appl. Phys. 68 5814
[14] Parthenopoulos D A, Rentzepis P M 1989 Science 245 843
[15] Dvornikov A S, Rentzepis P M 1995 Opt. Commun. 119 341
[16] Belfield K D, Schafer K J, Liu Y, Liu J, Ren X, Vanstryland E W 2000 J. Phys. Org. Chem. 13 837
[17] Cumpston B H, Ananthavel S P, Barlow S, Dyer D L, Ehrlich J E, Erskine L L, Heikal A A, Kuebler S M, Lee Sandy I Y, McCord-Maughon D, Qin J, Rochel H, Rumi M, Wu X L, Marder S R, Perry J W 1999 Nature 398 51
[18] Albota M A, Xu C, Webb W W 1998 Appl. Opt. 37 7352
[19] Florencio E H, Kevin D B, Ion C 2004 Chem. Phys. Lett. 391 22
[20] Liu J H, Li G F, Wang Y X 2012 J. Phys. Chem. A 116 7445
[21] Bhawalkar J D, He G S, Prasad P N 1996 Rep. Prog. Phys. 59 1041
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