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采用提拉法成功生长尺寸为30 mm 75 mm的15at.%Yb3+:Gd2SiO5单晶, 并用Reitveld全谱拟合方法确定了其晶格常数、原子坐标和温度因子等参数. 用吸收光谱计算了Yb3+离子2F7/2 2F5/2能级跃迁的振子强度、谱线强度、跃迁概率、能级寿命和积分发射截面等光谱参数, 并根据激光性能评估得出结论: 表明该晶体具有较大的阈值特性, 有望采用大功率激光二极管泵浦实现可调谐或超快激光输出.
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关键词:
- Yb3+ :Gd2SiO5晶体生长 /
- 晶体结构 /
- 吸收光谱 /
- 发射光谱
15at.%Yb3+:Gd2SiO5 crystal with a size of30 mm75 mm is grown by the Czochralski method, and its lattice parameters, atom coordinates and temperature factors are determined by the full-profile Rietveld refinement method. Its spectral parameters of oscillator strength, line strength, transition probability, energy lifetime and integral emission cross-section for Yb3+2F7/22F5/2 transition are calculated using the absorption spectraum. And the laser performance evaluation shows that this crystal is a potential laser crystal with relatively high threshold, and could be used as a medium of tunable or ultra-fast laser pumped by high-power laser diode.-
Keywords:
- crystal growth of Yb3+:Gd2SiO5 /
- crystal structure /
- absorption spectra /
- emission spectra
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[2] [3] Georges B 2008 Journal of Alloys and Compounds 451 1
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[8] Xue Y H, Wang Q Y, Chai Lu, Liu Q W, Zhao G J, Su L B, Xu X D, Xu J 2006 Acta Phys. Sin. 55 456 (in Chinese) [薛迎红, 王清月, 柴路, 刘庆文, 赵广军, 苏良碧, 徐晓东, 徐军 2006 55 456]
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[17] [18] Hao Q, Li W X, Wu E, Zeng H P 2009 IEEE J. Quantum Elect. 45 86
[19] [20] Li W X, Hao Q, Zhai H, Zeng H P, Lu W, Zhao G J, Zheng L H, Su L B, Xu J 2007 Opt. Express 15 2354
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[24] Larson A C, Von Dreele R B 2004 Los Alamos National Laboratory Report No. LAUR 86
[25] [26] [27] Zhang Q L, Xiao J Z, Sun D L, Wang A H, Yin S T 2004 Spectrosc. Spect. Anal. 24 1157 (in Chinese) [张庆礼, 肖敬忠, 孙敦陆, 王爱华, 殷绍唐 2004 光谱学与光谱分析 24 1157]
[28] [29] Zhang Q L, Zhou W L, Liu W P, Ding L H, Luo J Q, Yin S T, Jiang H H 2010 Acta Opt. Sin. 30 849 (in Chinese) [张庆礼, 周文龙, 刘文鹏, 丁丽华, 罗建乔, 殷绍堂, 江海河 2010 光学学报 30 849]
[30] [31] Zang J C, Li X, Shan B R, Liu Y H, Liu Y L 2006 Chin. J. Lasers 33 565 (in Chinese) [臧竞存, 李晓, 单秉锐, 刘燕行, 刘玉龙 2006 中国激光 33 565]
[32] [33] Deloach L D, Stephen A. Payne, Larry K. Smith, Wayne L. Kway, William F. Krupke 1994 J. Opt. Soc. Am. B 11 269
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[1] Krupke W F 2000 IEEE J. Sel. Top. Quantum Electron 6 1287
[2] [3] Georges B 2008 Journal of Alloys and Compounds 451 1
[4] [5] Siebold M, Bock S, Schramm U, Xu B, Doualan J L, Camy P, Moncorg R 2009 Appl. Phys B 97 327
[6] [7] Yan C F, Zhao G J, Su L B, Xu X D, Zhang L H, Jun X 2006 J. Phys.: Condens. Matter 18 1325
[8] Xue Y H, Wang Q Y, Chai Lu, Liu Q W, Zhao G J, Su L B, Xu X D, Xu J 2006 Acta Phys. Sin. 55 456 (in Chinese) [薛迎红, 王清月, 柴路, 刘庆文, 赵广军, 苏良碧, 徐晓东, 徐军 2006 55 456]
[9] [10] Li W X, Hao Q, Zhai H, Zeng H P, Lu W, Zhao G J, Yan C F, Su L B, Xu J 2006 Appl. Phys. Lett. 89 101125
[11] [12] [13] Li W X, Pan H F, Ding L E, Zeng H P, Lu W, Zhao G J, Yan C F, Su L B, Xu J 2006 Appl. Phys. Lett. 88 221117
[14] Hao Q, Li W X, Zeng H P 2007 Opt. Express 15 16754
[15] [16] Xue Y H, Wang C Y, Liu Q W, Li Y F, Chai Lu, Yan C F, Zhao G J, Su L B, Xu X D, Xu J 2006 IEEE J. Quantum Elect. 42 517
[17] [18] Hao Q, Li W X, Wu E, Zeng H P 2009 IEEE J. Quantum Elect. 45 86
[19] [20] Li W X, Hao Q, Zhai H, Zeng H P, Lu W, Zhao G J, Zheng L H, Su L B, Xu J 2007 Opt. Express 15 2354
[21] [22] [23] Smolin Y I, Tkachev S P 1969 Kristallogr. 14 14; ICSD No.27728
[24] Larson A C, Von Dreele R B 2004 Los Alamos National Laboratory Report No. LAUR 86
[25] [26] [27] Zhang Q L, Xiao J Z, Sun D L, Wang A H, Yin S T 2004 Spectrosc. Spect. Anal. 24 1157 (in Chinese) [张庆礼, 肖敬忠, 孙敦陆, 王爱华, 殷绍唐 2004 光谱学与光谱分析 24 1157]
[28] [29] Zhang Q L, Zhou W L, Liu W P, Ding L H, Luo J Q, Yin S T, Jiang H H 2010 Acta Opt. Sin. 30 849 (in Chinese) [张庆礼, 周文龙, 刘文鹏, 丁丽华, 罗建乔, 殷绍堂, 江海河 2010 光学学报 30 849]
[30] [31] Zang J C, Li X, Shan B R, Liu Y H, Liu Y L 2006 Chin. J. Lasers 33 565 (in Chinese) [臧竞存, 李晓, 单秉锐, 刘燕行, 刘玉龙 2006 中国激光 33 565]
[32] [33] Deloach L D, Stephen A. Payne, Larry K. Smith, Wayne L. Kway, William F. Krupke 1994 J. Opt. Soc. Am. B 11 269
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